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Related papers: Nonequilibrium RIXS study of an electron-phonon mo…

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In the past decade, Resonant Inelastic X-ray Scattering (RIXS) has made remarkable progress as a spectroscopic technique. This is a direct result of the availability of high-brilliance synchrotron X-ray radiation sources and of advanced…

Strongly Correlated Electrons · Physics 2012-12-03 Luuk J. P. Ament , Michel van Veenendaal , Thomas P. Devereaux , John P. Hill , Jeroen van den Brink

We present an exact Monte Carlo method to simulate the nonequilibrium dynamics of electron-phonon models in the adiabatic limit of zero phonon frequency. The classical nature of the phonons allows us to sample the equilibrium phonon…

Strongly Correlated Electrons · Physics 2022-02-16 Manuel Weber , James K. Freericks

We develop a formalism to calculate the L-edge resonant x-ray scattering (RIXS) spectra from transition-metal compounds. Using a multi-orbital tight-binding model, we derive useful formulas to calculate the spectra by collecting up the…

Strongly Correlated Electrons · Physics 2015-06-16 Jun-ichi Igarashi , Tatsuya Nagao

We study two-magnon excitations in resonant inelastic x-ray scattering (RIXS) at the transition-metal $K$-edge. Instead of working with effective Heisenberg spin models, we work with a Hubbard-type model ($d$-$p$ model) for a typical…

Strongly Correlated Electrons · Physics 2017-10-18 Takuji Nomura

We show that high resolution Resonant Inelastic X-ray Scattering (RIXS) provides direct, element-specific and momentum-resolved information on the electron-phonon (e-p) coupling strength. Our theoretical analysis demonstrates that the e-p…

Strongly Correlated Electrons · Physics 2012-12-03 Luuk J. P. Ament , Michel van Veenendaal , Jeroen van den Brink

Comprehending nonequilibrium electron-phonon dynamics at the microscopic level and at the short time scales is one of the main goals in condensed matter physics. Effective temperature models and time-dependent Boltzmann equations are…

Materials Science · Physics 2023-08-07 Nina Girotto , Fabio Caruso , Dino Novko

We present a novel derivation of resonant inelastic x-ray scattering (RIXS) which yields an expression for the RIXS cross section in terms of emission pathways between intermediate and final many-body states. Thereby electron-hole…

Materials Science · Physics 2020-10-14 Christian Vorwerk , Francesco Sottile , Claudia Draxl

We present a theoretical investigation of the origin of Raman-like and fluorescencelike (FL) features of resonant inelastic x-ray scattering (RIXS) spectra. Using a combination of local-density approximation + dynamical mean-field theory…

Strongly Correlated Electrons · Physics 2018-09-26 Atsushi Hariki , Mathias Winder , Jan Kuneš

Resonant inelastic X-ray scattering (RIXS) has become an important scientific tool. Nonetheless, conventional high-resolution RIXS measurements (<100 meV), especially in the soft x-ray range, require large and low-throughput grating…

Materials Science · Physics 2020-06-22 Daniel J. Higley , Hirohito Ogasawara , Sioan Zohar , Georgi L. Dakovski

We study resonant inelastic x-ray scattering (RIXS) peaks corresponding to low energy particle-hole excited states of metallic FeTe and semi-metallic TiSe$_2$ for photon incident energy tuned near the $L_{3}$ absorption edge of Fe and Ti…

Materials Science · Physics 2014-07-04 B. Barbiellini , J. N. Hancock , C. Monney , Y. Joly , G. Ghiringhelli , L. Braicovich , T. Schmitt

Resonant inelastic x-ray scattering (RIXS) tuned for the Cu L edge is a possible tool to detect charge excitations in cuprate superconductors. We theoretically investigate the possibility for observing a collective charge excitation by the…

Strongly Correlated Electrons · Physics 2015-08-03 Takami Tohyama , Kenji Tsutsui , Michiyasu Mori , Shigetoshi Sota , Seiji Yunoki

We calculate the resonant inelastic X-ray scattering (RIXS) response in a Mott insulator which is described by the Falicov-Kimball model. The model can be solved exactly within the single site dynamical mean-field theory (DMFT)…

Strongly Correlated Electrons · Physics 2015-03-31 Nandan Pakhira , J. K. Freericks , A. M. Shvaika

The coupled nonequilibrium dynamics of electrons and phonons in monolayer MoS2 is investigated by combining first-principles calculations of the electron-phonon and phonon-phonon interaction with the time-dependent Boltzmann equation.…

Materials Science · Physics 2021-02-12 Fabio Caruso

Resonant inelastic x-ray scattering (RIXS) is a well-established tool for studying electronic, nuclear and collective dynamics of excited atoms, molecules and solids. An extension of this powerful method to a time-resolved probe technique…

Chemical Physics · Physics 2015-11-03 Victor Kimberg , Nina Rohringer

We analyze the resonant x-ray scattering (RIXS) spectra from Sr$_2$IrO$_4$ in an itinerant electron approach. Employing a multi-orbital tight-binding model on the square lattice, we calculate the one-electron energy band within the…

Strongly Correlated Electrons · Physics 2015-06-22 Jun-ichi Igarashi , Tatsuya Nagao

The coupling between lattice vibration quanta and valence electrons can induce charge density modulations and decisively influence the transport properties of materials, e.g. leading to conventional superconductivity. In high critical…

We present two different theories for Raman scattering and Resonant Inelastic X-ray Scattering (RIXS) in the low temperature ferromagnetic phase of YTiO$_3$ and compare this to the available experimental data. For description of the orbital…

Strongly Correlated Electrons · Physics 2010-03-30 L. J. P. Ament , G. Khaliullin

We compute the K-edge indirect resonant inelastic x-ray scattering (RIXS) spectrum of a triangular lattice antiferromagnet in its ordered coplanar 3- sublattice 120 degree magnetic state. By considering the first order self$-$energy…

Materials Science · Physics 2015-07-07 Cheng Luo , Trinanjan Datta , Zengye Huang , Dao-Xin Yao

We develop a formalism to study the Resonant Inelastic X-ray Scattering (RIXS) response in metals based on the diagrammatic expansion for its cross section. The standard approach to the solution of the RIXS problem relies on two key…

Strongly Correlated Electrons · Physics 2019-11-20 A. M. Tsvelik , R. M. Konik , N. V. Prokof'ev , I. S. Tupitsyn

We determine the spin-exchange dynamical structure factor of the Heisenberg spin chain, as is measured by indirect Resonant Inelastic X-ray Scattering (RIXS). We find that two-spin RIXS excitations nearly entirely fractionalize into *two…

Strongly Correlated Electrons · Physics 2012-12-03 Antoine Klauser , Jorn Mossel , Jean-Sebastien Caux , Jeroen van den Brink