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We report on a systematic temperature dependent X-band electron paramagnetic resonance (EPR) study of nano-sized graphite particles prepared by ball-milling. In as-prepared samples a very intense and sharp EPR resonance at $g=2.0035$ has…

Strongly Correlated Electrons · Physics 2011-08-23 Jonas Kausteklis , Pavel Cevc , Denis Arcon , Lucia Nasi , Daniele Pontiroli , Marcello Mazzani , Mauro Ricco

We present gas-phase InfraRed Multiple Photon Dissociation (IRMPD) spectroscopy of cationic phenanthrene, pyrene, and perylene over the 100$-$1700 cm$^{-1}$ (6-95 $\mu$m) spectral range. This range covers both local vibrational modes…

Chemical Physics · Physics 2022-09-28 Sandra D. Wiersma , Alessandra Candian , Joost M. Bakker , Annemieke Petrignani

Using the weak-localization method, we have measured the electron-phonon scattering times $\tau_{ep}$ in Pd$_{60}$Ag$_{40}$ thick films prepared by DC- and RF-sputtering deposition techniques. In both series of samples, we find an anomalous…

Disordered Systems and Neural Networks · Physics 2009-05-05 Y. L. Zhong , J. J. Lin , L. Y. Kao

In this work, we study the development of a coplanar waveguide (CPW) resonator and its use in an electron spin resonance (ESR) spectrometer. The CPW resonator is designed to operate in S-band. It has a short circuit configuration which…

Applied Physics · Physics 2020-12-16 Subhadip Roy , Anuvab Nandi , Pronoy Das , Chiranjib Mitra

Rare-earth spin ensembles are a promising platform for microwave quantum memory applications due to their hyperfine transitions, which can exhibit exceptionally long coherence times when using an operation point with zero first-order Zeeman…

Films of metal-insulator nanogranular composites M$_x$D$_{100-x}$ with different composition and percentage of metal and dielectric phases (M = Fe, Co, CoFeB; D = Al$_2$O$_3$, SiO$_2$, LiNbO$_3$; x $\approx$ 15-70 at.%) are investigated by…

Materials Science · Physics 2023-12-12 A. B. Drovosekov , N. M. Kreines , D. A. Ziganurov , A. V. Sitnikov , S. N. Nikolaev , V. V. Rylkov

Multi-high-frequency electron paramagnetic resonance(EPR) spectrum for a supermolecular dimer $[ Mn_4]_2$ of single-molecule magnets recently reported [S. Hill, R. S. Edwards, N. Aliaga-Alcalde and G. Christou(HEAC), Science 302, 1015…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Xu Chang-Tan , Liang J-Q

Porous silica materials offer wide range of possibilities for enhancement of the productivity of oil reservoirs. However the mechanism of adsorption of polar components of crude oil on silica surface is poorly understood that hinders…

We present the experimental InfraRed Multiple Photon Dissociation (IRMPD) spectrum and fragmentation mass spectrum of the irregular, cationic PAH dibenzo[a,l]pyrene (C$_{24}$H$_{14}^+$) in the 6-40 $\mu$m / 250-1650 cm$^{-1}$ range. The use…

While several 2D thermometry techniques exist, there is a lack of 3D thermometry techniques that work for wide range of materials and offer good resolution in time, space and temperature. X-ray diffraction (XRD) and nuclear magnetic…

Materials Science · Physics 2023-01-19 Darshan Chalise , David G. Cahill

Paramagnetic centers in a solid-state environment usually give rise to inhomogenously broadened electron paramagnetic resonance (EPR) lines, making conventionally detected free induction decay (FID) signals disappear within the spectrometer…

We employ electron paramagnetic resonance (EPR) of the spin probe Mn2+ to study the paraelectric ferroelectric transition in DMAMnF and Mn2 doped DMZnF, which are considered to be model metal organic frameworks (MOF) with a Pb free…

Materials Science · Physics 2022-02-25 Nandita Abhyankar , Sylvain Bertaina , Maylis Orio , Naresh Dalal

The development of a new era of quantum devices requires an understanding of how paramagnetic dopants or impurity spins behave in crystal hosts. Here, we describe a new spectroscopic technique which uses traditional Electron Spin Resonance…

Simultaneous monitoring of ac and dc responses of the electrode-electrolyte interface with potentiodynamic electrochemical impedance spectroscopy (PDEIS) in silver underpotential and overpotential deposition on platinum has confirmed the…

Materials Science · Physics 2007-05-23 Genady Ragoisha , Alexander Bondarenko

Electron paramagnetic resonance (EPR) study of air-physisorbed defective carbon nano-onions evidences in favor of microwave assisted formation of weakly-bound paramagnetic complexes comprising negatively-charged O2- ions and edge carbon…

Mesoscale and Nanoscale Physics · Physics 2016-06-10 D. W. Boukhvalov , V. Yu. Osipov , A. I. Shames , K. Takai , T. Hayashi , T. Enoki

We present pulsed electrically detected magnetic resonance (EDMR) measurements at low magnetic fields using posphorus-doped silicon with natural isotope composition as a model system. Our measurements show that pulsed EDMR experiments, well…

Materials Science · Physics 2015-06-23 L. Dreher , F. Hoehne , H. Morishita , H. Huebl , M. Stutzmann , K. M. Itoh , M. S. Brandt

We report the results and unique instrument configuration of a novel experiment in which we successfully transitioned a DPPH sample from its natural paramagnetic state and essentially a non-magnetic material to a ferromagnetic state at room…

We report on terahertz (THz) electron paramagnetic resonance generalized spectroscopic ellipsometry (THz-EPR-GSE). Measurements of the field and frequency dependencies of the magnetic response due to the spin transitions associated with the…

We describe a pulsed multi-frequency electron paramagnetic resonance spectrometer operating at several frequencies in the range of 110-336 GHz. The microwave source at all frequencies consists of a multiplier chain starting from a solid…

Quantum Physics · Physics 2008-12-01 Gavin W. Morley , Louis-Claude Brunel , Johan van Tol

We present an alternative to conventional Electron Paramagnetic Resonance (EPR) spectroscopy equipment. Avoiding the use of bulky magnets and magnetron equipment, we use the photoluminescence of an ensemble of Nitrogen-Vacancy centers at…

Applied Physics · Physics 2023-03-08 C. Mignon , A. R. Ortiz Moreno , H. Shirzad , S. K. Padamati , V. Damle , Y. Ong , R. Schirhagl , M. Chipaux