Related papers: Characterizing the Zeeman slowing force for $^{40}…
Multistage Zeeman deceleration is a technique used to reduce the velocity of neutral molecules with a magnetic dipole moment. Here we present a Zeeman decelerator that consists of 100 solenoids and 100 magnetic hexapoles, that is based on a…
We present the properties of a magneto-optical trap (MOT) of CaF molecules. We study the process of loading the MOT from a decelerated buffer-gas-cooled beam, and how best to slow this molecular beam in order to capture the most molecules.…
We demonstrate and characterize Zeeman-Sisyphus (ZS) deceleration of a beam of ytterbium monohydroxide (YbOH). Our method uses a combination of large magnetic fields ($\sim$ 2.5 T) and optical spin-flip transitions to decelerate molecules…
The fast component of the barium fluoride (BaF$_{2}$) crystal luminescence with the emission peak at 220 nm allows those crystals to be employed in fast calorimeters operating in harsh radiation environment. However, the slow component with…
We demonstrate rapid loading of a magneto-optical trap (MOT) of cadmium atoms from a pulsed cryogenic helium buffer gas beam, overcoming strong photoionization losses. Using the $ ^1S_0 \rightarrow{} ^1P_1 $ transition at 229 nm, we capture…
The article presents the development of a new and innovative experimental method to fully characterize a solenoidal "spin-flip" Zeeman slower (ZS) using a Quartz Crystal $\mu$-balance (QCM) as a kinetic energy sensor. In this experiment, we…
Direct laser cooling of molecules has made significant progress in recent years. However, the selective cooling and manipulation of molecules based on their isotopic composition, which is ubiquitous in atomic laser cooling, has not yet been…
We report an experimental investigation on the Doppler-free saturated absorption spectroscopy of buffer-gas-cooled Barium monofluoride (BaF) molecules in a 4~K cryogenic cell. The obtained spectra with a resolution of 19~MHz, much smaller…
Strong optical forces with minimal spontaneous emission are desired for molecular deceleration and atom interferometry applications. We report experimental benchmarking of such a stimulated optical force driven by ultrafast laser pulses. We…
We demonstrate laser cooling of barium monofluoride (138BaF) molecules. We use serrodynes to synthesize time-sequenced optical spectra that can be precisely tailored to the hyperfine structure of this heaviest non-radioactive alkaline earth…
We propose a new method to cool gaseous samples of neutral atoms. The gas is confined in a non dissipative optical trap in the presence of an homogeneous magnetic field. The method accumulates atoms in the $m_F=0$ Zeeman sub-level. Cooling…
Slow beams of neutral molecules are of great interest for a wide range of applications, from cold chemistry through precision measurements to tests of the foundations of quantum mechanics. We report on the quantitative observation of…
For laser cooling considerations, we have theoretically investigated the electronic, rovibrational and hypefine structures of BaF molecule. The highly diagonal Franck-Condon factors and the branching ratios for all possible transitions…
We present a compact design of dual-beam Zeeman slower optimized for efficient production of cold atom applications. Traditional single-beam configurations face challenges from substantial residual atomic flux impacting downstream optical…
We propose a scheme for direct laser deceleration of molecules based on a vibrational transition-mediated bichromatic force (VBCF). By precisely engineering mid-infrared optical fields, we establish coherent absorption-stimulated emission…
We present the first crossed beam scattering experiment using a Zeeman decelerated molecular beam. The narrow velocity spreads of Zeeman decelerated NO ($X ^2\Pi_{3/2}, j=3/2$) radicals result in high-resolution scattering images, thereby…
We realize the first Zeeman slower of an atom in the Main Group III of the periodic table, otherwise known as the "triel elements". Despite that our atom of choice (namely indium) does not have a ground state cycling transition suitable for…
Decoupling of total electronic and nuclear spin moments of Cs atoms in external magnetic field for the case of atomic $D_1$ line, leading to onset of the hyperfine Paschen-Back regime has been studied theoretically and experimentally.…
Ultracold polar molecules are promising for quantum information processing and searches for physics beyond the Standard Model. Laser cooling to ultracold temperatures is an established technique for trapped diatomic and triatomic molecules.…
We demonstrate a combination of an isotopically purified atom beam and a magneto-optical trap which enables the single atom detection of all stable isotopes of calcium (40, 42, 43, 44, 46 and 48). These isotopes range in abundance from 96.9…