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We report the Stark deceleration of CaF molecules in the strong-field seeking ground state and in a weak-field seeking component of a rotationally-excited state. We use two types of decelerator, a conventional Stark decelerator for the…

Atomic Physics · Physics 2017-09-13 T. E. Wall , J. F. Kanem , J. M. Dyne , J. J. Hudson , B. E. Sauer , E. A. Hinds , M. R. Tarbutt

Calcium monofluoride (CaF) molecules are loaded into an optical dipole trap (ODT) and subsequently laser cooled within the trap. Starting with magneto-optical trapping, we sub-Doppler cool CaF and then load $150(30)$ CaF molecules into an…

Zeeman deceleration is a relatively new technique used to obtain full control over the velocity of paramagnetic atoms or molecules in a molecular beam. We present a detailed description of a multistage Zeeman decelerator that has recently…

Atomic Physics · Physics 2019-01-15 Theo Cremers , Niek Janssen , Edwin Sweers , Sebastian Y. T. van de Meerakker

We demonstrate a scheme for optical cycling in the polar, diatomic molecule strontium monofluoride (SrF) using the $X ^2\Sigma^+\toA^2\Pi_{1/2}$ electronic transition. SrF's highly diagonal Franck-Condon factors suppress vibrational…

Atomic Physics · Physics 2015-05-14 E. S. Shuman , J. F. Barry , D. R. Glenn , D. DeMille

In order to realize more sensitive eEDM measurement, it would be worthwhile to find some new laser-cooled molecules with larger internal effective electric field (E$_{eff}$), higher electric polarizability and longer lifetime of the eEDM…

Atomic Physics · Physics 2019-03-13 Zhenghai Yang , Jing Li , Qinning Lin , Liang Xu , Hailing Wang , Tao Yang , Jianping Yin

We investigated the optical cycling effect of the $\mathrm{X}^2\Sigma(v=0,\ N=1^-) - \mathrm{A}^2\Pi_{1/2}(v'=0,\ J'=1/2^+)$ band of MgF molecules, specifically the $\mathrm{P_1/Q_{12}(1)}$ transition, which serves as the main transition in…

Atomic and Molecular Clusters · Physics 2025-07-08 Kikyeong Kwon , Seunghwan Roh , Youngju Cho , Yongwoong Lee , Eunmi Chae

A cryogenic buffer gas beam, an electrostatic hexapole lens, and 2D transverse Doppler laser cooling are combined to produce a bright beam of barium monofluoride ($^{138}$Ba$^{19}$F) molecules. Experimental results and trajectory…

A supersonic beam of metastable neon atoms has been decelerated by exploiting the interaction between the magnetic moment of the atoms and time-dependent inhomogeneous magnetic fields in a multistage Zeeman decelerator. Using 91…

We present the first experimental demonstration of radiation pressure force deflection and direct laser cooling for barium monohydride (BaH) molecules resulting from multiple photon scattering. Despite a small recoil velocity (2.7 mm/s) and…

A transverse Zeeman slower composed of an array of compact discrete neodymium magnets is considered. A simple and precise model of such a slower based on magnetic dipoles is developed. The theory of a general Zeeman slower is modified to…

Atomic Physics · Physics 2009-11-13 Yuri B. Ovchinnikov

We describe a simple Zeeman slower design using permanent magnets. Contrary to common wire-wound setups no electric power and water cooling are required. In addition, the whole system can be assembled and disassembled at will. The magnetic…

A full density-matrix simulation is performed for optical deflection of a barium monofluoride ($^{138}$Ba$^{19}$F) beam using the bichromatic force, which employs pairs of counter-propagating laser beams that are offset in frequency. We…

Atomic Physics · Physics 2023-07-26 A. Marsman , M. Horbatsch , E. A. Hessels

A full density-matrix simulation is performed for optical deflection of a barium monofluoride (BaF) beam. Pairs of counter-propagating laser pulses are used for stimulated absorption followed by stimulated emission. The scheme produces a…

Atomic Physics · Physics 2023-01-18 A. Marsman , D. Heinrich , M. Horbatsch , E. A. Hessels

We present the design, construction, and characterisation of longitudinal- and transverse-field Zeeman slowers, based on arrays of permanent magnets, for slowing thermal beams of atomic Sr. The slowers are optimised for operation with…

Atomic Physics · Physics 2015-06-18 Ian R. Hill , Yuri B. Ovchinnikov , Elizabeth M. Bridge , E. Anne Curtis , Patrick Gill

We propose and demonstrate a novel technique that combines Raman scattering and optical cycling in molecules with diagonal Franck-Condon factors. This resonance Raman optical cycling manipulates molecules to behave like efficient…

Atomic Physics · Physics 2021-08-26 J. C. Shaw , J. C. Schnaubelt , D. J. McCarron

We theoretically and experimentally investigate nonlinear Zeeman effects within a polarised single-photon source that uses a single 87Rb atom strongly coupled to a high finesse optical cavity. The breakdown of the atomic hyperfine structure…

Quantum Physics · Physics 2018-08-15 Thomas D. Barrett , Dustin Stuart , Oliver Barter , Axel Kuhn

Since the advent of atom laser-cooling, trapping or cooling natural molecules has been a long standing and challenging goal. Here, we demonstrate a method for laser-trapping molecules that is radically novel in its configuration, in its…

Optics · Physics 2015-06-04 M. Alharbi , A. Husakou , B. Debord , F. Gerome , F. Benabid

We study collisions of ultracold CaF molecules in strong static electric fields. These fields allow the creation of long-range barriers in the interaction potential, effectively preventing the molecules from reaching the short-range region…

We present experimental results that demonstrate - for the first time - the Zeeman deceleration of helium atoms in the metastable 2^3S_1state. A more than 40% decrease of the kinetic energy of the beam is achieved for deceleration from 490…

Atomic Physics · Physics 2015-06-23 Katrin Dulitz , Atreju Tauschinsky , Timothy P Softley

We demonstrate the effect of Zeeman and hyperfine optical pumping and transverse laser cooling of a dysprosium (Dy) atomic beam on the $4f^{10}6s^2(J = 8) \rightarrow 4f^{10}6s6p(J = 9)$ transition at 421.291 nm. For $^{163}$Dy, an…

Atomic Physics · Physics 2026-02-09 Rohan Chakravarthy , Jonathan Agil , Arijit Sharma , Jung Bog Kim , Dmitry Budker