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A new theoretical approach to the description of the attosecond streaking measurements of atomic photoionization is presented. It is a fully quantum mechanical description based on numerical solving of the time-dependent Schroedinger…

Atomic Physics · Physics 2007-05-23 A. K. Kazansky , N. M. Kabachnik

Understanding initial electron thermalization has relevance to both fundamental scientific knowledge and application to the construction of novel devices. In this study, attosecond transient absorption is used to directly measure initial…

Materials Science · Physics 2024-06-07 Bethany R. de Roulet , Lorenz Drescher , Shunsuke A. Sato , Stephen R. Leone

Tunnelling, one of the key features of quantum mechanics, ignited an ongoing debate about the value, meaning and interpretation of 'tunnelling time'. Until recently the debate was purely theoretical, with the process considered to be…

As the simplest atomic system, the hydrogen atom plays a key benchmarking role in laser and quantum physics. Atomic hydrogen is a widely used atomic test system for theoretical calculations of strong-field ionization, since approximate…

Atomic Physics · Physics 2014-03-27 D. Kielpinski , R. T. Sang , I. V. Litvinyuk

We present experimental data on the non-adiabatic strong field ionization of atomic hydrogen using elliptically polarized femtosecond laser pulses at a central wavelength of 390 nm. Our measured results are in very good agreement with a…

The last decade has seen an intense renewed debate on tunnelling time, both from a theoretical and an experimental perspective. Here, we review recent developments and new insights in the field of strong-field tunnel ionization related to…

Atomic Physics · Physics 2019-04-26 C. Hofmann , A. S. Landsman , U. Keller

We perform a detailed analysis of how high-order harmonic generation (HHG) and above-threshold ionization (ATI) can be controlled by a time-delayed attosecond-pulse train superposed to a strong, near-infrared laser field. In particular we…

Atomic Physics · Physics 2009-11-11 C. Figueira de Morisson Faria , P. Salieres , P. Villain , M. Lewenstein

We analyze the attosecond electron dynamics in hydrogen molecular ion driven by an external intense laser field using ab-initio numerical simulations of the corresponding time-dependent Schr{\"{o}}dinger equation and Bohmian trajectories.…

Chemical Physics · Physics 2015-05-20 Norio Takemoto , Andreas Becker

Ultrashort electron pulses are crucial for time-resolved electron diffraction and microscopy of fundamental light-matter interaction. In this work, we study experimentally and theoretically the generation and characterization of attosecond…

Optics · Physics 2018-03-21 Yuya Morimoto , Peter Baum

Plasmonic catalysis is a rapidly growing field of research, both from experimental and computational perspectives. Experimental observations demonstrate an enhanced dissociation rate for molecules in the presence of plasmonic nanoparticles…

Chemical Physics · Physics 2025-12-18 Natalia E. Koval , J. Iñaki Juaristi , Maite Alducin

We study single-photon ionization of aligned H$_2^+$ in a high-frequency low-intensity laser field. We focus on the case where the laser frequency is not far larger than the ionization potential of the target. The calculated photoelectron…

Atomic Physics · Physics 2022-12-02 F. B. Zhang , J. Y. Che , W. Y. Li , C. Chen , Y. J. Chen

Attosecond interferometry in a two-color field is central to attosecond metrology and spectroscopy. In this technique, a photoelectron wave packet is released when a single photon from an extreme ultraviolet comb is absorbed. The wave…

In our model the electron dynamics are described by a two-state approximation. This might appear a rough approximation since it neglects coupling through excited electronic states and ionization channels. However at high intensity (laser…

Atomic Physics · Physics 2007-05-23 J F McCann , Liang-You Peng , I D Williams

In the recent work of Herath et al. [Phys. Rev. Lett. 109, 043004 (2012)] the first experimental observation of a dependence of strong-field ionization rate on the sign of the magnetic quantum number m (of the initial bound state (n,l.m))…

Atomic Physics · Physics 2015-06-23 J. H. Bauer , Francisca Mota-Furtado , Patrick F. O'Mahony , Bernard Piraux , K. Warda

Several recent attoclock experiments have investigated the fundamental question of a quantum mechanically induced time delay in tunneling ionization via extremely precise photoelectron momentum spectroscopy. The interpretations of those…

The dynamics of atomic levels resonantly coupled by a coherent and intense short high-frequency laser pulse is discussed and it is advocated that this dynamics is sensitively probed by measuring the spectra of the particles emitted. It is…

Atomic and Molecular Clusters · Physics 2013-01-11 Philipp V. Demekhin , Lorenz S. Cederbaum

In strong-field physics and attosecond science, intense light induces ultrafast electron dynamics. Such ultrafast dynamics of electrons in matter is at the core of phenomena such as high harmonic generation (HHG), where these dynamics lead…

Using extreme-ultraviolet attosecond-pulse-trains, we investigate the photoionization dynamics of a Helium atom in the presence of moderately-strong (~10^12 W/cm^2) femtosecond laser pulses. The electronic structure of a laser-dressed atom…

Atomic Physics · Physics 2011-08-02 Niranjan Shivaram , Henry Timmers , Xiao-Min Tong , Arvinder S. Sandhu

Attosecond chemistry involves developing strategies to manipulate electronic coherent waves in molecules, which can influence the outcome of photoinduced reactions. While recent progress in this field calls for investigations of…

Chemical Physics · Physics 2026-04-22 Evan Munaro-Langloÿs , Franck Lépine , Victor Despré

Strong-field phenomena driven by an intense infrared (IR) laser depend on during what part of the field cycle they are initiated. By changing the sub-cycle character of the laser electric field it is possible to control such phenomena. For…