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Time-resolved investigations of ultrafast electronic and molecular dynamics were not possible until recently. The typical time scale of these processes is in the picosecond to attosecond realm. The tremendous technological progress in…

Atomic Physics · Physics 2013-05-14 Stefan Pabst

Interferometry, as the key technique in modern precision measurements, has been used for length diagnosis in the fields of engineering metrology and astronomy. Analogous interferometric technique for time domain precision measurement is a…

Optics · Physics 2019-11-15 Zhen Yang , Wei Cao , Yunlong Mo , Huiyao Xu , Kang Mi , Pengfei Lan , Qingbin Zhang , Peixiang Lu

We propose the scheme of temporal double-slit interferometer to precisely measure the electric field of shaped intense femtosecond laser pulse directly, and apply it to control the electron tunneling wave packets in attosecond precision. By…

Atomic Physics · Physics 2023-11-13 Xiaoyun Zhao , Mingqing Liu , Yizhang Yang , Zhou Chen , Xiaolei Hao , Chuncheng Wang , Weidong Li , Jing Chen

Solids exposed to intense electric fields release electrons through tunnelling. This fundamental quantum process lies at the heart of various applications, ranging from high brightness electron sources in DC operation to petahertz vacuum…

The electric field governing the dynamics of space charge produced by high intensity femtosecond laser pulses focused on a copper surface is investigated by time-resolved low-energy-electron-scattering. The pump-probe experiment has a…

Materials Science · Physics 2009-11-13 C. Cirelli , M. Hengsberger , A. Dolocan , H. Over , J. Osterwalder , T. Greber

Transition metals with their densely confined and strongly coupled valence electrons are key constituents of many materials with unconventional properties, such as high-Tc superconductors, Mott insulators and transition-metal…

Atomic Physics · Physics 2020-01-08 M. Volkov , S. A. Sato , F. Schlaepfer , L. Kasmi , N. Hartmann , M. Lucchini , L. Gallmann , A. Rubio , U. Keller

Nonlocal potential models have been used in place of the Coulomb potential in the Schrodinger equation as an efficient means of exploring high field laser-atom interaction in previous works. Al- though these models have found use in…

Atomic Physics · Physics 2016-12-21 T. C. Rensink , T. M. Antonsen

Attosecond spectroscopy of materials has provided invaluable insight into light-driven coherent electron dynamics. However, attosecond spectroscopies have so far been focused on weakly-correlated materials. As a result, the behavior of…

Phase and time delays of atomic above-threshold ionization were recently experimentally explored in an $\omega -2\omega$ setting [Zipp et al, Optica 1, 361 (2014)]. The phases of wavepackets ejected from argon by a strong $2\omega$ pulse…

Atomic Physics · Physics 2022-11-23 Diego G. Arbó , Sebastián D. López , Joachim Burgdörfer

Previous attoclock experiments measuring the photoelectron momentum distribution (PMD) via strong-field ionization in an elliptically polarized laser field have shown anomalously large offset angles in the nonadiabatic regime with large…

Atomic Physics · Physics 2025-01-22 Q. Z. Lv , M. Klaiber , P. -L. He , K. Z. Hatsagortsyan , C. H. Keitel

Attosecond streaking of photoelectrons emitted by extreme ultraviolet light has begun to reveal how electrons behave during their transport within simple crystalline solids. Many sample types within nanoplasmonics, thin-film physics, and…

Attosecond science is based on steering of electrons with the electric field of well-controlled femtosecond laser pulses. It has led to, for example, the generation of XUV light pulses with a duration in the sub-100-attosecond regime, to…

Quantum Physics · Physics 2011-07-11 Michael Krüger , Markus Schenk , Peter Hommelhoff

By performing a joint theoretical and experimental investigation on the high-order above-threshold ionization (HATI) spectrum, the dominant role of the 3rd-return-recollision trajectories in the region near the cutoff due to the ionic…

This perspective introduces attosecond path qubits: measurement-defined two-level subsystems that arise naturally in strong-field physics from the coherent interference of distinguishable quantum pathways. These effective qubits are…

Optics · Physics 2026-01-14 Oren Cohen

We study laser-assisted photoionization by attosecond pulses using a time-independent formalism based on diagrammatic many-body perturbation theory. Our aim is to provide an ab inito route to the "delays" for this above-threshold ionization…

Atomic Physics · Physics 2015-06-12 J. M. Dahlström , T. Carette , E. Lindroth

Recent advances in strong x-ray laser techniques enable the study of nonlinear multiphoton ionization in extreme high-frequency fields. Although the stabilization regime in such fields is theoretically established, its modified properties…

Atomic Physics · Physics 2026-02-17 Aleksandr V. Boitsov , Karen Z. Hatsagortsyan , Christoph H. Keitel

Time-resolved photoelectron spectroscopy provides access to the electronic structure and non-equilibrium electron dynamics in matter. At solid surfaces photoemission dynamics can be investigated on its natural time scale by measuring…

Coherent processing of quantum information and attosecond science had so far little in common. We here show that recent data in high harmonic emission reveal quantum information processing at the attosecond timescale. By observing the…

Atomic Physics · Physics 2014-07-02 I. K. Kominis , G. Kolliopoulos , D. Charalambidis , P. Tzallas

We study strong-field molecular ionization as a function of pulse duration. Experimental measurements of the photoelectron yield for a number of molecules reveal competition between different ionization continua (cationic states) which…

We develop an analytical model of correlated two-electron ionization in strong infrared laser fields. The model includes all relevant interactions between the electrons, the laser field, and the ionic core nonperturbatively. We focus on the…

Atomic Physics · Physics 2009-02-14 Denys I. Bondar , Wing-Ki Liu , Misha Yu. Ivanov