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We explore the crystallization in a colloidal monolayer on a structured template starting from a few-particle nucleus. The competition between the substrate structure and that of the growing crystal induces a new crystal growth scenario.…

Soft Condensed Matter · Physics 2013-07-09 Tim Neuhaus , Michael Schmiedeberg , Hartmut Löwen

Modulating liquid-to-solid transitions and the resulting crystalline structure for tailored properties is much desired. Colloidal systems are exemplary to this end, but the fundamental knowledge gaps in relating the influence of…

Statistical Mechanics · Physics 2025-11-04 Porhouy Minh , Steven W. Hall , Ryan S. DeFever , Sapna Sarupria

In a recent class of phase field crystal (PFC) models, the density order parameter is coupled to powers of its mean field. This effectively introduces a phenomenology of higher-order direct correlation functions acting on long wavelengths,…

Materials Science · Physics 2024-08-21 Daniel L. Coelho , Duncan Burns , Emily Wilson , Nikolas Provatas

The critical dynamics of dislocation avalanches in plastic flow is examined using a phase field crystal (PFC) model. In the model, dislocations are naturally created, without any \textit{ad hoc} creation rules, by applying a shearing force…

Materials Science · Physics 2010-06-14 Pak Yuen Chan , Georgios Tsekenis , Jonathan Dantzig , Karin A. Dahmen , Nigel Goldenfeld

The crystal plasticity finite element method (CPFEM) is used to investigate the coupling between the cylindrical void growth or collapse and grain refinement in face-centered cubic (FCC) single crystals. A 2D plane strain model with one…

Materials Science · Physics 2023-07-06 Saketh Virupakshi , Katarzyna Kowalczyk-Gajewska

A new model of crystal growth is presented that describes the phenomena on atomic length and diffusive time scales. The former incorporates elastic and plastic deformation in a natural manner, and the latter enables access to times scales…

Materials Science · Physics 2009-11-07 K. R. Elder , Mark Katakowski , Mikko Haataja , Martin Grant

Crystal nucleation and growth processes induced by an externally applied shear strain in a model metallic glass are studied by means of nonequilibrium molecular dynamics simulations, in a range of temperatures. We observe that the…

Materials Science · Physics 2010-09-30 Anatolii Mokshin , J. -L. Barrat

Complex crystal structures are composed of multiple local environments, and how this type of order emerges spontaneously during crystal growth has yet to be fully understood. We study crystal growth across various structures and along…

Soft Condensed Matter · Physics 2024-06-03 Maya M. Martirossyan , Matthew Spellings , Hillary Pan , Julia Dshemuchadse

The search for effective methods to fabricate bulk single-phase quasicrystalline Al-Cu-Fe alloys is currently an important task. Crucial to solving this problem is to understand mechanisms of phase formation in this system. Here we study…

Chemical Physics · Physics 2020-01-08 L. V. Kamaeva , I. V. Sterkhova , V. I. Ladyanov , R. E. Ryltsev , N. M. Chtchelkatchev

Dendritic growth, and the formation of material microstructure in general, necessarily involves a wide range of length scales from the atomic up to sample dimensions. The phase field approach of Langer, enhanced by optimal asymptotic…

Materials Science · Physics 2015-06-25 Nigel Goldenfeld , Badrinarayan P. Athreya , Jonathan A. Dantzig

We carry out molecular dynamics (MD) and Monte Carlo (MC) simulations to characterize nucleation in liquid clusters of 600 Lennard-Jones particles over a broad range of temperatures. We use the formalism of mean first-passage times to…

Materials Science · Physics 2016-10-05 Shahrazad M. A. Malek , Gregory P. Morrow , Ivan Saika-Voivod

Nucleation is an activated process in which the system has to overcome a free energy barrier in order for a first-order phase transition between the metastable and the stable phases to take place. In the liquid-to-solid transition the…

Soft Condensed Matter · Physics 2016-11-28 John Russo , Hajime Tanaka

Using Monte Carlo simulations we study crystallization in the three-dimensional Ising model with four-spin interaction. We monitor the morphology of crystals which grow after placing crystallization seeds in a supercooled liquid. Defects in…

Materials Science · Physics 2009-11-07 A. Lipowski , D. Johnston

We introduce a non-isothermal phase-field crystal model including heat flux and thermal expansion of the crystal lattice. The thermal compatibility condition, as well as a positive entropy-production property, is derived analytically and…

Materials Science · Physics 2025-01-23 Maik Punke , Marco Salvalaglio , Axel Voigt , Steven M. Wise

In this work, we study the crystalline nuclei growth in glassy systems focusing primarily on the early stages of the process, at which the size of a growing nucleus is still comparable with the critical size. On the basis of molecular…

Disordered Systems and Neural Networks · Physics 2017-04-10 Anatolii V. Mokshin , Bulat N. Galimzyanov

We determine the full kinetic phase diagram for nucleation and growth of crystal phases in a suspension of charged colloids. We calculate nucleation barrier heights for face-centered cubic (fcc) and body-centered cubic (bcc) crystal phases…

Soft Condensed Matter · Physics 2022-08-31 Willem Gispen , Marjolein Dijkstra

Crucial to gaining control over crystallisation in multicomponent materials or accurately modelling rheological behaviour of magma flows is to understand the mechanisms by which crystal nuclei form. The microscopic nature of such nuclei,…

Soft Condensed Matter · Physics 2019-08-07 Trond S. Ingebrigtsen , Jeppe C. Dyre , Thomas B. Schrøder , C. Patrick Royall

An eutectic LiCl/KCl flux method in a horizontal configuration has been used to grow a series of homogeneous Fe$_{1+\delta}$Se$_{1-x}$Te$_x$ single crystals of high quality with 0.5 $\leq$ $x$ $\leq$ 1. Compared with previously used…

The properties of welded components are dominated by the microstructure evolution in the pool, where the solidification conditions are space-time variational. To represent the variational solidification conditions in the pool, the…

Materials Science · Physics 2022-09-16 Fengyi Yu , Yanhong Wei , Qiaodan Hu , Jianguo Li

A novel analysis of homogeneous nucleation of dislocations in sheared two-dimensional crystals described by periodized discrete elasticity models is presented. When the crystal is sheared beyond a critical strain $F=F_{c}$, the strained…

Materials Science · Physics 2008-05-09 I. Plans , A. Carpio , L. L. Bonilla
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