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The energy acquisition based on resonant excitations are of great importance in chemical and biological systems. Here, the intramolecular resonant absorption of polarized mid-infrared pulses by bulk water and surface water is investigated…

Mesoscale and Nanoscale Physics · Physics 2022-02-16 Rong-Yao Yang , Wei-Zhou Jiang , Pei-Ying Huo

The optical absorption spectrum of the three most stable isomers of the Ag11 system was calculated using the time-dependent density functional theory, with the generalized gradient approximation for the exchange and correlation potential,…

Atomic and Molecular Clusters · Physics 2009-11-13 Jose I. Martinez , Eva M. Fernandez

The x-ray absorption spectra of water and ice are calculated with a many-body approach for electron-hole excitations. The experimental features, including the small effects of temperature change in the liquid, are quantitatively reproduced…

Soft Condensed Matter · Physics 2015-05-14 Wei Chen , Xifan Wu , Roberto Car

By measuring the transmission of near-resonant light through an atomic vapor confined in a nano-cell we demonstrate a mesoscopic optical response arising from the non-locality induced by the motion of atoms with a phase coherence length…

Helicenes, a class of organic molecules consisting of ortho-fused benzene rings in a spring-like configuration have found several interesting applications in nonlinear optical materials and opto-electronic devices. Under the action of…

Chemical Physics · Physics 2023-03-08 Veera Sundararaghavan , Vikas Varshney , Davide Simone

Epitaxially-grown quantum well and quantum dot solar cells suffer from weak light absorption, strongly limiting their performance. Light trapping based on optical resonances is particularly relevant for such devices to increase light…

Applied Physics · Physics 2023-11-10 Maxime Giteau , Yusuke Oteki , Kento Kitahara , Naoya Miyashita , Ryo Tamaki , Yoshitaka Okada

We demonstrate a large light absorptance (80%) in a nanometric layer of quantum dots in rods (QRs) with a thickness of 23 nm. This behavior is explained in terms of the coherent absorption by interference of the light incident at a certain…

The optical spectrum of liquid water is analyzed by subsystem time-dependent density functional theory. We provide simple explanations for several important (and so far elusive) features. Due to the disordered environment surrounding each…

Materials Science · Physics 2017-06-23 Sudheer Kumar P. , Michele Pavanello

We analyze optical soliton propagation in the presence of weak absorption lines with much narrower linewidths as compared to the soliton spectrum width using the novel perturbation analysis technique based on an integral representation in…

Optics · Physics 2010-03-25 V. L. Kalashnikov , E. Sorokin

We demonstrate that variations in molecular chemisorption energy on different metals, different surface terminations, and different strain conditions can be accounted for by orbital-specific changes in the substrate electronic structure.…

Materials Science · Physics 2007-05-23 Sara E. Mason , Ilya Grinberg , Andrew M. Rappe

The possibility of spatially resolving the optical properties of atomically thin materials is especially appealing as they can be modulated at the micro- and nanoscale by reducing their thickness, changing the doping level or applying a…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 Andres Castellanos-Gomez , Jorge Quereda , Herko P. van der Meulen , Nicolás Agraït , Gabino Rubio-Bollinger

We report on a survey for associated HI 21-cm and OH 18-cm absorption with the Giant Metrewave Radio Telescope at redshifts z = 0.2-0.4. Although the low redshift selection ensures that our targets are below the critical ultra-violet…

Astrophysics of Galaxies · Physics 2017-03-29 S. J. Curran , M. T. Whiting , J. R. Allison , A. Tanna E. M. Sadler , R. Athreya

UV ice photodesorption is an important non-thermal desorption pathway in many interstellar environments that has been invoked to explain observations of cold molecules in disks, clouds and cloud cores. Systematic laboratory studies of the…

A new method for calculating optical absorption spectra within linear-scaling density-functional theory (LS-DFT) is presented, incorporating a scheme for optimizing a set of localized orbitals to accurately represent unoccupied Kohn-Sham…

Materials Science · Physics 2015-05-30 Laura E. Ratcliff , Nicholas D. M. Hine , Peter D. Haynes

We have made radio- and millimeter-wavelength interferometric observations of a variety of molecular absorption lines toward the gravitational lens systems B0218+357 and PKS1830-211. The absorption occurs in the lensing galaxies at…

Astrophysics · Physics 2007-05-23 Karl M. Menten , Christopher L. Carilli , Mark J. Reid

We report on very high enhancement of thin layer's absorption through band-engineering of a photonic crystal structure. We realized amorphous silicon (aSi) photonic crystals, where slow light modes improve absorption efficiency. We show…

Silicon p-n junction diodes emit low-intensity, broad-spectrum light near 1120 nm in forward bias and between 400-900 nm in reverse bias (avalanche). For the first time, we experimentally achieve optical absorption sensing of pigment in…

Optics · Physics 2020-12-15 Satadal Dutta , Peter G. Steeneken , Gerard J. Verbiest

The time-of-flight method is a fundamental approach for characterizing the transport properties of semiconductors. Recently, the transient photocurrent and optical absorption kinetics have been simultaneously measured for thin films;…

Chemical Physics · Physics 2023-03-21 Kazuhiko Seki , Naoya Muramatsu , Tomoaki Miura , Tadaaki Ikoma

Effects of coupling between an molecular exciton and a surface plasmon (exciton-plasmon coupling) on the luminescence properties of the molecule and the surface plasmons are investigated using nonequilibrium Green's function method.…

Materials Science · Physics 2013-11-12 Kuniyuki Miwa , Mamoru Sakaue , Hideaki Kasai

Due to its low symmetry, $\beta$-Ga$_{2}$O$_{3}$ exhibits a strongly anisotropic optical response. As a result, the absorption spectra change with the polarization state of the incoming photons. To understand this phenomenon, here we…

Materials Science · Physics 2024-07-02 Md Mohsinur Rahman Adnan , Darpan Verma , Chris Sturm , Matthias Schubert , Roberto C. Myers