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The photomolecular effect has been hypothesized to enhance evaporation of water at visible wavelengths. This study develops a measurement technique to investigate its presence and magnitude at the liquid-vapor interface of water. The…

Optics · Physics 2026-03-19 Preston Bohm , Mingjun Li , Akanksha K. Menon , Zhuomin M. Zhang

We present a method for computing optical absorption spectra by means of a Bethe-Salpeter equation approach, which is based on a conserving linear response calculation for electron-hole coherences in the presence of an external…

Materials Science · Physics 2010-12-21 George Pal , Yaroslav Pavlyukh , Wolfgang Hübner , Hans Christian Schneider

An optical absorption spectrum constitutes one of the most fundamental material characteristics, with relevant applications ranging from material identification to energy harvesting and optoelectronics. However, the database of both…

Materials Science · Physics 2022-09-20 Ruo Xi Yang , Matthew K. Horton , Jason Munro , Kristin A. Persson

Optical absorption spectra of C_70 and C_76 are calculated by a tight binding model with a long ranged Coulomb interaction. The spectrum of C_70 is in overall agreement with the experiment of molecules in a solution. The variations of the…

Condensed Matter · Physics 2007-05-23 Kikuo Harigaya , Shuji Abe

In this paper, we report on the optical absorption in porous silicon. We model the absorption process assuming that porous silicon is a pseudo 1D material system having a distribution of band gaps. We show that in order to explain the…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Shouvik Datta , K. L. Narasimhan

It is well-known that water in both liquid and vapor phases exhibits exceptionally weak absorption of light in the visible range. Recent experiments, however, have demonstrated that at the liquid-air interface, absorption in the visible…

Soft Condensed Matter · Physics 2025-01-16 Michael J. Landry , Chuliang Fu , James H. Zhang , Jiachen Li , Gang Chen , Mingda Li

Absorption spectra of liquid water at 300 K are calculated from both classical and density functional theory molecular dynamics simulation data, which together span from 1 MHz to hundreds of THz, agreeing well with experimental data…

Chemical Physics · Physics 2020-09-09 Shane Carlson , Florian N. Brünig , Philip Loche , Douwe Jan Bonthuis , Roland R. Netz

Using Linear Response Theory, with appropriate wave functions and energies from perturbation method, the absorption profiles can be calculated for all three classes of mixed-valence systems as defined by Robin and Day : Class III…

Materials Science · Physics 2024-10-18 Kin Yip Wong

Linear and nonlinear optical absorption coefficients of the two-dimensional semiconductor ring in the perpendicular magnetic field $\bf B$ are calculated within independent electron approximation. Characteristic feature of the energy…

Mesoscale and Nanoscale Physics · Physics 2014-03-03 O. Olendski , T. Barakat

We have investigated the simultaneous absorption of near-infrared photons by pairs of neighboring molecules in liquid methanol. Simultaneous absorption by two OH-stretching modes is found to occur at an energy higher than the sum of the two…

Soft Condensed Matter · Physics 2009-11-13 Sander Woutersen

The strength of light-matter interaction is of central importance in photonics and optoelectronics. For many widely studied two-dimensional semiconductors, such as MoS2, the optical absorption due to exciton resonances increases with…

Mesoscale and Nanoscale Physics · Physics 2020-04-16 Guowei Zhang , Shenyang Huang , Fanjie Wang , Qiaoxia Xing , Chaoyu Song , Chong Wang , Yuchen Lei , Mingyuan Huang , Hugen Yan

In this paper, we analyse the optical absorption in porous silicon . This is the first attempt to explicitly demonstrate that it is not possible to extract the band gap of such low dimensional nanostructures like porous silicon from a Tauc…

Soft Condensed Matter · Physics 2007-05-23 Shouvik Datta , K. L. Narasimhan

The effects of random distribution of magnetic impurities with concentration $x$ in a semiconductor alloy multilayer at a paramagnetic temperature are investigated by means of coherent potential approximation and tight-binding model. The…

Mesoscale and Nanoscale Physics · Physics 2012-09-20 Leili Gharaee , Alireza Saffarzadeh

Cloud absorption is acknowledged as the biggest source of uncertainty in the climate models. For over 70 years, many experiments have reported clouds absorbing more solar radiation than theory could predict. In the visible spectrum,…

Atmospheric and Oceanic Physics · Physics 2025-02-24 Gang Chen

We propose a new method to measure the absolute photon absorption cross section of neutral molecules in a molecular beam. It is independent of our knowledge of the particle beam density, nor does it rely on photo-induced fragmentation or…

Quantum Physics · Physics 2008-12-31 Stefan Nimmrichter , Klaus Hornberger , Hendrik Ulbricht , Markus Arndt

Absorption microscopy is a powerful technique, enabling the detection of single non- fluorescent molecules at room temperature. So far, the molecular absorption has been probed optically via the attenuation of a probing laser. The…

Applied Physics · Physics 2018-11-21 Miao-Hsuan Chien , Mario Brameshuber , Gerhard J. Schütz , Silvan Schmid

Water wires, quasi-one-dimensional chains composed of hydrogen-bonded (H-bonded) water molecules, play a fundamental role in numerous chemical, physical, and physiological processes. Yet direct experimental detection of water wires has been…

Materials Science · Physics 2025-03-07 Fujie Tang , Diana Y. Qiu , Xifan Wu

We present results for the optical absorption spectra of small-diameter single-wall carbon and boron nitride nanotubes obtained by {\it ab initio} calculations in the framework of time-dependent density functional theory. We compare the…

Materials Science · Physics 2010-07-01 A. G. Marinopoulos , Ludger Wirtz , Andrea Marini , Valerio Olevano , Angel Rubio , Lucia Reining

The evaporation of water is ubiquitous in nature and industrial technologies. The known mechanism for evaporation is "thermal evaporation" which highlights the energy input for evaporation is via heat. Due to the weak absorption of water to…

Atomic and Molecular Clusters · Physics 2024-04-24 Yaodong Tu , Gang Chen

Ultraviolet photodesorption of molecules from icy interstellar grains can explain observations of cold gas in regions where thermal desorption is negligible. This non-thermal desorption mechanism should be especially important where UV…