Related papers: Disentangling Dynamical Quantum Coherences in the …
Equations of motion for weakly coupled excitonic complexes are derived. The description allows to treat the system in the basis of electronic states localized on individual chromophores, while at the same time accounting for experimentally…
A generic and intuitive model for coherent energy transport in multiple minima systems coupled to a quantum mechanical bath is shown. Using a simple spin-boson system, we illustrate how a generic donor-acceptor system can be brought into…
Efficient energy transport is highly desirable for organic semiconductor (OSC) devices such as photovoltaics, photodetectors, and photocatalytic systems. However, photo-generated excitons in OSC films mostly occupy highly localized states…
Experimental/theoretical evidence for sustained vibration-assisted electronic (vibronic) coherence in the Photosystem II Reaction Center (PSII RC) indicates that photosynthetic solar-energy conversion might be optimized through the…
Photons excited into ground state modes at finite temperature display partitioning among photon phases, lifetimes and distances travelled since creation. These distributions set the distance from an interface a created photon has some…
We investigate the excitation of phonons in photoexcited antimony and demonstrate that the entire electron-lattice interactions, in particular coherent and incoherent electron-phonon coupling, can be probed simultaneously. Using femtosecond…
We derive quantum kinetic equations for fermions in a homogeneous time-dependent background in presence of decohering collisions, by use of the Schwinger-Keldysh CTP-formalism. The quantum coherence (between particles and antiparticles) is…
We investigate the temperature dependence of photon coherence properties through two photon interference (TPI) measurements from a single QD under resonant excitation. We show that the loss of indistinguishability is only related to the…
Phycobilisomes are antenna protein complexes in cyanobacteria and red algae. In phycobilisomes, energy transfer is unidirectional with an extremely high quantum efficiency close to unity. We investigate intraprotein energy relaxation and…
How quantum coherence influences thermodynamic behavior remains an open question in quantum thermodynamics. Here we investigate this relation within the pure dephasing framework, where a central qubit interacts with a finite Ising-like spin…
Decoherence in Nature has become one of the most pressing problems in physics. Many applications, including quantum information processing, depend on understanding it; and fundamental theories going beyond quantum mechanics have been…
Long-lived oscillations in 2D spectra of chlorophylls are at the heart of an ongoing debate. Their physical origin is either a multi-pigment effect, such as excitonic coherence, or primarily stems from localized vibrations. In the present…
Fluctuations in the energy gap and coupling constants in and between chromophores can play important role in the absorption and energy transfer across a collection of two level systems. In a noisy environment, fluctuations can control…
Determining how energy flows within and between molecules is crucial for understanding chemical reactions, material properties, and even vital processes such as photosynthesis. While the general principles of energy transfer are well…
Most discussions of decoherence in the literature consider the high-temperature regime but it is also known that, in the presence of dissipation, decoherence can occur even at zero temperature. Whereas most previous investigations all…
The coherent optical response from 140~nm and 65~nm thick ZnO epitaxial layers is studied using transient four-wave-mixing spectroscopy with picosecond temporal resolution. Resonant excitation of neutral donor-bound excitons results in…
The ultrastrong and deep strong coupling regimes exhibit a variety of intriguing physical phenomena. In this work, we utilize the Hopfield model of a two-mode bosonic system, with each mode interacts with a heat reservoir, to research the…
We investigate resonant photoluminescence arising from incompressible quantum liquids formed in two-dimensional electron systems. We demonstrate that, for excitons composed of a photoexcited electron occupying the upper spin sublevel of the…
An initial local excitation in a confined quantum system evolves exploring the whole system, returning to the initial position as a mesoscopic echo at the Heisenberg time. We consider a two weakly coupled spin chains, a spin ladder, where…
We present a theory that efficiently describes the quantum dynamics of an electronic excitation that is coupled to a continuous, highly structured phonon environment. Based on a stochastic approach to non-Markovian open quantum systems, we…