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We investigate the role of electron correlation in the two-photon double ionization of helium for ultrashort XUV pulses with durations ranging from a hundred attoseconds to a few femtoseconds. We perform time-dependent ab initio…

Time-delays in the photoionization of molecules are investigated. As compared to atomic ionization, the time-delays expected from molecular ionization present a much richer phenomenon, with a strong spatial dependence due to the anisotropic…

Atomic Physics · Physics 2017-02-14 P. Hockett , E. Frumker , D. M. Villeneuve , P. B. Corkum

We study tunneling ionization of HeH+ in strong elliptical laser fields numerically and analytically. The calculated photoelectron momentum distribution (PMD) show two different offset angles corresponding to ionization events occurring in…

Atomic Physics · Physics 2025-11-18 Jiayin Che , Sheng Ye , Shiqi Shen , Weiyan Li , Yanjun Chen

In nuclear collisions, nuclear bremsstrahlung can cause nuclear Coulomb excitation via photon exchange in the projectile as well as the target nuclei. Such a process originating in nuclear timescales (zeptoseconds) can also influence the…

Atomic Physics · Physics 2025-03-25 T. Nandi , Soumya Chatterjee , Adya P. Mishra , Y. Azuma , F. Koike , A. S. Kheifets

A comprehensive theoretical understanding of electron-photon correlation is essential for describing the reshaping of molecular orbitals in quantum electrodynamics (QED) environments. The strong coupling QED Hartree-Fock (SC-QED-HF) theory…

Chemical Physics · Physics 2024-09-04 Yassir El Moutaoukal , Rosario R. Riso , Matteo Castagnola , Henrik Koch

In a recent paper [Phys. Rev. Lett. 125, 043201 (2020)] (Ref.1) Liao et al. propose a theory of the interferometric photoemission delay based on the concepts of the photoelectron phase and photoelectron effective mass. The present comment…

Materials Science · Physics 2021-04-26 E. E. Krasovskii , R. O. Kuzian

It is shown that the amplitude of elastic ed scattering beyond Born approximation contains six generalized form factors, but only three linearly independent combinations of them (generalized charge, quadrupole and magnetic form factors)…

Nuclear Theory · Physics 2015-03-17 A. P. Kobushkin , Ya. D. Krivenko-Emetov

The development of reliable ab initio methods for light-matter strong coupling is necessary for a deeper understanding of molecular polaritons. The recently developed strong coupling quantum electrodynamics Hartree-Fock model (SC-QED-HF)…

Chemical Physics · Physics 2025-02-21 Matteo Castagnola , Rosario R. Riso , Yassir El Moutaoukal , Enrico Ronca , Henrik Koch

The energy density functional (EDF) method is very widely used in nuclear physics, and among the various existing functionals those based on the relativistic Hartree (RH) approximation are very popular because the exchange contributions…

Nuclear Theory · Physics 2014-05-16 Nguyen Van Giai , Haozhao Liang , Huai-Qiang Gu , Wenhui Long , Jie Meng

The coherent interaction between free electrons and optical fields can produce free-electron compression and push the temporal resolution of ultrafast electron microscopy to the attosecond regime. However, a large electron-light interaction…

Quantum Physics · Physics 2025-03-27 Cruz I. Velasco , F. Javier García de Abajo

The present review addresses the technical advances and the theoretical developments to realize and rationalize attosecond-science experiments that reveal a new dynamical time scale ($10^{-15}$-$10^{-18}$ s), with a particular emphasis on…

Chemical Physics · Physics 2020-02-07 Denitsa Baykusheva , Hans Jakob Wörner

We calculate the transient absorption of an isolated attosecond pulse by helium atoms subject to a delayed infrared (\ir) laser pulse. With the central frequency of the broad attosecond spectrum near the ionization threshold, the absorption…

Atomic Physics · Physics 2015-06-12 Shaohao Chen , Mengxi Wu , Mette B. Gaarde , Kenneth J. Schafer

We show that the complete photoemission dynamics in situations of electron-ion entanglement can be retrieved from photoelectron spectral measurements without information on the ion. To this end, we develop an energy-time analysis of the…

We develop a first-principles simulation method for attosecond time-resolved photoelectron spectroscopy. This method enables us to directly simulate the whole experimental processes, including excitation, emission and detection on equal…

Atomic Physics · Physics 2018-08-01 Shunsuke A. Sato , Hannes Hübener , Angel Rubio , Umberto De Giovannini

Ionization by relativistically intense short laser pulses is studied in the framework of strong-field quantum electrodynamics. Distinctive patterns are found in the energy probability distributions of photoelectrons. Except of the already…

Atomic Physics · Physics 2018-03-14 F. Cajiao Vélez , J. Z. Kamiński , K. Krajewska

Exchange interaction strongly influences the long-range behavior of localized electron orbitals and quantum tunneling amplitudes.In the Hartree-Fock approximation the exchange produces a power-law decay instead of the usual exponential…

Quantum Physics · Physics 2015-05-14 V. V. Flambaum

Measuring the delay for an electron to emerge from different states is one of the major achievements of attosecond science. This delay can have two origins - the electron wave packet is reshaped during departure by the electrostatic field…

Atomic Physics · Physics 2020-10-14 Graham G. Brown , Dong Hyuk Ko , Chunmei Zhang , P. B. Corkum

We analyze the time delay between emission of photoelectrons from the outer valence $ns$ and $np$ sub-shells in noble gas atoms following absorption of an attosecond XUV pulse. By solving the time dependent Schr\"odinger equation and…

Atomic Physics · Physics 2010-12-07 A. S. Kheifets , I. A. Ivanov

Helium nanodroplets are ideal model systems to unravel the complex interaction of condensed matter with ionizing radiation. Here we study the effect of purely elastic electron scattering on angular and energy distributions of photoelectrons…

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