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The photoionization of the CO molecule from the C$-1s$ orbital does not obey the Franck-Condon approximation, as a consequence of the nuclear recoil that accompanies the direct emission and intra-molecular scattering of the photoelectron.…

Atomic Physics · Physics 2021-11-24 Bejan Ghomashi , Nicolas Douguet , Luca Argenti

We investigate theoretically the relative time delay of photoelectrons originating from different atomic subshells of noble gases. This quantity was measured via attosecond streaking and studied theoretically by Schultze et al. [Science…

Atomic Physics · Physics 2015-06-22 Jonas Wätzel , Andrey Moskalenko , Yaroslav Pavlyukh , Jamal Berakdar

Imaging in real time the complete dynamics of a process as fundamental as photoemission has long been out of reach due to the difficulty of combining attosecond temporal resolution with fine spectral and angular resolutions. Here, we…

Using a spectrally resolved electron interferometry technique, we measure photoionization time delays between the $3s$ and $3p$ subshells of argon over a large 34-eV energy range covering the Cooper minima in both subshells. The observed…

Ji \etal [New J. Phys. {\bf 26}, 093014 (2024)] established a direct link between the photoionization cross section and the attosecond time delay near Cooper minima (CM) in the valence shells of noble-gas atoms. This link is based on the…

Atomic Physics · Physics 2026-03-03 Adam J. C. Singor , Dmitry V. Fursa , Igor Bray , Anatoli S. Kheifets

Attosecond spectroscopy is currently restricted to photon energies around 100 eV. We show that under these conditions, electron-electron scatterings, as the photoelectrons leave the metal give rise to a tail of secondary electrons with…

Other Condensed Matter · Physics 2015-05-13 Jan Conrad Baggesen , Lars Bojer Madsen

We propose a two-dimensional interferometry based on electron wave packet interference with a cycle-shaped orthogonally polarized two-color laser field. With such method, sub-cycle and inter-cycle interferences can be disentangled into…

Atomic Physics · Physics 2015-06-04 Xinhua Xie

We analyze the real-time electron-photon dynamics in long-range polariton-mediated energy transfer using a real-time quantum electrodynamics coupled cluster (RT-QED-CC) model, which allows for spatial and temporal visualization of transport…

Chemical Physics · Physics 2024-04-16 Matteo Castagnola , Marcus T. Lexander , Enrico Ronca , Henrik Koch

Measuring the time it takes to remove an electron from an atom or molecule during photoionization using newly developed attosecond spectroscopies has been a focus of many recent experiments. However, the outcome of such measurement depends…

Atomic Physics · Physics 2017-03-08 Lisa Torlina , Olga Smirnova

We use the non-relativistic random phase approximation with exchange to perform calculations of valence shell photoionization of Ne, Ar, Kr and Xe from their respective thresholds to photon energy of 200 eV. The energy derivative of the…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets

We identify peak and valley structures in the exact exchange-correlation potential of time-dependent density functional theory that are crucial for time-resolved electron scattering in a model one-dimensional system. These structures are…

Chemical Physics · Physics 2018-01-03 Yasumitsu Suzuki , Lionel Lacombe , Kazuyuki Watanabe , Neepa T. Maitra

Recently the time delay in the attosecond photoemission was observed (Science,2010). In this paper we propose the description of that time delay in the framework of hyperbolic heat transport equation. We argue that the observed time delay…

General Physics · Physics 2013-02-20 J. Marciak-Kozlowska , M. Kozlowski

Attosecond photoionization delays have mostly been interpreted within the single-particle approximation of multi-electron systems. The strong electron correlation between the photoionization channels associated with the 3p and 3s orbitals…

The toolbox for imaging molecules is well-equipped today. Some techniques visualize the geometrical structure, others the electron density or electron orbitals. Molecules are many-body systems for which the correlation between the…

We investigate multi-electron effects in strong-field ionization of Helium using a semi-classical model that, unlike other commonly used theoretical approaches, takes into account electron-electron correlation. Our approach has an…

Atomic Physics · Physics 2016-10-12 A. Emmanouilidou , A. Chen , C. Hofmann , U. Keller , A. S. Landsman

Proton emission, $\alpha$ decay, and cluster radioactivity play an important role in nuclear physics. We show that high-frequency alternative electric fields could deform Coulomb barriers that trap the charged particle, and raise the…

Nuclear Theory · Physics 2018-06-13 Dong Bai , Daming Deng , Zhongzhou Ren

With a combination of numerical methods, including quantum Monte Carlo, exact diagonalization, and a simplified dynamical mean-field model, we consider the attosecond charge dynamics of electrons induced by strong-field laser pulses in…

Strongly Correlated Electrons · Physics 2021-10-08 Christopher Orthodoxou , Amelle Zaïr , George H. Booth

Two-photon exchange contributions to elastic electron-proton scattering cross sections are evaluated in a simple hadronic model including the finite size of the proton. The corrections are found to be small in magnitude, but with a strong…

Nuclear Theory · Physics 2008-11-26 P. G. Blunden , W. Melnitchouk , J. A. Tjon

In time-resolved photoemission experiments, more than one electron can be emitted from the solid by a single ultra-short pulse. We theoretically demonstrate how correlations between the momenta of outgoing electrons relate to time-dependent…

Strongly Correlated Electrons · Physics 2019-06-26 Christopher Stahl , Martin Eckstein

We investigate the effects of the multielectron polarization of the ion described by the induced dipole potential in photoelectron momentum distributions produced in ionization of the CO molecule by a strong laser field. We present results…

Atomic Physics · Physics 2024-04-23 Mahmoud Abu-samha , L. B. Madsen , N. I. Shvetsov-Shilovski