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Magnetic resonance spectroscopy is universally regarded as one of the most important tools in chemical and bio-medical research. However, sensitivity limitations typically restrict imaging resolution to length scales greater than 10 \mu m.…

Measuring spins is the corner stone of a variety of analytical techniques including modern magnetic resonance imaging (MRI). The full potential of spin imaging and sensing across length scales is hindered by the achievable signal-to-noise…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 S. Steinert , F. Ziem , L. Hall , A. Zappe , M. Schweikert , A. Aird , G. Balasubramanian , L. Hollenberg , J. Wrachtrup

Recently, there have been significant developments to detect nuclear spins with an nitrogen vacancy (NV) center in diamond. However, due to the nature of the short range dipole-dipole interaction, it takes a long time to detect distant…

Quantum Physics · Physics 2021-08-11 Hideaki Hakoshima , Yuichiro Matsuzaki , Toyofumi Ishikawa

Highly sensitive nuclear spin detection is crucial in many scientific areas including nuclear magnetic resonance spectroscopy (NMR), imaging (MRI) and quantum computing. The tiny thermal nuclear spin polarization represents a major obstacle…

Conventional nuclear magnetic resonance (NMR) spectroscopy relies on acquiring signal from a macroscopic ensemble of molecules to gain information about molecular structure and dynamics. Transferring this technique to nanoscale sample sizes…

Mesoscale and Nanoscale Physics · Physics 2019-02-06 Jeffrey Holzgrafe , Qiushi Gu , Jan Beitner , Dhiren Kara , Helena S. Knowles , Mete Atatüre

Nonlinear spectroscopy is widely used for studying physical systems. Conventional nonlinear optical spectroscopy and magnetic resonance spectroscopy, which use classical probes such as electromagnetic waves, can only access certain types of…

Nuclear quadrupolar resonance (NQR) spectroscopy reveals chemical bonding patterns in materials and molecules through the unique coupling between nuclear spins and local fields. However, traditional NQR techniques require macroscopic…

Mesoscale and Nanoscale Physics · Physics 2025-01-14 S. Alex Breitweiser , Mathieu Ouellet , Tzu-Yung Huang , Tim H. Taminiau , Lee C. Bassett

Nitrogen vacancy (NV) color centers in diamond are a leading modality for both superresolution optical imaging and nanoscale magnetic field sensing. In this work, we solve the remaining key challenge of performing optical magnetic imaging…

Nanomagnetometry using the nitrogen-vacancy (NV) centre in diamond has attracted a great deal of interest because of the combined features of room temperature operation, nanoscale resolution and high sensitivity. One of the important goals…

Nuclear magnetic resonance (NMR) spectroscopy is widely used in fields ranging from chemistry, material science to neuroscience. Nanoscale NMR spectroscopy using Nitrogen-vacancy (NV) centers in diamond has emerged as a promising platform…

Detecting nuclear spins using single Nitrogen-Vacancy (NV) centers is of particular importance in nano-scale science and engineering, but often suffers from the heating effect of microwave fields for spin manipulation, especially under high…

Quantum Physics · Physics 2024-09-06 Zhiyi Hu , Fengjian Jiang , Jingyan He , Yulin Dai , Ya Wang , Nanyang Xu , Jiangfeng Du

Single-spin magnetic resonance spectroscopy promises to yield structural and chemical information at the level of individual atoms or molecules, in a non-invasive way. Here, we use an Er3+ paramagnetic center in a CaWO4 crystal, detected by…

Nuclear magnetic resonance (NMR) at the single-molecule level with atomic resolution holds transformative potential for structural biology and surface chemistry. Near-surface solid-state spin sensors with optical readout ability offer a…

Quantum Physics · Physics 2025-12-12 Yu Chen , Qi Zhang , Yuanhong Teng , Chihang Luo , Zhijie Li , Jinpeng Liu , Ya Wang , Fazhan Shi , Jiangfeng Du

We propose a method to measure the hyperfine vectors between a nitrogen-vacancy (NV) center and an environment of interacting nuclear spins. Our protocol enables the generation of tunable electron-nuclear coupling Hamiltonians while…

Quantum Physics · Physics 2016-05-12 Zhen-Yu Wang , Jan F. Haase , Jorge Casanova , Martin B. Plenio

We recently showed that macroscopic nuclear spin ensembles prepared in coherent spin states can dramatically enhance the interaction rates of weakly interacting cosmic relics-such as dark matter and the cosmic neutrino background-through…

High Energy Physics - Phenomenology · Physics 2026-05-01 Marios Galanis , Onur Hosten , Asimina Arvanitaki , Savas Dimopoulos

The field of nanoscale magnetic resonance imaging (NanoMRI) was started 30 years ago. It was motivated by the desire to image single molecules and molecular assemblies, such as proteins and virus particles, with near-atomic spatial…

Magnetic resonance with ensembles of electron spins is nowadays performed in frequency ranges up to 240 GHz and in corresponding magnetic fields of up to 10 T. However, experiments with single electron and nuclear spins so far only reach…

Individual electron spins have been observed using magnetic resonance in combination with a number of distinct detection approaches. The coordinates of an individual electron spin can then in principle be determined by introducing a 10 to…

Mesoscale and Nanoscale Physics · Physics 2018-02-21 Hoang Long Nguyen , John A. Marohn

We review recent efforts to detect small numbers of nuclear spins using magnetic resonance force microscopy. Magnetic resonance force microscopy (MRFM) is a scanning probe technique that relies on the mechanical measurement of the weak…

Mesoscale and Nanoscale Physics · Physics 2010-08-03 M. Poggio , C. L. Degen

Mapping the positions of single electron spins is a highly desired capability for applications such as nanoscale magnetic resonance imaging and quantum network characterization. Here, we demonstrate a method based on rotating an external…

Mesoscale and Nanoscale Physics · Physics 2022-11-11 Dan Yudilevich , Rainer Stöhr , Andrej Denisenko , Amit Finkler