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The nuclear spin is a prime candidate for quantum information applications due to its weak coupling to the environment and inherently long coherence times. However, this weak coupling also challenges the addressability of the nuclear spin.…

Quantum Physics · Physics 2025-12-15 Hester G. Vennema , Cristina Mier , Evert W. Stolte , Leonard Edens , Jinwon Lee , Sander Otte

Magnetic resonance imaging (MRI) revolutionized diagnostic medicine and biomedical research by allowing a noninvasive access to spin ensembles. To enhance MRI resolution to the nanometer scale, new approaches including scanning probe…

Mesoscale and Nanoscale Physics · Physics 2019-10-23 Philip Willke , Kai Yang , Yujeong Bae , Andreas J. Heinrich , Christopher P. Lutz

Spin defects in solids, such as the nitrogen-vacancy (NV) center in diamond, have emerged as a key tool for detecting nuclear spins at the nanoscale. While active nuclear spin control via radio-frequency (RF) irradiation is often…

The detection of a nuclear spin in an individual molecule represents a key challenge in physics and biology whose solution has been pursued for many years. The small magnetic moment of a single nucleus and the unavoidable environmental…

Quantum Physics · Physics 2015-03-19 Jianming Cai , Fedor Jelezko , Martin B. Plenio , Alex Retzker

Sensing, localising and identifying individual nuclear spins or frequency components of a signal in the presence of a noisy environments requires the development of robust and selective methods of dynamical decoupling. An important…

We report a method for accelerated nanoscale nuclear magnetic resonance imaging by detecting several signals in parallel. Our technique relies on phase multiplexing, where the signals from different nuclear spin ensembles are encoded in the…

Mesoscale and Nanoscale Physics · Physics 2015-08-11 B. A. Moores , A. Eichler , Y. Tao , H. Takahashi , P. Navaretti , C. L. Degen

Optically detected magnetic resonance (ODMR) provides ultrasensitive means to detect and image a small number of electron and nuclear spins, down to the single spin level with nanoscale resolution. Despite the significant recent progress in…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Aharon Blank , Guy Shapiro , Ran Fischer , Paz London , David Gershoni

Different approaches have improved the sensitivity of either electron or nuclear magnetic resonance to the single spin level. For optical detection it has essentially become routine to observe a single electron spin or nuclear spin.…

Mesoscale and Nanoscale Physics · Physics 2016-06-29 Jörg Wrachtrup , Amit Finkler

Nuclear magnetic resonance (NMR) has enormous applications. Two-dimensional NMR is an essential technique to characterize correlations between nuclei and, hence, molecule structures. Towards the ultimate goal of single-molecule NMR,…

Quantum Physics · Physics 2016-11-30 Wen-Long Ma , Ren-Bao Liu

We propose a scheme to increase the sensitivity and thus the detection volume of nanoscale single molecule magnetic resonance imaging. The proposal aims to surpass the T1 limited detection of the sensor by taking advantage of a long-lived…

Quantum Physics · Physics 2015-11-05 Johannes N. Greiner , D. D. Bhaktavatsala Rao , Philipp Neumann , Jörg Wrachtrup

Quantum control of individual spins in condensed matter systems is an emerging field with wide-ranging applications in spintronics, quantum computation, and sensitive magnetometry. Recent experiments have demonstrated the ability to address…

Mesoscale and Nanoscale Physics · Physics 2011-09-09 M. S. Grinolds , P. Maletinsky , S. Hong , M. D. Lukin , R. L Walsworth , A. Yacoby

The hyperpolarisation of nuclear spins within target molecules is a critical and complex challenge in magnetic resonance imaging (MRI) and nuclear magnetic resonance (NMR) spectroscopy. Hyperpolarisation offers enormous gains in signal and…

Detecting and controlling nuclear spin nano-ensembles is crucial for the further development of nuclear magnetic resonance (NMR) spectroscopy and for the emerging solid state quantum technology. Here we present the fabrication of a…

Nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) are well-established techniques that provide valuable information in a diverse set of disciplines but are currently limited to macroscopic sample volumes. Here we…

Methods for achieving quantum control and detection of individual nuclear spins by single electrons of solid-state defects play a central role for quantum information processing and nano-scale nuclear magnetic resonance (NMR). However, with…

Quantum Physics · Physics 2017-03-06 Zhen-Yu Wang , Jorge Casanova , Martin B. Plenio

Optically-detected paramagnetic centers in wide-bandgap semiconductors are emerging as a promising platform for nanoscale metrology at room temperature. Of particular interest are applications where the center is used as a probe to…

Mesoscale and Nanoscale Physics · Physics 2015-12-09 Abdelghani Laraoui , Daniela Pagliero , Carlos A. Meriles

We report on Fourier spectroscopy experiments performed with near-surface nitrogen-vacancy centers in a diamond chip. By detecting the free precession of nuclear spins rather than applying a multipulse quantum sensing protocol, we are able…

Quantum Physics · Physics 2016-05-18 J. M. Boss , K. Chang , J. Armijo , K. Cujia , T. Rosskopf , J. R. Maze , C. L. Degen

Mechanical resonators operating in the high-frequency regime have become a versatile platform for fundamental and applied quantum research. Their exceptional properties, such as low mass and high quality factor, make them also very…

Mesoscale and Nanoscale Physics · Physics 2023-11-29 Diego A. Visani , Letizia Catalini , Christian L. Degen , Alexander Eichler , Javier del Pino

Nanoscale nuclear magnetic resonance (NMR) signals can be measured through hyperfine interaction to paramagnetic electron sensor spins. A heterodyne approach is widely used to overcome the electron spin lifetime limit in spectral…

Spins associated to optically accessible solid-state defects have emerged as a versatile platform for exploring quantum simulation, quantum sensing and quantum communication. Pioneering experiments have shown the sensing, imaging, and…