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It has been observed experimentally [H.R. Xia, C.Y. Ye, and S.Y. Zhu, Phys. Rev. Lett. {\bf 77}, 1032 (1996)] that quantum interference between two molecular transitions can lead to a suppression or enhancement of spontaneous emission. This…

Quantum Physics · Physics 2009-10-31 Jin Wang , H. M. Wiseman , Z. Ficek

Two-photon excitation is an attractive means for controlling chemistry in both space and time. Isoenergetic one- and two-photon excitations (OPE and TPE) in non-centrosymmetric molecules are often assumed to reach the same excited state…

The ability to entangle distant quantum nodes is essential for the construction of quantum networks and for quantum information processing. For solid-state quantum emitters used as qubits, it can be achieved by photon interference. When the…

Quantum Physics · Physics 2019-10-23 Herbert F Fotso

When two-color femtosecond laser pulses interact with matter, electrons can be emitted through various multiphoton excitation pathways. Quantum interference between these pathways gives rise to a strong oscillation of the photoemitted…

Optics · Physics 2022-05-24 Ang Li , Yiming Pan , Philip Dienstbier , Peter Hommelhoff

We consider the interaction of one- and two-photon pulses in a waveguide with two two-level systems (TLS) that are also able to interact directly either through an exchange- or a dipole-type interaction. We focus on the system's transport…

Quantum Physics · Physics 2017-12-27 William Konyk , Julio Gea-Banacloche

We describe optimized coherent control methods for two-photon transitions in atoms of a ladder-type three-state energy configuration. Our approach is based on the spatial coherent control scheme which utilizes counter-propagating ultrashort…

Atomic Physics · Physics 2015-10-28 Woojun Lee , Hyosub Kim , Kyungtae Kim , Jaewook Ahn

Ultrafast photoexcitation offers a novel approach to manipulating quantum materials. One of the long-standing goals in this field is to achieve optical control over topological properties. However, the impact on their electronic structures,…

Materials Science · Physics 2024-12-10 Masataka Mogi , Dongsung Choi , Louis Primeau , Baiqing Lv , Doron Azoury , Yifan Su , Liang Fu , Yang Zhang , Nuh Gedik

State mapping between atoms and photons, and photon-photon interactions play an important role in scalable quantum information processing. We consider the interaction of a two-level atom with a quantized \textit{propagating} pulse in free…

Quantum Physics · Physics 2013-05-29 Yimin Wang , Jiří Minář , Lana Sheridan , Valerio Scarani

We explore the effects of ultrafast shaped pulses for two-level systems that do not have a single photon resonance by developing a multiphoton density-matrix approach. We take advantage of the fact that the dynamics of the intermediate…

Optics · Physics 2009-11-07 S. Abbas Hosseini , Debabrata Goswami

We report a two-photon interference effect, in which the entangled photon pairs are generated from two laser pulses well-separated in time. In a single pump pulse case, interference effects did not occur in our experimental scheme. However,…

We analyze particular two-photon processes as possible means to explore electronic quadrupole states in free small deformed atomic clusters. The analysis is done in the time-dependent local density approximation (TDLDA). It is shown that…

Atomic and Molecular Clusters · Physics 2011-05-26 V. O. Nesterenko , P. -G. Reinhard , Th. Halfmann , E. Suraud

The purpose of this paper is to study the interaction between a two-level system and two continuous-mode photons. Two scenarios are investigated: Case 1, how a two-level system changes the pulse shapes of two input photons propagating in a…

Quantum Physics · Physics 2019-10-14 Zhiyuan Dong , Guofeng Zhang , Nina H. Amini

Multiphoton interference is an important phenomenon in modern quantum mechanics and experimental quantum optics, and it is fundamental for the development of quantum information science and technologies. Over the last three decades, several…

Quantum Physics · Physics 2021-10-20 Heonoh Kim , Osung Kwon , Han Seb Moon

Coherent manipulation of single-photon wave packets is essentially important for optical quantum communication and quantum information processing. In this paper, we realize controllable splitting and modulation of single-photon-level pulses…

Quantum Physics · Physics 2015-05-13 Sheng-Jun Yang , Xiao-Hui Bao , Jian-Wei Pan

Efficient excitation of a single two-level system usually requires that the driving field is at the same frequency as the atomic transition. However, the scattered laser light in solid-state implementations can dominate over the single…

We present results on a multiple-optical-path quantum interference project suitable for the advanced undergraduate laboratory. The experiments combine a conceptually rich set of atomic physics experiments which may be economically developed…

Physics Education · Physics 2018-07-25 Clark Vandam , Aaron Hankin , A. Sieradzan , M. D. Havey

Recent evidence suggests that the multi charge-separation pathways can contribute to the photosynthetic performance. In this work, the influence of coupled-dipoles on the photosynthetic performance was investigated in a two-charge…

Chemical Physics · Physics 2025-01-14 Ling-Fang Li , Shun-Cai Zhao

We propose an architecture for achieving high-fidelity deterministic quantum logic gates on dual-rail encoded photonic qubits by letting photons interact with a two-level emitter (TLE) inside an optical cavity. The photon wave packets that…

Quantum Physics · Physics 2022-09-12 Stefan Krastanov , Kurt Jacobs , Gerald Gilbert , Dirk R. Englund , Mikkel Heuck

We demonstrate how dynamic Stark control (DSC) can be achieved on molecular photodissociation in the dipole limit, using single-cycle (FWHM) laser pulses in the terahertz (THz) regime. As the laser-molecule interaction follows the…

Chemical Physics · Physics 2020-03-25 A. Tóth , A. Csehi , G. J. Halász , Á. Vibók

We use orthogonally polarized two-colour (OTC) laser pulses to separate quantum paths in multiphoton ionization of Ar atoms. Our OTC pulses consist of 400~nm and 800~nm light at a relative intensity ratio of 10:1. We find a hitherto…

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