Related papers: Controlling quantum interference between virtual a…
Multi-photon propagation in connected structures - a quantum walk - offers the potential for simulating complex physical systems and provides a route to universal quantum computation. Increasing the complexity of quantum photonic networks…
Electronic excitation energy transfer along a molecular wire depends on the relative orientation of the electronic transition dipole moments of neighboring chromophores. In porphycenes this orientation is changed upon double proton transfer…
Path-entangled multi-photon states allow optical phase-sensing beyond the shot-noise limit, provided that an efficient parity measurement can be implemented. Realising this experimentally is technologically demanding, as it requires…
We study the quantum interference between the excitation pathways in a three-level $\Lambda$-type atom interacting with two short laser pulse trains under the conditions of electromagnetically induced transparency. The probability amplitude…
Femtosecond pulses have been used to reveal hidden broken symmetry states and induce transitions to metastable states. However, these states are mostly transient and disappear after laser removal. Photoinduced phase transitions towards…
We study non-classical pathways and quantum interference in enhanced ionisation of diatomic molecules in strong laser fields using machine learning techniques. Quantum interference provides a bridge, which facilitates intramolecular…
Excitation energy transfer is a photophysical process upon which many chemical and biological phenomena are built. From natural small systems to synthetic multichromophoric macromolecules, energy transfer deals with the process of migration…
Microscopic and dynamic control over quantum states is essential for bridging fundamental studies of material properties to device function. Realizing such control at combined high spatial resolution and ultrafast temporal precision remains…
We report a new method of two-pathway coherent control using three narrow-band cw laser sources, phase locked in an optical phase-lock loop, to maintain the high degree of optical coherence required for the coherent control process. In…
The absorption of traveling photons resonant with electric dipole transitions of an atomic gas naturally leads to electric dipole spin wave excitations. For a number of applications, it would be highly desirable to shape and coherently…
We suggest to excite dipole-forbidden transitions in quantum-mechanical systems by using appropriately designed optical nanoantennas. The antennas are tailored such that their near-field contains sufficiently strong contributions of…
We study a means of creating multiparticle entanglement of neutral atoms using pairwise controlled dipole-dipole interactions in a three dimensional optical lattice. For tightly trapped atoms the dipolar interaction energy can be much…
This article reviews experimental work on the ultrafast electron dynamics in the topological surface state (TSS) of three-dimensional (3D) topological insulators (TIs) observed with time- and angle-resolved two-photon photoemission (2PPE).…
We investigate coherent electron dynamics in graphene, interacting with the electric field waveform of two orthogonally polarized, few-cycle laser pulses. Recently, we demonstrated that linearly polarized driving pulses lead to…
We report on two-photon interference (TPI) experiments using remote deterministic single-photon sources. Employing 3D in-situ electron-beam lithography, we fabricate quantum-light sources at specific target wavelengths by integrating…
Dipole spin-wave states of atomic ensembles with wave vector ${\bf k}(\omega)$ mismatched from the dispersion relation of light are difficult to access by far-field excitation but may support rich phenomena beyond the traditional…
Photoassociation with short laser pulses has been proposed as a technique to create ultracold ground state molecules. A broad-band excitation seems the natural choice to drive the series of excitation and deexcitation steps required to form…
We show that very large nonlocal nonlinear interactions between pairs of colliding slow-light pulses can be realized in atomic vapors in the regime of electromagnetically induced transparency. These nonlinearities are mediated by strong,…
In this work we present a cavity-enhanced InAs/$\mathrm{In_{0.53}Al_{0.23}Ga_{0.24}As}$ quantum dot (QD) single-photon source in the telecom C-band with a record-low biexciton emitter decay time of \SI{67.4(2)}{ps} under resonant two-photon…
We propose an efficient all-optical phase modulation based on a double-{\Lambda} system and demonstrate a {\pi} phase shift of a few-photon pulse induced by another few-photon pulse in cold rubidium atoms with this scheme. By changing the…