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The application of magnetic resonance (MR) spectroscopy at progressively smaller length scales may eventually permit "chemical imaging" of spins at the surfaces of materials and biological complexes. In particular, the negatively charged…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Hai-Jing Wang , Chang S. Shin , Scott J. Seltzer , Claudia E. Avalos , Alexander Pines , Vikram S. Bajaj

We investigate optically detected magnetic resonance signals from an ensemble of nitrogen-vacancy centers in diamond. The signals are measured for different light powers and microwave powers, and the contrast and linewidth of the…

Quantum Physics · Physics 2015-06-11 K. Jensen , V. M. Acosta , A. Jarmola , D. Budker

We use tunable dipolar-interactions between the spins of nitrogen-vacancy (NV) centers in diamond to rotate a diamond crystal. Specifically, we employ cross-relaxation between the electronic spin of pairs of NV centers in a trapped diamond…

Mesoscale and Nanoscale Physics · Physics 2021-09-22 C. Pellet-Mary , P. Huillery , M. Perdriat , G. Hétet

In this work we use fluorescence from nitrogen-vacancy defects in diamond to detect and explore other paramagnetic defects in the diamond, such as P1 defects, which are commonly undetectable through optical detection of magnetic resonance…

Quantum Physics · Physics 2019-07-03 Nir Alfasi , Sergei Masis , Oleg Shtempluck , Eyal Buks

We present a protocol that detects molecular conformational changes with two nitroxide electron-spin labels and a nitrogen-vacancy (NV) center in diamond. More specifically, we demonstrate that the NV can detect energy shifts induced by the…

Quantum Physics · Physics 2022-12-21 C. Munuera-Javaloy , R. Puebla , B. D'Anjou , M. B. Plenio , J. Casanova

Optically detected magnetic resonance of nitrogen vacancy centers in diamond offers novel routes to both DC and AC magnetometry in diamond anvil cells under high pressures ($>3$ GPa). However, a serious challenge to realizing experiments…

Instrumentation and Detectors · Physics 2017-11-29 L. Steele , M. Lawson , M. Onyszczak , B. T. Bush , Z. Mei , A. P. Dioguardi , J. King , A. Parker , A. Pines , S. T. Weir , W. Evans , K. Visbeck , Y. K. Vohra , N. J. Curro

We study the coupling of a single nitrogen-vacancy center in diamond to a nearby single nitrogen defect at room temperature. The magnetic dipolar coupling leads to a splitting in the electron spin resonance frequency of the nitrogen-vacancy…

Quantum Physics · Physics 2007-05-23 R. Hanson , F. M. Mendoza , R. J. Epstein , D. D. Awschalom

Polarons can control carrier mobility and can also be used in the design of quantum devices. Although much effort has been directed into investigating the nature of polarons, observation of defect-related polarons is challenging due to…

Materials Science · Physics 2024-09-11 Takuto Ichikawa , Junjie Guo , Paul Fons , Dwi Prananto , Toshu An , Muneaki Hase

We report a study of the magnetic field dependence of photoluminescence of NV$^-$ centers (negatively charged nitrogen-vacancy centers) in diamond single crystals. In such a magnetic field dependence characteristic sharp features are…

Quantum Physics · Physics 2017-09-27 Sergei V. Anishchik , Konstantin L. Ivanov

We give instructions for the construction and operation of a simple apparatus for performing optically detected magnetic resonance measurements on diamond samples containing high concentrations of nitrogen-vacancy (NV) centers. Each NV…

Mesoscale and Nanoscale Physics · Physics 2018-03-14 Haimei Zhang , Carina Belvin , Wanyi Li , Jennifer Wang , Julia Wainwright , Robbie Berg , Joshua Bridger

Magnetic Resonance Imaging (MRI) can characterize and discriminate among tissues using their diverse physical and biochemical properties. Unfortunately, submicrometer screening of biological specimens is presently not possible, mainly due…

Mesoscale and Nanoscale Physics · Physics 2010-11-03 C. A. Meriles , L. Jiang , G. Goldstein , J. S. Hodges , J. R. Maze , M. D. Lukin , P. Cappellaro

Nitrogen-vacancy centers in diamond allow for coherent spin state manipulation at room temperature, which could bring dramatic advances to nanoscale sensing and quantum information technology. We introduce a novel method for the optical…

We study the depolarization dynamics of a dense ensemble of dipolar interacting spins, associated with nitrogen-vacancy centers in diamond. We observe anomalously fast, density-dependent, and non-exponential spin relaxation. To explain…

The coherence characteristics of a tin-vacancy color center in diamond are investigated through optical means including coherent population trapping between the ground state orbital levels and linewidth broadening effects. Due to the large…

Magnetic resonance techniques provide a powerful tool for controlling spin systems, with applications ranging from quantum information processing to medical imaging. Nevertheless, the behavior of a spin system under strong excitation…

Quantum Physics · Physics 2015-05-19 Lilian Childress , Jean McIntyre

Using an optical tweezers apparatus, we demonstrate three-dimensional control of nanodiamonds in solution with simultaneous readout of ground-state electron-spin resonance (ESR) transitions in an ensemble of diamond nitrogen-vacancy (NV)…

We report quantitative measurements of optically detected ferromagnetic resonance (ODFMR) of ferromagnetic thin films that use nitrogen-vacancy (NV) centers in diamonds to transduce FMR into a fluorescence intensity variation. To uncover…

Symmetry considerations are used in presenting a model of the electronic structure and the associated dynamics of the nitrogen-vacancy center in diamond. The model accounts for the occurrence of optically induced spin polarization, for the…

Materials Science · Physics 2013-05-29 N. B. Manson , J. P. Harrison , M. J. Sellars

We report a study of the magnetic field dependence of the photo-luminescence of NV$^-$ centers (negatively charged nitrogen-vacancy centers) in diamond single crystals. In such a magnetic field dependence characteristic lines are observed,…

Quantum Physics · Physics 2016-09-23 Sergei V. Anishchik , Konstantin L. Ivanov

We study features in the optically detected magnetic resonance (ODMR) signals associated with negatively charged nitrogen-vacancy (NV) centers coupled to other paramagnetic impurities in diamond. Our results are important for understanding…

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