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Frequency mixing processes in spin systems have a variety of applications in meteorology and in quantum data processing. Spin spectroscopy based on frequency mixing offers some advantages, including the ability to eliminate crosstalk…

Quantum Physics · Physics 2023-10-13 Mohammed Attrash , Sergei Masis , Sergey Hazanov , Oleg Shtempluck , Eyal Buks

The protocols for the control and readout of Nitrogen Vacancy (NV) centres electron spins in diamond offer an advanced platform for quantum computation, metrology and sensing. These protocols are based on the optical readout of photons…

Mesoscale and Nanoscale Physics · Physics 2019-06-26 E. Bourgeois , A. Jarmola , M. Gulka , J. Hruby , D. Budker , M. Nesladek

Paramagnetic magnetic resonance, a powerful technique for characterizing and identifying chemical targets, is increasingly used for imaging; however, low spin polarization at room temperature and moderate magnetic fields poses challenges…

Mesoscale and Nanoscale Physics · Physics 2019-09-04 C. M. Purser , V. P. Bhallamudi , C. S. Wolfe , H. Yusuf , B. A. McCullian , C. Jayaprakash , M. E. Flatté , P. C. Hammel

Near-surface nitrogen-vacancy (NV) centers have been created in diamond through low energy implantation of 15N to sense electron spins that are external to the diamond. By performing double resonance experiments, we have verified the…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 H. J. Mamin , M. H. Sherwood , D. Rugar

Nanodiamonds containing nitrogen vacancy (NV-) centers show promise for a number of emerging applications including targeted in vivo imaging and generating nuclear spin hyperpolarization for enhanced NMR spectroscopy and imaging. Here, we…

We present the development of an optically detected magnetic resonance (ODMR) system, which enables us to perform the ODMR measurements of a single defect in solids at high frequencies and high magnetic fields. Using the high-frequency and…

Mesoscale and Nanoscale Physics · Physics 2015-02-12 Viktor Stepanov , Franklin H. Cho , Chathuranga Abeywardana , Susumu Takahashi

We investigate spin and optical properties of individual nitrogen-vacancy centers located within 1-10 nm from the diamond surface. We observe stable defects with a characteristic optically detected magnetic resonance spectrum down to lowest…

Mesoscale and Nanoscale Physics · Physics 2012-08-27 B. K. Ofori-Okai , S. Pezzagna , K. Chang , M. Loretz , R. Schirhagl , Y. Tao , B. A. Moores , K. Groot-Berning , J. Meijer , C. L. Degen

The nitrogen-vacancy (NV) defect center in diamond has demonstrated great capability for nanoscale magnetic sensing and imaging for both static and periodically modulated target fields. However, it remains a challenge to detect and image…

Mesoscale and Nanoscale Physics · Physics 2014-09-19 Lan Luan , Michael S. Grinolds , Sungkun Hong , Patrick Maletinsky , Ronald L. Walsworth , Amir Yacoby

Optically active spin defects in solids are promising platforms for quantum technologies. Here, we present a first-principles framework to investigate intersystem crossing processes, which represent crucial steps in the optical…

Nitrogen-vacancy (NV) centers in diamond can be used for nanoscale sensing with atomic resolution and sensitivity; however, it has been observed that their properties degrade as they approach the diamond surface. Here we report that in…

The nitrogen-vacancy (NV) color center in diamond is an atom-like system in the solid-state which specific spin properties can be efficiently used as a sensitive magnetic sensor. An external magnetic field induces Zeeman shifts of the NV…

Mesoscale and Nanoscale Physics · Physics 2015-07-17 M. Chipaux , A. Tallaire , J. Achard , S. Pezzagna , J. Meijer , V. Jacques , J. -F. Roch , T. Debuisschert

Using pulsed photoionization the coherent spin manipulation and echo formation of ensembles of NV- centers in diamond are detected electrically realizing contrasts of up to 17 %. The underlying spin-dependent ionization dynamics are…

Mesoscale and Nanoscale Physics · Physics 2017-01-25 Florian M. Hrubesch , Georg Braunbeck , Martin Stutzmann , Friedemann Reinhard , Martin S. Brandt

We discuss the side resonances of optically detected magnetic resonance in diamond crystal and propose the new approach to the calculation of hyperfine interaction in composed system, consisted of negatively charged nitrogen-vacancy NV-…

Mesoscale and Nanoscale Physics · Physics 2017-01-17 Alexander Ivanov , Alexei Ivanov

We report sensitive detection of the nuclear quadrupolar interaction of the 14N nuclear spin of the nitrogen-vacancy (NV) center using the electron spin echo envelope modulation technique. We applied a weak transverse magnetic field to the…

Statistical mechanics underlies our understanding of macroscopic quantum systems. It is based on the assumption that out-of-equilibrium systems rapidly approach their equilibrium states, forgetting any information about their microscopic…

The excited orbitals of color centers typically show stronger electric dipoles, which can serve as a resource for entanglement, emission tuning, or electric field sensing. Here, we use resonant laser excitation to expose strong transition…

The nitrogen-vacancy center in diamond attracts a lot of attention in sensing applications, mainly for temperature, magnetic field, and rotation measurements. Nuclear spins of carbon-13 surrounding the nitrogen-vacancy center can be used as…

In this paper we study the dynamics of an ensemble of nitrogen-vacancy centers in diamond when its photoluminescence is detected by means of a widefield imaging system. We develop a seven-level model and use it to simulate the widefield…

Quantum Physics · Physics 2023-09-13 Simone Magaletti , Ludovic Mayer , Jean-François Roch , Thierry Debuisschert

We study spin relaxation and diffusion in an electron-spin ensemble of nitrogen impurities in diamond at low temperature (0.25-1.2 K) and polarizing magnetic field (80-300 mT). Measurements exploit mode- and temperature-dependent coupling…

Mesoscale and Nanoscale Physics · Physics 2013-02-13 V. Ranjan , G. de Lange , R. Schutjens , T. Debelhoir , J. P. Groen , D. Szombati , D. J. Thoen , T. M. Klapwijk , R. Hanson , L. DiCarlo

We report a study of high-resolution microwave spectroscopy of nitrogen-vacancy centers in diamond crystals at and around zero magnetic field. We observe characteristic splitting and transition imbalance of the hyperfine transitions, which…