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Few-layer CrI$_3$ is the most known example among two-dimensional (2D) ferromagnets, which have attracted growing interest in recent years. Despite considerable efforts and progress in understanding the properties of 2D magnets both from…

Strongly Correlated Electrons · Physics 2021-01-14 I. V. Kashin , V. V. Mazurenko , M. I. Katsnelson , A. N. Rudenko

The latest discovery of ferromagnetism in atomically thin films of semiconductors Cr$_2$Ge$_2$Te$_6$ and CrI$_3$ has unleashed numerous opportunities for fundamental physics of magnetism in two-dimensional (2D) limit and also for…

Mesoscale and Nanoscale Physics · Physics 2019-05-09 Vijay Kumar Gudelli , Guang-Yu Guo

After the discovery of magnetism in monolayer CrI3, the magnetic properties of different 2D materials from the chromium-trihalide family are intuitively assumed to be similar, yielding magnetic anisotropy from the spin-orbit coupling on…

Mesoscale and Nanoscale Physics · Physics 2021-03-24 C. Bacaksiz , D. Šabani , R. M. Menezes , M. V. Milošević

Atomically thin films of layered chromium triiodide (CrI$_3$) have recently been regarded as suitable candidates to a wide spectrum of technologically relevant applications, mainly owing to the opportunity they offer to achieve a reversible…

Strongly Correlated Electrons · Physics 2020-05-01 Michele Pizzochero , Oleg V. Yazyev

We performed the detailed microscopic analysis of the inter-layer magnetic couplings for bilayer CrI$_3$. As the first step toward understanding the recent experimental observations and utilizing them for device applications, we estimated…

Materials Science · Physics 2019-04-10 Seung Woo Jang , Min Yong Jeong , Hongkee Yoon , Siheon Ryee , Myung Joon Han

The discovery of 2-dimensional (2D) materials, such as CrI3, that retain magnetic ordering at monolayer thickness has resulted in a surge of research in 2D magnetism from both pure and applied perspectives. Here, we report a magneto-Raman…

We conduct a comprehensive study of three different magnetic semiconductors, CrI$_3$, CrBr$_3$, and CrCl$_3$, by incorporating both few- and bi-layer samples in van der Waals tunnel junctions. We find that the interlayer magnetic ordering,…

Motivated by the recent wealth of exotic magnetic phases emerging in two-dimensional frustrated lattices, we investigate the origin of possible magnetism in the monolayer family of triangular lattice materials $MX_2$ ($M$={V, Mn, Ni},…

The first magnetic 2D material discovered, monolayer (ML) CrI$_3$, is particularly fascinating due to its ground state ferromagnetism. Yet, because monolayer materials are difficult to probe experimentally, much remains unresolved about ML…

We apply the density-functional theory to study various phases (including non-magnetic (NM), anti-ferromagnetic (AFM), and ferromagnetic (FM)) in monolayer magnetic chromium triiodide (CrI$_3$), a recently fabricated 2D magnetic material.…

Mesoscale and Nanoscale Physics · Physics 2018-10-17 Lucas Webster , Liangbo Liang , Jia-An Yan

The marked interplay between the crystalline, electronic, and magnetic structure of atomically thin magnets has been regarded as the key feature for designing next-generation magneto-optoelectronic devices. In this respect, a detailed…

Strongly Correlated Electrons · Physics 2020-05-25 Michele Pizzochero , Ravi Yadav , Oleg V. Yazyev

Curved magnets attract considerable interest for their unusually rich phase diagram, often encompassing exotic (e.g., topological or chiral) spin states. Micromagnetic simulations are playing a central role in the theoretical understanding…

Materials Science · Physics 2022-05-11 Alexander Edström , Danila Amoroso , Silvia Picozzi , Paolo Barone , Massimiliano Stengel

Bright excitons in ferromagnetic monolayers CrI$_3$ efficiently interact with lattice magnetization, which makes possible all-optical resonant magnetization control in this material. Using the combination of ab-initio simulations within…

Mesoscale and Nanoscale Physics · Physics 2023-05-23 A. Kudlis , M. Kazemi , Y. Zhumagulov , H. Schrautzer , P. F. Bessarab , I. V. Iorsh , I. A. Shelykh

Following the recent isolation of monolayer CrI3, there has been a surge of new two-dimensional van der Waals magnetic materials, whose incorporation in van der Waals heterostructures offers a new platform for spintronics, proximity…

A recent theoretical study reported large effects of perpendicular electric fields on the atomic structure of a monolayer CrI3, which could be related to the microscopic origin of the technologically promising and experimentally observed…

Materials Science · Physics 2019-07-24 S. Ghosh , N. Stojic , N. Binggeli

The exploration of magnetism in two-dimensional layered materials has attracted extensive research interest. For the monoclinic phase CrI3 with interlayer antiferromagnetism, finding a static and robust way of realizing the intrinsic…

Materials Science · Physics 2022-11-30 Shiyang Sun , Xuyan Chen , Xuqi Li , Huihui Zhang , Haidan Sang , Shifei Qi , Zhenhua Qiao

The newly discovered 2D magnetic materials provide new opportunities for basic physics and device applications. However, their low Curie temperature (TC) is a common weakness. In this paper, by combining magnetic Hamiltonian, Wannier…

Materials Science · Physics 2020-11-06 Hongxing Li , Zi-Peng Cheng , Bin-Guang He , Wei-Bing Zhang

The pertinent need for microscopic understanding of magnetic exchange motivated us to go beyond the existing theories and develop a systematic method to quantify all possible mechanisms that contribute to magnetic exchange for an arbitrary…

Materials Science · Physics 2025-02-13 Denis Šabani , Cihan Bacaksız , Milorad V. Milošević

Chromium triiodide is an intrinsically magnetic van der Waals material down to the single-layer limit. Here, we provide a first-principles description of finite-temperature magnetic and spectral properties of monolayer (ML) CrI$_3$ based on…

Strongly Correlated Electrons · Physics 2022-05-24 Yaroslav O. Kvashnin , Alexander N. Rudenko , Patrik Thunström , Malte Rösner , Mikhail I. Katsnelson

Two-dimensional (2D) materials with intrinsic ferromagnetism provide unique opportunity to engineer new functionalities in nano-spintronics. One such material is CrI$_3$, showing long-range magnetic order in monolayer with the Curie…

Strongly Correlated Electrons · Physics 2019-09-20 Yu Liu , Lijun Wu , Xiao Tong , Jun Li , Jing Tao , Yimei Zhu , C. Petrovic
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