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Excitons in monolayer semiconductors have large optical transition dipole for strong coupling with light field. Interlayer excitons in heterobilayers, with layer separation of electron and hole components, feature large electric dipole that…

Mesoscale and Nanoscale Physics · Physics 2019-03-07 Wei-Ting Hsu , Bo-Han Lin , Li-Syuan Lu , Ming-Hao Lee , Ming-Wen Chu , Lain-Jong Li , Wang Yao , Wen-Hao Chang , Chih-Kang Shih

Topological insulators represent a paradigm shift in surface physics. The most extensively studied Bi$_2$Se$_3$-type topological insulators exhibit layered structures, wherein neighboring layers are weakly bonded by van der Waals…

Materials Science · Physics 2016-01-22 Can Li , Torben Winzer , Aron Walsh , Binghai Yan , Catherine Stampfl , Aloysius Soon

Monolayers of transition metal dichalcogenides (TMdC) are promising candidates for realization of a new generation of optoelectronic devices. The optical properties of these two-dimensional materials, however, vary from flake to flake, or…

Materials Science · Physics 2020-01-22 Pavel V. Kolesnichenko , Qianhui Zhang , Changxi Zheng , Michael S. Fuhrer , Jeffrey A. Davis

We have realized ambipolar ionic liquid gated field-effect transistors based on WS2 mono- and bilayers, and investigated their opto-electronic response. A thorough characterization of the transport properties demonstrates the high quality…

Mesoscale and Nanoscale Physics · Physics 2014-04-11 Sanghyun Jo , Nicolas Ubrig , Helmuth Berger , Alexey B. Kuzmenko , Alberto F. Morpurgo

We present thermoelectric properties of Be$_2$C monolayer based on density functional theory and semi-classical Boltzmann transport theory. Electronic structure calculations predict this material as a semiconductor with a direct bandgap of…

Materials Science · Physics 2022-01-27 Gautam Sharma , K. C. Bhamu

It has been shown recently that the coefficient of collective diffusion in a colloidal monolayer is divergent due to the hydrodynamic interactions mediated by the ambient fluid in bulk. The analysis is extended to allow for time--dependent…

Soft Condensed Matter · Physics 2015-01-23 Alvaro Domínguez

Optically generated excitons dictate the absorption and emission spectrum of doped semiconductor transition metal dichalcogenide monolayers. We show that upon increasing the electron density, the elementary optical excitations develop a…

Mesoscale and Nanoscale Physics · Physics 2020-05-20 Ovidiu Cotlet , Dominik S. Wild , Mikhail D. Lukin , Atac Imamoglu

The polarization analysis of optical transitions in monolayer and bilayer transition-metal dichalcogenides provides invaluable information on the spin and valley (pseudospin) degrees of freedom. To explain optical properties of a given…

Materials Science · Physics 2015-10-06 Hanan Dery , Yang Song

The first magnetic 2D material discovered, monolayer (ML) CrI$_3$, is particularly fascinating due to its ground state ferromagnetism. Yet, because monolayer materials are difficult to probe experimentally, much remains unresolved about ML…

Optical spectroscopy in high magnetic fields $B\leq65$ T is used to reveal the very different nature of carriers in monolayer and bulk transition metal dichalcogenides. In monolayer WSe$_{2}$, the exciton emission shifts linearly with the…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 A. A. Mitioglu , P. Plochocka , Á. Granados del Aguila , P. C. M. Christianen , G. Deligeorgis , S. Anghel , L. Kulyuk , D. K. Maude

The topological properties of the bulk band structure of a three-dimensional topological insulator (TI) manifest themselves in the form of metallic surface states. In this paper, we propose a probe which directly couples to an exotic…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Sthitadhi Roy , Kush Saha , Sourin Das

The twist angle between the monolayers in van der Waals heterostructures provides a new degree of freedom in tuning material properties. We compare the optical properties of WSe2 homobilayers with 2H and 3R stacking using photoluminescence,…

Monolayer MnBi$_{2}$Te$_{4}$ (MBT) is an intrinsically magnetic topological insulator whose magnetic response is strongly affected by strain and electron correlation. In density functional theory with an on-site Hubbard correction…

Monolayers of transition metal dichalcogenides present an intriguing platform to investigate the interplay of excitonic complexes in two dimensional semiconductors. Here, we use optical spectroscopy to study light-matter coupling and…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 Jonas Zipfel , Koloman Wagner , Jonas D. Ziegler , Takashi Taniguchi , Kenji Watanabe , Marina A. Semina , Alexey Chernikov

We determined the complex dielectric functions of $\varepsilon$-Ga$_2$O$_3$ using optical transmittance and reflectance spectroscopies at temperatures from 10 K to room temperature. The measured dielectric-function spectra reveal distinct…

Materials Science · Physics 2023-11-01 T. Makino , S. Yusa , D. Oka , T. Fukumura

In heterostructures consisting of different transition-metal dichalcogenide monolayers, a staggered band alignment can occur, leading to rapid charge separation of optically generated electron-hole pairs into opposite monolayers. These…

We report a post-growth aging mechanism of Bi$_2$Te$_3$(111) films with scanning tunneling microscopy in combination with density functional theory calculation. It is found that a monolayered structure with a squared lattice symmetry…

Materials Science · Physics 2017-04-05 Zhi-Wen Wang , Wen-Kai Huang , Kai-Wen Zhang , Da-Jun Shu , Mu Wang , Shao-Chun Li

Beyond-diffraction-limit optical absorption spectroscopy provides profound information on the graded band structures of composition-spread and stacked two-dimensional materials, in which direct/indirect bandgap, interlayer coupling,…

Atomically thin two-dimensional crystals have revolutionized materials science. In particular, monolayer transition metal dichalcogenides promise novel optoelectronic applications, due to their direct energy gaps in the optical range. Their…

Single-layer WS$_2$ is a direct-gap semiconductor showing strong excitonic photoluminescence features in the visible spectral range. Here, we present temperature-dependent photoluminescence measurements on mechanically exfoliated…

Mesoscale and Nanoscale Physics · Physics 2015-09-08 Gerd Plechinger , Philipp Nagler , Julia Kraus , Nicola Paradiso , Christoph Strunk , Christian Schüller , Tobias Korn