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We propose a distant-neighbor quantum-mechanical (DNQM) approach to study the linear and nonlinear optical properties of graphene nanoflakes (GNFs). In contrast to the widely used tight-binding description of the electronic states that…

Mesoscale and Nanoscale Physics · Physics 2018-02-08 Hanying Deng , David Zs. Manrique , Xianfeng Chen , Nicolae C. Panoiu , Fangwei Ye

Localized plasmons in metallic nanostructures have been widely used to enhance nonlinear optical effects due to their ability to concentrate and enhance light down to extreme-subwavelength scales. As alternatives to noble metal…

Mesoscale and Nanoscale Physics · Physics 2015-02-24 Joel D. Cox , F. Javier Garcia de Abajo

Intense efforts have been made in recent years to realize nonlinear optical interactions at the single-photon level. Much of this work has focused on achieving strong third-order nonlinearities, such as by using single atoms or other…

Mesoscale and Nanoscale Physics · Physics 2015-08-25 Marco T. Manzoni , Iván Silveiro , F. Javier García de Abajo , Darrick E. Chang

Electrically tunable graphene plasmons are anticipated to enable strong light-matter interactions with resonant quantum emitters. However, plasmon resonances in graphene are typically limited to infrared frequencies, below those of optical…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Joel D. Cox , F. Javier García de Abajo

The optical nonlinear effects can provide different advanced electromagnetic functionalities, such as wave mixing and phase conjugation, which can be applied in a variety of new applications. However, these effects usually suffer from…

Optics · Physics 2020-06-29 Boyuan Jin , Christos Argyropoulos

Graphene is known to possess strong optical nonlinearity. Its nonlinear response can be further enhanced by graphene plasmons. Here, we report a novel nonlinear electro-absorption effect observed in nanostructured graphene due to excitation…

Mesoscale and Nanoscale Physics · Physics 2018-02-14 D. Kundys , B. Van Duppen , O. P. Marshall , F. Rodriguez , I. Torre , A. Tomadin , M. Polini , A. N. Grigorenko

We study topologically-protected four-wave mixing (FWM) interactions in a plasmonic metasurface consisting of a periodic array of nanoholes in a graphene sheet, which exhibits a wide topological bandgap at terahertz frequencies upon the…

Optics · Physics 2020-04-07 Jian Wei You , Zhihao Lan , Nicolae C. Panoiu

We analyze nonlinear optics schemes for generating pairs of quantum entangled plasmons in the terahertz-infrared range in graphene. We predict that high plasmonic field concentration and strong optical nonlinearity of monolayer graphene…

Mesoscale and Nanoscale Physics · Physics 2022-06-17 Zhiyuan Sun , D. N. Basov , M. M. Fogler

Infrared spectroscopy, especially for molecular vibrations in the fingerprint region between 600 and 1500 cm-1, is a powerful characterization method for bulk materials. However, molecular fingerprinting at the nanoscale level still remains…

Optics · Physics 2016-08-24 Hai Hu , Xiaoxia Yang , Feng Zhai , Debo Hu , Ruina Liu , Kaihui Liu , Zhipei Sun , Qing Dai

Although plasmon modes exist in doped graphene, the limited range of doping achieved by gating restricts the plasmon frequencies to a range that does not include visible and infrared. Here we show, through the use of first-principles…

Mesoscale and Nanoscale Physics · Physics 2018-05-30 Sharmila N. Shirodkar , Marios Mattheakis , Paul Cazeaux , Prineha Narang , Marin Soljačić , Efthimios Kaxiras

Using a powerful homogenization technique, one- and two-dimensional graphene metasurfaces are homogenized both at the fundamental frequency (FF) and second harmonic (SH). In both cases, there is excellent agreement between the predictions…

Optics · Physics 2019-05-17 Qun Ren , J. W. You , N. C. Panoiu

It has recently been demonstrated that difference frequency mixing (DFM) can generate surface plasmons in graphene [1]. Here, we present detailed calculations comparing the contributions to this effect from substrate and from graphene…

We investigate the nonlinear optical response of graphene nanoribbon (GNR) heterojunctions both without and with one or multiple topological interface states. By implementing a distant-neighbor quantum-mechanical (DNQM) method, we…

Mesoscale and Nanoscale Physics · Physics 2024-12-10 Hanying Deng , Yaxin Li , Zhihao qu , Jing Deng , Yingji He , Fangwe Ye

The linear electronic dispersion relation of graphene endows the atomically thin carbon layer with a large intrinsic optical nonlinearity, with regard to both parametric and photothermal processes. While plasmons in graphene nanostructures…

Mesoscale and Nanoscale Physics · Physics 2026-02-05 Line Jelver , Joel D. Cox

The observation and electrical manipulation of infrared surface plasmons in graphene have triggered a search for similar photonic capabilities in other atomically thin materials that enable electrical modulation of light at visible and…

Mesoscale and Nanoscale Physics · Physics 2017-02-08 F. Javier Garcia de Abajo , Alejandro Manjavacas

The ability of graphene to support long-lived, electrically tunable plasmons that interact strongly with light, combined with its highly nonlinear optical response, has generated great expectations for application of the atomically-thin…

Mesoscale and Nanoscale Physics · Physics 2017-04-12 Joel D. Cox , Iván Silveiro , F. Javier García de Abajo

Nonlinear nanophotonics leverages engineered nanostructures to funnel light into small volumes and intensify nonlinear optical processes with spectral and spatial control. Due to its intrinsically large and electrically tunable nonlinear…

We study the nonlinear optical properties of heterojunctions made of graphene nanoribbons (GNRs) consisting of two segments with either the same or different topological properties. By utilizing a quantum mechanical approach that…

The directional control of light in miniaturized plasmonic waveguides holds appealing possibilities for emerging nanophotonic technologies, but is hindered by the intrinsic reciprocal optical response of conventional plasmonic materials.…

Mesoscale and Nanoscale Physics · Physics 2026-02-05 Álvaro Rodríguez Echarri , F. Javier García de Abajo , Joel D. Cox

We present the first experimental investigation of nonlinear optical properties of graphene flakes. We find that at near infrared frequencies a graphene monolayer exhibits a remarkably high third-order optical nonlinearity which is…

Materials Science · Physics 2011-01-13 E. Hendry , P. J. Hale , J. J. Moger , A. K. Savchenko , S. A. Mikhailov
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