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Dynamical simulations of polaron transport in conjugated polymers in the presence of an external time-dependent electric field have been performed within a combined extended Hubbard model (EHM) and Su-Schrieffer-Heeger (SSH) model. Nearly…

Materials Science · Physics 2016-09-28 Haibo Ma , Ulrich Schollwoeck

While the dynamics of a fully flexible polymer ejecting a capsid through a nanopore has been extensively studied, the ejection dynamics of semiflexible polymers has not been properly characterized. Here we report results from simulations of…

Biological Physics · Physics 2017-11-08 Riku P. Linna , Pauli M. Suhonen , Joonas Piili

The characterization of the interactions between two fully flexible self-avoiding polymers is one of the classic and most important problems in polymer physics. In this paper we measure these interactions in the presence of active…

Soft Condensed Matter · Physics 2022-04-06 M. C. Gandikota , A. Cacciuto

Molecular dynamics simulations of interacting soft disks confined in a heterogeneous quenched matrix of soft obstacles show dynamics which is fundamentally different from that of hard disks. The interactions between the disks can enhance…

Soft Condensed Matter · Physics 2018-02-21 Simon Kaspar Schnyder , Jürgen Horbach

We study the effect of the crowded nature of the cellular cytoplasm on the translocation of a polymer through a pore in a membrane. By systematically treating the entropic penalty due to crowding, we show that the translocation dynamics are…

Soft Condensed Matter · Physics 2009-11-13 Ajay Gopinathan , Yong Woon Kim

Starting from the reported experimental evidence that the residence time of contacts between the ends of biopolymers is length dependent, we investigate the kinetics of contact breaking in simple polymer models from a theoretical point of…

Soft Condensed Matter · Physics 2024-12-19 E. Marchi , G. Tiana

The phase behaviour of a single large semiflexible polymer immersed in a suspension of spherical particles is studied. All interactions are simple excluded volume interactions and the diameter of the spherical particles is an order of…

Soft Condensed Matter · Physics 2009-10-30 Richard P. Sear

We present a Brownian dynamics model of driven polymer translocation, in which non-equilibrium memory effects arising from tension propagation (TP) along the cis side subchain are incorporated as a time-dependent friction. To solve the…

Soft Condensed Matter · Physics 2015-06-03 Timo Ikonen , Aniket Bhattacharya , Tapio Ala-Nissila , Wokyung Sung

We analyze the translocation of a charged particle across an Alpha-Hemolysin (aHL) pore in the framework of a driven diffusion over an extended energy barrier generated by the electrical charges of the aHL. A one-dimensional electrostatic…

Biomolecules · Quantitative Biology 2015-10-15 Patrizio Ansalone , Mauro Chinappi , Lamberto Rondoni , Fabio Cecconi

Monte Carlo simulations have been performed to analyze the sub-diffusion dynamics of a tagged monomer in self-avoiding polymerized membranes in the flat phase. By decomposing the mean square displacement into the out-of-plane ($\parallel$)…

Soft Condensed Matter · Physics 2015-06-22 Ken-ichi Mizuochi , Hiizu Nakanishi , Takahiro Sakaue

We discuss multiscale simulations of long biopolymer translocation through wide nanopores that can accommodate multiple polymer strands. The simulations provide clear evidence of folding quantization, namely, the translocation proceeds…

Biological Physics · Physics 2009-11-13 Simone Melchionna , Massimo Bernaschi , Maria Fyta , Efthimios Kaxiras , Sauro Succi

Sensitive sequencing of biopolymers by nanopore-based translocation techniques requires extension of the time spent by the molecule in the pore. We develop an electrostatic theory of polymer translocation to show that the translocation time…

Soft Condensed Matter · Physics 2018-11-12 Sahin Buyukdagli , Jalal Sarabadani , Tapio Ala-Nissila

We study analytically a model of a two dimensional, partially directed, flexible or semiflexible polymer, attached to an attractive wall which is perpendicular to the preferred direction. In addition, the polymer is stretched by an…

Statistical Mechanics · Physics 2015-05-13 Pui-Man Lam , Yi Zhen , Haijun Zhou , Jie Zhou

We consider the statics and dynamics of a flexible polymer confined between parallel plates both in the presence and absence of hydrodynamic interactions. The hydrodynamic interactions are described at the level of the fluctuating,…

Soft Condensed Matter · Physics 2012-11-01 Santtu T. T. Ollila , Colin Denniston , Mikko Karttunen , Tapio Ala-Nissila

We analyze the conformational dynamics and statistical properties of an active polymer model. The polymer is described as a freely-jointed bead-rod chain subject to stochastic active force dipoles that act on the suspending solvent where…

Soft Condensed Matter · Physics 2022-02-09 Achal Mahajan , David Saintillan

Stretched polymers with attractive interaction are studied in two and three dimensions. They are described by biased self-avoiding random walks with nearest neighbour attraction. The bias corresponds to opposite forces applied to the first…

Statistical Mechanics · Physics 2009-11-07 Peter Grassberger , Hsiao-Ping Hsu

Polymer transport is investigated for two paradigmatic laminar flows having open and closed streamlines, respectively. For both types of flows we find transport depletion owing to the action of the polymers elastic degree of freedom. For…

Chaotic Dynamics · Physics 2007-05-23 M. De Lucia , A. Mazzino , A. Vulpiani

The way tension propagates along a chain is a key to govern many of anomalous dynamics in macromolecular systems. After introducing the weak and the strong force regimes of the tension propagation, we focus on the latter, in which the…

Soft Condensed Matter · Physics 2015-04-27 Takuya Saito , Takahiro Sakaue

We present a hybrid quantum-classical simulation of charge-polaron transport in conjugated polymers. The charge, which couples to the angular rotations of the monomers, is modeled via the time-dependent Schr\"odinger equation, while the…

Statistical Mechanics · Physics 2022-01-11 Laszlo Berencei , William Barford , Stephen R. Clark

We study the dynamics of the passage of a stiff chain through a pore into a cell containing particles that bind reversibly to it. Using Brownian Molecular Dynamics simulations we investigate the mean-first-passage time as a function of the…

Soft Condensed Matter · Physics 2009-11-10 Roya Zandi , David Reguera , Joseph Rudnick , William M. Gelbart