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Protons at the water/vapor interface are relevant for atmospheric and environmental processes, yet to characterize their surface affinity on the quantitative level is still challenging. Here we utilize phase-sensitive sum-frequency…

Chemical Physics · Physics 2019-08-27 Kuo-Yang Chiang , Laetitia Dalstein , Yu-Chieh Wen

Raman scattering experiments have been carried out on single crystals of Nd$_{0.5}$Sr$_{0.5}$MnO$_3$ as a function of temperature in the range of 320-50 K, covering the paramagnetic insulator-ferromagnetc metal transition at 250 K and the…

Materials Science · Physics 2007-05-23 Md. Motin Seikh , A. K. Sood , Chandrabhas Narayana

Water/glycerol mixtures are common for experiments with biomacromolecules at cryogenic temperatures due to their vitrification properties. Above the glass transition temperature, they undergo liquid-liquid phase separation. Using the novel…

Soft Condensed Matter · Physics 2025-09-11 Sergei Kuzin , Maxim Yulikov

We have performed high-resolution inelastic neutron scattering studies on three samples of hydrogenated tetrahydrofuran-water clathrates, containing either H2 at different para/ortho concentrtion, or HD. By a refined analysis of the data,…

Materials Science · Physics 2009-11-13 L. Ulivi , M. Celli , A. Giannasi , A. J. Ramirez-Cuesta , D. J. Bull , M. Zoppi

Spectrally-resolved observations of three pure rotational lines of H$_2$, conducted with the EXES instrument on SOFIA toward the classic bow shock HH7, reveal systematic velocity shifts between the S(5) line of ortho-H$_2$ and the two…

Astrophysics of Galaxies · Physics 2019-06-19 David A. Neufeld , Curtis DeWitt , Pierre Lesaffre , Sylvie Cabrit , Antoine Gusdorf , Le Ngoc Tram , Matthew Richter

Dielectric spectra (10^4-10^11 Hz) of water and ice at 0 {\deg}C are considered in terms of proton conductivity and compared to each other. In this picture, the Debye relaxations, centered at 1/{\tau}_W ~ 20 GHz (in water) and 1/{\tau}_I ~…

Soft Condensed Matter · Physics 2020-05-19 V. G. Artemov , A. A. Volkov

Theoretical cross sections for the pressure broadening by hydrogen of rotational transitions of water are compared to the latest available measurements in the temperature range 65-220 K. A high accuracy interaction potential is employed in…

Chemical Physics · Physics 2015-05-19 Laurent Wiesenfeld , Alexandre Faure

Infrared vibration-rotation lines can be valuable probes of interstellar and circumstellar molecules, especially symmetric molecules, which have no pure rotational transitions. But most such observations have been interpreted with an…

Astrophysics of Galaxies · Physics 2015-06-15 John H. Lacy

Single crystals of the methylammonium (MA) lead halides MAPbI3, MAPbBr3, and MAPbCl3 have been investigated using infrared spectroscopy with the aim of analyzing structural and dynamical aspects of processes that enable the ordering of the…

Materials Science · Physics 2018-03-29 Götz Schuck , Daniel M. Többens , Monika Koch-Müller , Ilias Efthimiopoulos , Susan Schorr

High resolution spectra of Comet 8P/Tuttle were obtained in the frequency range 3440.6-3462.6 cm-1 on 3 January 2008 UT using CGS4 with echelle grating on UKIRT. In addition to recording strong solar pumped fluorescent (SPF) lines of H2O,…

Astrophysics · Physics 2010-05-12 R. J. Barber , S. Miller , N. Dello Russo , M. J. Mumma , J. Tennyson , P. Guio

This work explores the dynamics of capillary effects in pure H2O excited by hydrodynamic cavitation, which has been reported to introduce a non-equilibrium state of para- and ortho- isomers of water. Differential measurements are conducted…

Fluid Dynamics · Physics 2023-02-09 Serge Kernbach , Sergey M. Pershin

Recently we reported a high precision optical frequency measurement of the (v,L):(0,2)->(8,3) vibrational overtone transition in trapped deuterated molecular hydrogen (HD+) ions at 10 mK temperature. Achieving a resolution of 0.85…

Atomic Physics · Physics 2017-02-20 J. Biesheuvel , J. -Ph. Karr , L. Hilico , K. S. E. Eikema , W. Ubachs , J. C. J. Koelemeij

Absorption spectroscopy is a fundamental tool for probing molecular structure. However, performing absorption spectroscopy on individual molecules is challenging due to the low signal-to-noise ratio. Here, we report on a nondestructive…

Halogenated groups are relevant in pharmaceutical applications and potentially useful spectroscopic probes for infrared spectroscopy. In this work, the structural dynamics and infrared spectroscopy of $para$-fluorophenol (F-PhOH) and phenol…

We consider how the infrared intensity of an O-H stretch in a hydrogen bonded complex varies as the strength of the H-bond varies from weak to strong. We obtain trends for the fundamental and overtone transitions as a function of…

Chemical Physics · Physics 2017-03-30 Bijyalaxmi Athokpam , Sai G. Ramesh , Ross H. McKenzie

We have detected the S(1), S(2), S(3), S(4) and S(5) pure rotational lines of molecular hydrogen toward the outflow source HH 54, using the Short Wavelength Spectrometer (SWS) on board the Infrared Space Observatory (ISO). The observed H2…

Astrophysics · Physics 2007-05-23 David A. Neufeld , Gary J. Melnick , Martin Harwit

This work presents ground-based spectrally-resolved water emission at R = 30000-100000 over infrared wavelengths covered by JWST (2.9-12.8 $\mu$m). Two new surveys with iSHELL and VISIR are combined with previous spectra from CRIRES and…

In this work, we measured the absorption by CO2+H2O mixtures from 2400 to 2600 cm-1 which corresponds to the spectral region beyond the nu3 band head of CO2. Transmission spectra of CO2 mixed with water vapor were recorded with a…

Earth and Planetary Astrophysics · Physics 2018-02-28 Ha Tran , Martin Turbet , Pascale Chelin , Xavier Landsheere

Water is an important molecule in interstellar and circumstellar environments. Previous observations of mid-infrared rotational lines of OH suggest that these lines may be used to probe the photodissociation of water. In this work, cross…

Astrophysics of Galaxies · Physics 2021-06-30 Benoît Tabone , Marc C. van Hemert , Ewine F. van Dishoeck , John H. Black

Using a mid-infrared quantum cascade laser and wavelength modulation absorption spectroscopy, we measure the frequencies of ro-vibrational transitions of N$_2$O in the 17 $\mu$m region with uncertainties below 5 MHz. These lines,…

Atomic Physics · Physics 2025-12-10 Y. Wang , J. Rodewald , O. Lopez , M. Manceau , B. Darquié , B. E. Sauer , M. R. Tarbutt
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