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Two-photon excitation spectroscopy is a nonlinear technique that has gained rapidly in interest and significance for studying the complex energy-level structure and transition probabilities of materials. While the conventional spectroscopy…

Quantum Physics · Physics 2022-11-23 Yuanyuan Chen , Roberto de J. León-Montiel , Lixiang Chen

We propose a scheme for ultrafast real-time imaging of laser-induced collective electron oscillations (Mie plasmons) in gas phase metal clusters by interferometrically stable scanning of two intense few-cycle optical laser pulses. The…

Atomic Physics · Physics 2017-09-13 Jörg Köhn , Thomas Fennel

Forming new hybrid quasiparticles by strong light-matter coupling is a promising tool for tailoring photophysics and photochemistry of molecules. Thus, the ultrafast dynamics of polaritons formed upon strong light-matter coupling has been…

Chemical Physics · Physics 2025-05-23 Luca Nils Philipp , Eva Münzel , Julian Lüttig , Roland Mitrić

A common challenge in quantum information processing with photons is the limited ability to manipulate and measure correlated states. An example is the inability to measure picosecond scale temporal correlations of a multi-photon state,…

Photophysical and photochemical processes are ruled by the interplay between transient vibrational and electronic degrees of freedom, which are ultimately determined by the multidimensional potential energy surfaces (PESs). Differences…

We apply a pulsed-light interferometer to measure both the intensity and the phase of light that is transmitted through a strongly scattering disordered material. From a single set of measurements we obtain the time-resolved intensity,…

Disordered Systems and Neural Networks · Physics 2009-11-10 I. M. Vellekoop , P. Lodahl , A. Lagendijk

Another way to evaluate the spectral-correlation properties of thermal fields of solids is suggested. Such a method takes into account detailed structure of the interface transition layer separating one bulk region from those of the vacuum…

Quantum Physics · Physics 2015-06-15 Illarion Dorofeyev

We have developed x-ray diffraction measurements with high energy-resolution and accuracy to study water structure at three different temperatures (7, 25 and 66 C) under normal pressure. Using a spherically curved Ge crystal an energy…

Soft Condensed Matter · Physics 2017-09-13 Congcong Huang , K. T. Wikfeldt , D. Nordlund , U. Bergmann , T. McQueen , J. Sellberg , L. G. M. Pettersson , A. Nilsson

We propose a novel femtosecond stimulated Raman spectroscopy (FSRS) technique that combines entangled photons with interference detection to select matter pathways and enhance the resolution. Following photo excitation by an actinic pump,…

Quantum Physics · Physics 2014-07-15 Konstantin E. Dorfman , Frank Schlawin , Shaul Mukamel

X-ray photon correlation spectroscopy (XPCS) allows for the resolution of dynamic processes within a material across a wide range of length and time scales. X-ray speckle visibility spectroscopy (XSVS) is a related method that uses a single…

Numerical Analysis · Mathematics 2023-01-09 Shaswat Mohanty , Christopher B. Cooper , Hui Wang , Mengning Liang , Wei Cai

We present a study of the spectral properties of photon pairs generated through the process of spontaneous four wave mixing (SFWM) in single mode fiber. Our analysis assumes narrowband pumps, which are allowed to be frequency-degenerate or…

Gas-filled hollow-core photonic crystal fiber (PCF) is used for efficient nonlinear temporal compression of femtosecond laser pulses, two main schemes being direct soliton-effect self-compression, and spectral broadening followed by phase…

Optics · Physics 2020-07-15 F. Köttig , F. Tani , P. St. J. Russell

Ultrafast electron-photon spectroscopy in electron microscopes commonly requires ultrafast laser setups. Photoemission from an engineered electron source is used to generate pulsed electrons, interacting with a sample that is excited by the…

Mesoscale and Nanoscale Physics · Physics 2023-06-28 Masoud Taleb , Mario Hentschel , Kai Rossnagel , Harald Giessen , Nahid Talebi

Control of the temporal waveform of photons produced during spontaneous emission from single quantum emitters provides a crucial tool in the establishment of hybrid quantum systems, optimization of quantum state transfer protocols and…

Atomic Physics · Physics 2026-02-11 Carl Thomas , Rebecca Munk , Boris Blinov

Correlation-function expressions are derived for the coherent nonlinear response of molecules to three resonant ultrafast pulses in the x-ray regime. The ability to create two-core-hole states with controlled attosecond timing in…

Strongly Correlated Electrons · Physics 2009-11-11 Shaul Mukamel

The investigation of fluorescence lifetime became an important tool in biology and medical science. So far, established methods of fluorescence lifetime measurements require the illumination of the investigated probes with pulsed or…

Nonlinear spectroscopic techniques using entangled photon pairs can provide an opportunity to exploit non-classical correlations encoded in two-photon wavefunctions to manipulate two-exciton wavefunctions. We propose an entangled photon…

Quantum Physics · Physics 2026-04-10 Arunangshu Debnath , Shaul Mukamel

Measuring fluctuations in matter's low energy excitations is the key to unveil the nature of the nonequilibrium response of materials. A promising outlook in this respect is offered by spectroscopic methods that address matter fluctuations…

Two-color side-view probing of light-matter interaction from minute focal volume of a tightly focused fs-laser pump pulse reveals charge dynamics with high 0.9 micrometers optical resolution and approximately ~20 fs temporal resolution in…

Dye experimentation is a widely used method in experimental fluid mechanics for flow analysis or for the study of the transport of particles within a fluid. This technique is particularly useful in biomedical diagnostic applications ranging…

Fluid Dynamics · Physics 2023-09-25 Faisal Amlani , Heng Wei , Niema M. Pahlevan