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A quantum spin-liquid might be realized in $\alpha$-RuCl$_{3}$, a honeycomb-lattice magnetic material with substantial spin-orbit coupling. Moreover, $\alpha$-RuCl$_{3}$ is a Mott insulator, which implies the possibility that novel exotic…

The interplay between itinerant electrons and local magnetic moments in quantum materials brings about rich and fascinating phenomena and stimulates various developments in the theoretical framework. In this work, thermodynamic, electric…

In the effective Ising spin-1/2 antiferromagnetic chain system BaCo$_2$V$_2$O$_8, the magnetic-field influence is highly anisotropic. For magnetic fields along the easy axis $c$, the N\'{e}el order is strongly suppressed already for low…

Strongly Correlated Electrons · Physics 2015-06-15 S. K. Niesen , G. Kolland , M. Seher , O. Breunig , M. Valldor , M. Braden , B. Grenier , T. Lorenz

Recently, there have been contrary claims of Kitaev spin-liquid behaviour and ordered behavior in the honeycomb compound Ag$_3$LiIr$_2$O$_6$ based on various experimental signatures. Our investigations on this system reveal a…

We report a combined $^{115}$In NQR, $^{51}$V NMR and $\mu$SR spectroscopic study of the low-temperature magnetic properties of InCu$_{2/3}$V$_{1/3}$O$_3$, a quasi-two dimensional (2D) compound comprising in the spin sector a honeycomb…

Quantum fluctuations endow spin systems with surprisingly enriched magnetic phase diagrams. In frustrated magnets, strong quantum fluctuations boosted by either geometrical incompatibility or competitive exchange interactions stabilize…

The honeycomb magnet $\alpha$-RuCl$_{3}$ has been a leading candidate for realizing the Kitaev quantum spin liquid (QSL), but its intrinsic spin dynamics have remained obscured by crystal twinning. Here we apply biaxial anisotropic strain…

Topologically ordered states of matter are generically characterized by excitations with quantum number fractionalization. A prime example is the spin liquid realized in Kitaev's honeycomb-lattice compass model where spin-flip excitations…

Strongly Correlated Electrons · Physics 2018-11-12 C. Wellm , J. Zeisner , A. Alfonsov , A. U. B. Wolter , M. Roslova , A. Isaeva , T. Doert , M. Vojta , B. Büchner , V. Kataev

Here we report the observation of pressure-induced melting of antiferromagnetic (AFM) order and emergence of a new quantum state in the honeycomb-lattice halide alpha-RuCl3, a candidate compound in the proximity of quantum spin liquid…

We study the finite temperature phase diagram of the Heisenberg-Kitaev model on a three dimensional hyperhoneycomb lattice. Using semiclassical analysis and classical Monte-Carlo simulations, we investigate quantum and thermal…

Strongly Correlated Electrons · Physics 2015-06-17 SungBin Lee , Eric Kin-Ho Lee , Arun Paramekanti , Yong Baek Kim

The nature of the effective spin Hamiltonian and magnetic order in the honeycomb iridates is explored by considering a trigonal crystal field effect and spin-orbit coupling. Starting from a Hubbard model, an effective spin Hamiltonian is…

Strongly Correlated Electrons · Physics 2012-07-10 Subhro Bhattacharjee , Sung-Sik Lee , Yong Baek Kim

The magnetism of Kitaev materials has been widely studied, but their charge properties and the coupling to other degrees of freedom are less known. Here we investigate the charge states of $\alpha$-RuCl$_3$, a promising Kitaev quantum spin…

Strongly Correlated Electrons · Physics 2024-08-27 Xiaohu Zheng , Zhengxin Liu , Cuiwei Zhang , Huaxue Zhou , Chongli Yang , Youguo Shi , Katsumi Tanigaki , Rui-Rui Du

We have successfully synthesized the novel antiferromagnets with Ir$^{4+}$ honeycomb lattice ZnIrO$_3$ and MgIrO$_3$ and investigated their magnetic and thermodynamic properties. The two iridates are isomorphic but exhibit qualitatively…

Strongly Correlated Electrons · Physics 2018-08-09 Yuya Haraguchi , Chishiro Michioka , Hiroaki Ueda , Akira Matsuo , Koichi Kindo , Kazuyoshi Yoshimura

We consider layered decorated honeycomb lattices at two-thirds filling, as realized in some trinuclear organometallic complexes. Localized $S=1$ moments with a single-spin anisotropy emerge from the interplay of Coulomb repulsion and spin…

Strongly Correlated Electrons · Physics 2017-11-15 J. Merino , A. C. Jacko , A. L. Khosla , B. J. Powell

Recent numerical studies indicate that the antiferromagnetic Kitaev honeycomb lattice model undergoes a magnetic-field-induced quantum phase transition into a new spin-liquid phase. This intermediate-field phase has been previously…

Strongly Correlated Electrons · Physics 2022-03-02 Shang-Shun Zhang , Gábor B. Halász , Cristian D. Batista

The silver ruthenium oxide AgRuO$_3$ consists of honeycomb [Ru$_2^{5+}$O$_6^{2-}$] layers, and can be considered an analogue of SrRu$_2$O$_6$ with a different intercalation stage. We present measurements of magnetic susceptibility and…

We report on terahertz spectroscopy of quantum spin dynamics in $\alpha$-RuCl$_3$, a system proximate to the Kitaev honeycomb model, as a function of temperature and magnetic field. An extended magnetic continuum develops below the…

Strongly Correlated Electrons · Physics 2017-11-30 Zhe Wang , S. Reschke , D. Hüvonen , S. -H. Do , K. -Y. Choi , M. Gensch , U. Nage , T. Rõõm , A. Loidl

We derive and study a spin one-half Hamiltonian on a honeycomb lattice describing the exchange interactions between Ir$^{4+}$ ions in a family of layered iridates $A_2$IrO$_3$ ($A$=Li,Na). Depending on the microscopic parameters, the…

Strongly Correlated Electrons · Physics 2014-11-20 Jiri Chaloupka , George Jackeli , Giniyat Khaliullin

Under the hydrostatic pressure $P=1.48$ GPa, polarized neutron elastic scattering experiments have been carried out on the coupled spin dimer system TlCuCl$_3$ with the gapped ground state at ambient pressure. Pressure-induced magnetic…

Strongly Correlated Electrons · Physics 2009-11-10 A. Oosawa , K. Kakurai , T. Osakabe , M. Nakamura , M. Takeda , H. Tanaka

We present detailed calculations of the magnetic ground state properties of Cs$_2$CuCl$_4$ in an applied magnetic field, and compare our results with recent experiments. The material is described by a spin Hamiltonian, determined with…

Strongly Correlated Electrons · Physics 2007-05-23 M. Y. Veillette , J. T. Chalker , R. Coldea