Related papers: Interaction between vortex beams and diatomic mole…
Energy transfer between different mechanical degrees of freedom in atom-molecule collisions has been widely studied and largely understood. However, systems involving spins remain less explored, especially with a state-to-state precision.…
We propose a new model suitable for a nonequilibrium molecular dynamics (MD) simulation of electrical conductors. The model consists of classical electrons and atoms. The atoms compose a lattice vibration system. The electrons are scattered…
Recently Rydberg atom-ion bound states have been observed using a high resolution ion microscope (Nature 605, 453 (2022)) and the corresponding vibrational dynamics has been spectroscopically analyzed. The atom-ion bond is created by an…
Laboratory optics, typically dealing with monochromatic light beams in a single reference frame, exhibits numerous spin-orbit interaction phenomena due to the coupling between the spin and orbital degrees of freedom of light. Similar…
Vortex lines in superconductors in an external magnetic field slightly tilted from randomly-distributed parallel columnar defects can be modeled by a system of interacting bosons in a non-Hermitian vector potential and a random scalar…
We present a theoretical study of the inelastic scattering of vortex electrons by a hydrogen atom. In our study, special emphasis is placed on the effects of the Coulomb interaction between a projectile electron and a target atom. To…
We numerically investigate the transfer of optical information from a vector-vortex control beam to an unstructured probe beam, as mediated by an atomic vapour. The right and left circular components of these beams drive the atomic…
The rotational excitation of the three asymmetric-top molecular ion isotopologues H$_2$O$^+$, HDO$^+$, and D$_2$O$^+$ is studied theoretically using a combined framework of electron-molecule R-matrix scattering theory, multichannel…
We analyze the entanglement between electronic and nuclear motions in molecular wave functions, by using different widely used ansatzes in molecular Hamiltonian models (H$^+_2$ in 1D and the Shin-Metiu model); namely, i) Born-Oppenheimer…
Quantum vortices play an important role in the physics of two-dimensional quantum many-body systems, though they usually are understood in the single-particle framework like the mean-field approach. Inspired by the study on the relations…
A deformable body can rotate even with no angular momentum, simply by changing its shape. A good example is a falling cat, how it maneuvers in air to land on its feet. Here a first principles molecular level example of the phenomenon is…
We analyze theoretically the interplay between the torsional and the rotational motion of an aligned biphenyl-like molecule. To do so, we consider a transition between two electronic states with different internal torsional potentials,…
The transfer of orbital angular momentum from an optical vortex to an atomic Bose-Einstein condensate changes the vorticity of the condensate. The spatial mismatch between initial and final center-of-mass wavefunctions of the condensate…
As pioneering experiments have shown, strong vibrational coupling between molecular vibrations and light modes in an optical cavity can significantly alter molecular properties and even affect chemical reactivity. However, the current…
When circularly polarized light is scattered from a rotating target, a rotational Doppler shift (RDS) emerges from an exchange of angular momentum between the spinning object and the electromagnetic field. Here, we used coherently spinning…
Studies of quantum thermal effects on molecular excitation dynamics have often relied on oversimplified models, such as energy eigenstates or low-dimensional potentials, which fail to capture the complexity of real chemical systems. In…
This paper presents an analysis of a model problem, consisting of two interacting rigid rings, for the rotation of molecules in liquid $^4$He. Due to Bose symmetry, the excitation of the rotor corresponding to a ring of N helium atoms is…
Vortex $\gamma$ photons carrying orbital angular momenta (OAM) hold great potential for various applications. However, their generation remains a great challenge. Here, we successfully generate sub-MeV vortex $\gamma$ photons via…
We analyze in detail the possibility to use charge-dipole interaction between a single polar molecule or a 1D molecular array and a single Rydberg atom to read out rotational populations. The change in the Rydberg electron energy is…
Quantum vortices in superfluids may capture matter and deposit it inside their core. By doping vortices with foreign particles one can effectively visualize them and study experimentally. To acquire a better understanding of the interaction…