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We study theoretically the excitonic nonlinearity in hybrid organic-inorganic Ruddlesden-Popper perovskite thin films. The composite layered structure of these materials allows for flexible modulation of their excitonic response between the…

Mesoscale and Nanoscale Physics · Physics 2022-11-14 D. A. Baghdasaryan , E. S. Hakobyan , D. B. Hayrapetyan , I. V. Iorsh , I. A. Shelykh , V. Shahnazaryan

Exciton-polaritons - coherently hybridized states of excitons and photons - are instrumental for solid-state nonlinear optics and quantum simulations. To enable engineered polariton energy landscapes and interactions, local control over the…

Excitons, Coulomb bound electron-hole pairs, are composite bosons and their interactions in traditional semiconductors lead to condensation and light amplification. The much stronger Coulomb interaction in transition metal dichalcogenides…

Mesoscale and Nanoscale Physics · Physics 2017-04-05 M. Manca , M. M. Glazov , C. Robert , F. Cadiz , T. Taniguchi , K. Watanabe , E. Courtade , T. Amand , P. Renucci , X. Marie , G. Wang , B. Urbaszek

In recent years, the investigation of low-dimensional ferroelectrics has attracted great attention for their promising applications in nano devices. Piezoelectricity is one of the most core properties of ferroelectric materials, which plays…

Materials Science · Physics 2024-12-06 Ning Ding , Shuai Dong

Excitonic insulators (EIs), arising in semiconductors when the electron-hole binding energy exceeds the band gap, are a solid-state prototype for bosonic phases of matter. Unlike the charged excitations that are frozen and unable to…

Mesoscale and Nanoscale Physics · Physics 2023-09-27 Phuong X. Nguyen , Liguo Ma , Raghav Chaturvedi , Kenji Watanabe , Takashi Taniguchi , Jie Shan , Kin Fai Mak

Two-dimensional transition metal dichalcogenides (TMDs) provide an attractive platform for studying strain dependent exciton transport at room temperature due to large exciton binding energy and strong bandgap sensitivity to mechanical…

Mesoscale and Nanoscale Physics · Physics 2022-03-23 Kanak Datta , Zhengyang Lyu , Zidong Li , Takashi Taniguchi , Kenji Watanabe , Parag B. Deotare

We determine the zero temeperature phase diagram of excitons in the symmetric transition-metal dichalcogenide tri-layer heterosctructure WSe2/MoSe2/WSe2. First principle calculations reveal two distinct types of interlayer excitonic states,…

Extended efforts have been devoted to the study of strongly-interacting excitons and their dynamics, towards macroscopic quantum states of matter such as Bose-Einstein condensates of excitons and polaritons. Momentum-direct layer-hybridized…

Heterostructures of layered transition metal dichalcogenides (TMDs) host long-lived, tunable excitons, making them intriguing candidates for material-based quantum information applications. Light absorption in these systems induces a…

Materials Science · Physics 2023-08-25 Tomer Amit , Sivan Refaely-Abramson

Due to their low surface mass density, two-dimensional materials with a strong piezoelectric response are interesting for nanoelectromechanical systems with high force sensitivity. Unlike graphene, the two sublattices in a monolayer of…

Mesoscale and Nanoscale Physics · Physics 2016-08-05 Matthias Droth , Guido Burkard , Vitor M. Pereira

By combining electron energy-loss spectroscopy and state-of-the-art computational methods, we were able to provide an extensive picture of the excitonic processes in $1T$-HfS$_2$. The results differ significantly from the properties of the…

Mesoscale and Nanoscale Physics · Physics 2018-10-17 Carsten Habenicht , Lorenzo Sponza , Roman Schuster , Martin Knupfer , Bernd Büchner

Charge neutrality and their expected itinerant nature makes excitons potential transmitters of information. However, exciton mobility remains inaccessible to traditional optical experiments that only create and detect excitons with…

The giant exciton binding energy and the richness of degrees of freedom make monolayer transition metal dichalcogenide an unprecedented playground for exploring exciton physics in 2D systems. Thanks to the well energetically separated…

Mesoscale and Nanoscale Physics · Physics 2023-07-26 Bairen Zhu , Ke Xiao , Siyuan Yang , Kenji Watanabe , Takashi Taniguchi , Xiaodong Cui

Diffusion currents are theoretically examined in two-dimensional Dirac materials, such as those of the transition metal dichalcogenides (TMD) family. The transversal effects are analogues of the valley Hall (VHE) and photogalvanic (PGE)…

Mesoscale and Nanoscale Physics · Physics 2023-03-01 A. V. Snegirev , V. M. Kovalev , M. V. Entin

When transition-metal dichalcogenide monolayers lack inversion symmetry, their low-energy single particle spectrum can described by tilted massive Dirac Hamiltonians. The so-called Janus materials fall into that category. Inversion symmetry…

Mesoscale and Nanoscale Physics · Physics 2022-09-15 M. F. C. Martins Quintela , A. T. Costa , N. M. R. Peres

Two-dimensional semiconducting transition metal dichalcogenides embedded in optical microcavities in the strong exciton-photon coupling regime may lead to promising applications in spin and valley addressable polaritonic logic gates and…

Monolayers of transition metal dichalcogenides (TMDs) have a remarkable excitonic landscape with deeply bound bright and dark exciton states. Their properties are strongly affected by lattice distortions that can be created in a controlled…

Dipolar bosonic gases are currently the focus of intensive research due to their interesting many-body physics in the quantum regime. Their experimental embodiments range from Rydberg atoms to GaAs double quantum wells and van der Waals…

Mesoscale and Nanoscale Physics · Physics 2024-06-25 Zhe Sun , Alberto Ciarrocchi , Fedele Tagarelli , Juan Francisco Gonzalez Marin , Kenji Watanabe , Takashi Taniguchi , Andras Kis

Controlling interlayer excitons in van der Waals heterostructures holds promise for exploring Bose-Einstein condensates and developing novel optoelectronic applications, such as excitonic integrated circuits. Despite intensive studies,…

Mesoscale and Nanoscale Physics · Physics 2024-04-09 Lifu Zhang , Ruihao Ni , Liuxin Gu , Ming Xie , Suji Park , Houk Jang , Takashi Taniguchi , Kenji Watanabe , You Zhou

In semiconductors, exciton or charge carrier diffusivity is typically described as an inherent material property. Here, we show that the transport of excitons (i.e., bound electron-hole pairs) in CsPbBr3 perovskite nanocrystals (NCs)…