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Electrochemical strains are a ubiquitous feature of solid state ionic devices ranging from ion batteries and fuel cells to electroresistive and memristive memories. Recently, we proposed a scanning probe microscopy (SPM) based approach,…

Materials Science · Physics 2015-06-03 A. N. Morozovska , E. A. Eliseev , S. V. Kalinin

We have explored the light induced dynamics in superfluid helium nanodroplets with wide-angle scattering in a pump-probe measurement scheme. The droplets are doped with xenon atoms to facilitate the ignition of a nanoplasma through…

Light-matter interactions are of fundamental scientific and technological interest. Ultrafast electron microscopy and diffraction with combined femtosecond-nanometer resolution elucidate the laser-induced dynamics in structurally…

Materials Science · Physics 2025-04-08 Till Domröse , Leonardo da Camara Silva , Claus Ropers

We report on the observation of subcycle interferences of electron wave packets released during the strong field ionization of H$_2$ with cycle-shaped two-color laser fields. With a reaction microscope, channel-resolved photoelectron…

Chemical Physics · Physics 2016-12-08 Xinhua Xie , Stefan Roither , Daniil Kartashov , Li Zhang , Andrius Baltuška , Markus Kitzler

This paper investigates subcycling of particle orbits in variational, geometric particle-in-cell methods addressing the Vlasov--Maxwell system in magnetized plasmas. The purpose of subcycling is to allow different time steps for different…

Computational Physics · Physics 2020-11-13 Eero Hirvijoki , Katharina Kormann , Filippo Zonta

We demonstrate how the technique of ultrafast resonant x-ray scattering can be applied to imaging dynamics of electronic wave packets in crystals. We study scattering patterns from crystals with electron dynamics in valence bands taking…

Optics · Physics 2018-12-11 Daria Popova-Gorelova , Robin Santra

Control over various fragmentation reactions of a series of polyatomic molecules (acetylene, ethylene, 1,3-butadiene) by the optical waveform of intense few-cycle laser pulses is demonstrated experimentally. We show both experimentally and…

When a high-contrast ultra-relativistic laser beam enters a micro-sized plasma waveguide, the pulse energy is coupled into waveguide modes, which remarkably modifies the interaction of electrons and electromagnetic wave. The electrons that…

Plasma Physics · Physics 2016-08-03 Longqing Yi , Alexander Pukhov , Baifei Shen

We demonstrate X-ray phase contrast microscopy performed at the European X-ray Free-Electron Laser sampled at 1.128 MHz rate. We have applied this method to image stochastic processes induced by an optical laser incident on water-filled…

The coupling of electronic and nuclear motion in polyatomic molecules is at the heart of attochemistry. The molecular properties, transient structures and reaction mechanism of these many-body quantum objects are defined on the level of…

Chemical Physics · Physics 2024-03-12 David Schwickert , Andreas Przystawik , Dian Diaman , Detlef Kip , Jon P. Marangos , Tim Laarmann

Manipulating at will the propagation dynamics of high power laser pulses is a long-standing dream whose accomplishment would lead to the control of a plethora of fascinating physical phenomena emerging from laser-matter interaction. The…

Optics · Physics 2015-11-18 P. Béjot , G. Karras , F. Billard , J. Doussot , E. Hertz , B. Lavorel , O. Faucher

We present a combined theoretical and experimental study of X-ray optical wave mixing. This class of nonlinear phenomena combines the strengths of spectroscopic techniques from the optical domain, with the high-resolution capabilities of…

Free-electron lasers (FELs) can now generate temporally short, high power x-ray pulses of unprecedented brightness, even though their longitudinal coherence is relatively poor. The longitudinal coherence can be potentially improved by…

Accelerator Physics · Physics 2013-05-30 Ryan R. Lindberg , Yuri V. Shvyd'ko

Here we propose to exploit the low energy bandwidth, small wavelength and penetration power of ultrashort pulses from XFELs for resonant Small Angle Scattering (SAXS) on plasma structures in laser excited plasmas. Small angle scattering…

Plasma Physics · Physics 2016-03-09 Thomas Kluge , M. Bussmann , H. -K. Chung , C. Gutt , L. G. Huang , M. Zacharias , U. Schramm , T. E. Cowan

Time-resolved ultrafast x-ray scattering is an emerging approach to probe the temporally evolving electronic charge distribution in real-space and in real-time. In this contribution, time-resolved ultrafast x-ray scattering from an…

Atomic Physics · Physics 2015-06-18 Gopal Dixit , Robin Santra

X-ray photoelectron diffraction is a powerful tool for determining the structure of clean and adsorbate-covered surfaces. Extending the technique into the ultrafast time domain will open the door to studies as diverse as the direct…

The interaction of high-energy electrons and X-ray photons with soft semiconductors such as halide perovskites is essential for the characterisation and understanding of these optoelectronic materials. Using nano-probe diffraction…

We develop a new general formulation to explore light-driven electron transport through a single-molecule device with multiple pathways. Three individual systems are proposed including (i) a two-terminal molecular junction based on…

Mesoscale and Nanoscale Physics · Physics 2014-01-20 Liang-Yan Hsu , Herschel Rabitz