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We theoretically investigate the laser wavelength dependence of asymmetric dissociation of H$_2^+$. It is found that the electron localization in molecular dissociation is significantly manipulated by varying the wavelength of the driving…

Atomic and Molecular Clusters · Physics 2015-06-03 Kunlong Liu , Weiyi Hong , Qingbin Zhang , Peixiang Lu

We propose a method to study the time evolution of correlated electrons driven by an harmonic perturbation. Combining Floquet formalism to include the time-dependent field and Cluster Perturbation Theory to solve the many-body problem in…

Strongly Correlated Electrons · Physics 2016-10-19 M. Puviani , F. Manghi

The development of intense high-energy radiation sources and the improvement of techniques for detecting charged fragments have made possible experiments on multiple ionization of a molecule with registration of the momentum and charge of…

Ultrafast dynamics are generally investigated using stroboscopic pump-probe measurements, which characterize the sample properties for a single, specific time delay. These measurements are then repeated for a series of discrete time delays…

Achieving precise and adjustable control over laser frequency is an essential requirement in numerous applications such as precision spectroscopy, quantum control, and sensing. In many such applications it is desired to stabilize a laser…

Applied Physics · Physics 2024-05-22 Heleni Krelman , Ori Nefesh , Kfir Levi , Douglas G. Bopp , Songbai Kang , John E. Kitching , Liron Stern

We present measurements of high-order harmonics and relativistic electrons emitted into the vacuum from a plasma mirror driven by temporally-shaped ultra-intense laser waveforms, produced by collinearly combining the main laser field with…

Two-dimensional materials with hexagonal symmetry such as graphene and transition metal dichalcogenides} are unique materials to study light-field-controlled electron dynamics inside of a solid. Around the $K$-point, the dispersion relation…

Optics · Physics 2020-02-14 Christian Heide , Tobias Boolakee , Takuya Higuchi , Peter Hommelhoff

Electrodynamical processes induced in complex systems like semiconductors by strong electromagnetic fields, have traditionally/conventionally been described using semi-classical approaches. Although these approaches, allowed the…

The intercalation of alkali ions into layered materials has played an essential role in battery technology since the development of the first lithium-ion electrodes. Coulomb repulsion between the intercalants leads to ordering of the…

The electronic excitation occurring on adsorbates at ultrafast time scales from optical lasers that initiate surface chemical reactions is still an open question. Here, we report the ultrafast temporal evolution of X-ray absorption…

Ongoing developments in ultrafast X-ray sources offer powerful new means of probing the com- plex non-adiabatically coupled structural and electronic dynamics of photoexcited molecules. These non-Born-Oppenheimer effects are governed by…

Chemical Physics · Physics 2018-07-04 Simon P. Neville , Majed Chergui , Albert Stolow , Michael S. Schuurman

We demonstrate a two-dimensional time-domain spectroscopy method to extract amplitude and phase modifications of excited atomic states caused by the interaction with ultrashort laser pulses. The technique is based on Fourier analysis of the…

Atomic Physics · Physics 2015-06-19 Alexander Blättermann , Christian Ott , Andreas Kaldun , Thomas Ding , Thomas Pfeifer

Recent advances in time-resolved angle-resolved photoemission spectroscopy have enabled access to ultrafast electron states and their spin dynamics in solids. Atomically thin transition metal dichalcogenides are paradigmatic two-dimensional…

Mesoscale and Nanoscale Physics · Physics 2025-02-13 Alejandro S. Gómez , Yuriko Baba , Francisco Domínguez-Adame , Rafael A. Molina

The spatiotemporal response of crystals in x-ray Bragg diffraction resulting from excitation by an ultra-short, laterally confined x-ray pulse is studied theoretically. The theory presents an extension of the analysis in symmetric…

Optics · Physics 2012-10-22 Yuri Shvyd'ko , Ryan Lindberg

The emission of high-order harmonics from solids \cite{ghimire11a,schubert14a,luu15a,golde08a} under intense laser-pulse irradiation is revolutionizing our understanding of strong-field solid-light interactions…

We investigate both theoretically and experimentally the rotational dynamics of micrometric droplets of dye-doped and pure liquid crystal induced by circularly and elliptically polarized laser light. The droplets are dispersed in water and…

Optics · Physics 2007-12-06 C. Manzo , D. Paparo , L. Marrucci , I. Janossy

Ultrafast manipulation of vibrational coherence is an emergent route to control the structure of solids. However, this strategy can only induce long-range correlations and cannot modify atomic structure locally, which is required in many…

A new version of the R-matrix Floquet theory for laser-assisted electron-atom scattering is presented. The theory is non-perturbative and applicable to a non-relativistic many-electron atom or ion in a homogeneous linearly polarized field.…

Atomic Physics · Physics 2009-11-07 Mariko Terao-Dunseath , Kevin Dunseath

The ultrafast dynamics of charge carriers in solids plays a pivotal role in emerging optoelectronics, photonics, energy harvesting, and quantum technology applications. However, the investigation and direct visualization of such…

Particle acceleration consequences from fluctuating electric fields superposed on an X-type magnetic field in collisionless solar plasma are studied. Such a system is chosen to mimic generic features of dynamic reconnection, or the…

Astrophysics · Physics 2009-11-13 P. Petkaki , A. L. MacKinnon