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The low energy excitations in Na2IrO3 have been investigated using resonant inelastic x-ray scattering (RIXS). A magnetic excitation branch can be resolved, whose dispersion reaches a maximum energy of about 35 meV at the \Gamma-point. The…

Strongly Correlated Electrons · Physics 2013-07-08 H. Gretarsson , J. P. Clancy , Yogesh Singh , P. Gegenwart , J. P. Hill , Jungho Kim , M. H. Upton , A. H. Said , D. Casa , T. Gog , Young-June Kim

Fe3-xGeTe2 is an itinerant ferromagnet composed of two-dimensional layers weakly connected by van der Waals bonding that shows a variety of intriguing phenomena. Inelastic neutron scattering measurements on bulk single crystals of…

Strongly Correlated Electrons · Physics 2019-03-27 S. Calder , A. I. Kolesnikov , A. F. May

To reveal the structure-property relationship in quasi-one-dimensional (1D) spin-chain system Ca$_3$ZnMnO$_6$, we present comprehensive results, combining basic physical characterizations such as muon spin relaxation/rotation ($\mu$SR),…

Using high-resolution resonant inelastic x-ray scattering (RIXS), we performed a momentum-resolved study of magnetic excitations in the model spin-1/2 2D antiferromagnetic insulator Sr_2CuCl_2O_2. We identify both a single-spin-wave feature…

We study two-magnon excitations in resonant inelastic x-ray scattering (RIXS) at the transition-metal $K$-edge. Instead of working with effective Heisenberg spin models, we work with a Hubbard-type model ($d$-$p$ model) for a typical…

Strongly Correlated Electrons · Physics 2017-10-18 Takuji Nomura

The pyrovanadate alpha-Cu2V2O7 belongs to the orthorhombic (Fdd2) class of crystals with noncentrosymmetric crystal structure. Recently, the compound has been identified to be a magnetic multiferroic with a substantial electric polarization…

Strongly Correlated Electrons · Physics 2016-11-23 A. Banerjee , J. Sannigrahi , S. Bhowal , I. Dasgupta , S. Majumdar , H. C. Walker , A. Bhattacharyya , D. T. Adroja

Using the three-orbital Hubbard model, we investigate the low-energy excitation spectra in the antiferromagnetic phase of Ca$_2$RuO$_4$. We calculate the dynamical susceptibilities in the low-energy region by the random phase approximation…

Strongly Correlated Electrons · Physics 2022-07-27 Shunsuke Yamamoto , Yukinori Ohta , Koudai Sugimoto

Metal-insulator transitions in pyrochlore iridates (A2Ir2O7) are believed to occur due to subtle interplay of spin-orbit coupling, geometric frustration, and electron interactions. In particular, the nature of magnetic ordering of iridium…

Strongly Correlated Electrons · Physics 2014-07-29 Eric Kin-Ho Lee , Subhro Bhattacharjee , Yong Baek Kim

$\gamma$-triclinic and $\alpha$-monoclinic polymorphs of CoV$_{2}$O$_{6}$ are two of the few known transition metal ion based materials that display stepped $1/3$ magnetization plateaus at low temperatures. Neutron diffraction [M. Markkula…

Strongly Correlated Electrons · Physics 2015-12-23 F. Wallington , A. M. Arevalo-Lopez , J. W. Taylor , J. R. Stewart , V. Garcia-Sakai , J. P. Attfield , C. Stock

Magnetic excitations and magnetic structure of EuRbFe$_4$As$_4$ were investigated by inelastic neutron scattering (INS), neutron diffraction, and random phase approximation (RPA) calculations. Below the superconducting transition…

A resonant inelastic x-ray scattering study of the electronic structure of the semiconductor cuprous oxide, $\rm Cu_2O$, is reported. When the incident x-ray energy is tuned to the Cu K-absorption edge, large enhancements of the spectral…

Materials Science · Physics 2012-06-18 Young-June Kim , J. P. Hill , H. Yamaguchi , T. Gog , D. Casa

We report on the observation of orbital excitations in YVO3 by means of resonant inelastic x-ray scattering (RIXS) at energies across the vanadium L3 and oxygen K absorption edges. Due to the excellent experimental resolution we are able to…

The magnetic excitation spectrum in the bilayer iridate Sr$_3$Ir$_2$O$_7$ has been investigated using high-resolution resonant inelastic x-ray scattering (RIXS) performed at the iridium L$_3$ edge and theoretical techniques. A study of the…

Among condensed matter systems, Mott insulators exhibit diverse properties that emerge from electronic correlations. In itinerant metals, correlations are usually weak, but can also be enhanced via geometrical confinement of electrons, that…

We performed inelastic neutron scattering experiments on Cu$_2$$^{114}$Cd$^{11}$B$_2$O$_6$ powder. The magnetic excitations at low temperatures are similar to those of the interacting spin-1/2 tetramers in the ordered state. The weak…

Strongly Correlated Electrons · Physics 2015-12-09 Masashi Hase , Kenji Nakajima , Seiko Ohira-Kawamura , Yukinobu Kawakita , Tatsuya Kikuchi , Masashige Matsumoto

Electronic spin and orbital (dd) excitation spectra of (Ca{x}La{1-x})(Ba{1.75-x}La{0.25+x})Cu{3}O{y} samples are measured by resonant inelastic x-ray scattering (RIXS). In this compound, Tc of samples with identical hole dopings is strongly…

Inelastic neutron scattering experiments have been conducted to investigate the semimetal system Yb$_3$Ir$_4$Ge$_{13}$. No clear crystal-field-split levels were observed up to an excitation energy of 60 meV, while a magnetic excitation…

Strongly Correlated Electrons · Physics 2019-01-28 Kazuaki Iwasa , C. -L. Huang , Binod K. Rai , E. Morosan , Seiko Ohira-Kawamura , Kenji Nakajima

Taking spinon excitations in the quantum antiferromagnet CaCu2O3 as an example, we demonstrate that femtosecond dynamics of magnetic excitations can be probed by direct resonant inelastic x-ray scattering (RIXS). To this end, we isolate the…

In the study of dynamic charge order correlations in the cuprates, most high energy-resolution resonant inelastic x-ray scattering (RIXS) measurements have focused on momenta along the high-symmetry directions of the copper oxide plane.…

Although chromium trihalides are widely regarded as a promising class of two-dimensional magnets for next-generation devices, an accurate description of their electronic structure and magnetic interactions has proven challenging to achieve.…

Mesoscale and Nanoscale Physics · Physics 2024-09-04 Ravi Yadav , Lei Xu , Michele Pizzochero , Jeroen van den Brink , Mikhail I. Katsnelson , Oleg V. Yazyev