English

Correlation driven near-flat band Stoner excitations in a Kagome magnet

Strongly Correlated Electrons 2022-11-29 v1

Abstract

Among condensed matter systems, Mott insulators exhibit diverse properties that emerge from electronic correlations. In itinerant metals, correlations are usually weak, but can also be enhanced via geometrical confinement of electrons, that manifest as `flat' dispersionless electronic bands. In the fast developing field of topological materials, which includes Dirac and Weyl semimetals, flat bands are one of the important components that can result in unusual magnetic and transport behaviour. To date, characterisation of flat bands and their magnetism is scarce, hindering the design of novel materials. Here, we investigate the ferromagnetic Kagom\'{e} semimetal Co3_3Sn2_2S2_2 using resonant inelastic X-ray scattering. Remarkably, nearly non-dispersive Stoner spin excitation peaks are observed, sharply contrasting with the featureless Stoner continuum expected in conventional ferromagnetic metals. Our band structure and dynamic spin susceptibility calculations, and thermal evolution of the excitations, confirm the nearly non-dispersive Stoner excitations as unique signatures of correlations and spin-polarized electronic flat bands in Co3_3Sn2_2S2_2. These observations serve as a cornerstone for further exploration of band-induced symmetry-breaking orders in topological materials.

Keywords

Cite

@article{arxiv.2211.15292,
  title  = {Correlation driven near-flat band Stoner excitations in a Kagome magnet},
  author = {Abhishek Nag and Yiran Peng and Jiemin Li and Stefano Agrestini and H. C. Robarts and Mirian Garcia-Fernandez and A. C. Walters and Qi Wang and Qiangwei Yin and Hechang Lei and Zhiping Yin and Ke-Jin Zhou},
  journal= {arXiv preprint arXiv:2211.15292},
  year   = {2022}
}

Comments

15 pages, 4 figures, and Supplementary Information