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The kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of great debate. We conducted 17-O single crystal NMR…

Strongly Correlated Electrons · Physics 2015-11-09 M. Fu , T. Imai , T. -H. Han , Y. S. Lee

The structural-magnetic models of 25 AFM kagome cuprates similar to herbertsmithite (ZnCu3(OH)6Cl2) - a perspective spin liquid - have been calculated and analyzed. Main correlations between the structure and magnetic properties of these…

Materials Science · Physics 2021-08-13 L. M. Volkova , D. V. Marinin

Quantum spin liquids represent exotic states of spin systems characterized by long-range entanglement and emergent fractionalized quasiparticles. It is generally believed that disorder is hostile to quantum spin liquids. In our study, we…

Strongly Correlated Electrons · Physics 2024-08-30 Aini Xu , Qinxin Shen , Bo Liu , Zhenyuan Zeng , Lankun Han , Liqin Yan , Jun Luo , Jie Yang , Rui Zhou , Shiliang Li

The quantum spin liquid (QSL) is a highly entangled magnetic state characterized by the absence of static magnetism in its ground state. Instead, the spins fluctuate in a highly correlated way down to the lowest temperatures. The QSL is…

The intrinsic magnetic susceptibility and local magnetization of the near-kagome quantum magnet vesignieite, Cu3BaV2O8(OH)2, are presented as measured using 51V NMR. The NMR line shift gives an accurate measurement of the intrinsic…

Strongly Correlated Electrons · Physics 2015-05-28 J. A. Quilliam , F. Bert , R. H. Colman , D. Boldrin , A. S. Wills , P. Mendels

The Kagome-lattice-based material, Volborthite, $\mathrm{Cu_3 V_2 O_7 (OH)_2 \cdot 2 H_2 O}$, has been considered as a promising platform for discovery of unusual quantum ground states due to the frustrated nature of spin interactions. Here…

Strongly Correlated Electrons · Physics 2017-07-19 Li Ern Chern , Kyusung Hwang , Tomonari Mizoguchi , Yejin Huh , Yong Baek Kim

The face-centered-cubic lattice is composed of edge-sharing tetrahedra, making it a leading candidate host for strongly frustrated magnetism, but relatively few face-centered frustrated materials have been investigated. In the hydroxide…

The ground state of the quantum kagome antiferromagnet Zn-brochantite, ZnCu$_3$(OH)$_6$SO$_4$, which is one of only a few known spin-liquid (SL) realizations in two or three dimensions, has been described as a gapless SL with a spinon Fermi…

Strongly Correlated Electrons · Physics 2017-10-03 M. Gomilšek , M. Klanjšek , R. Žitko , M. Pregelj , F. Bert , P. Mendels , Y. Li , Q. M. Zhang , A. Zorko

The kagome lattice sits at the crossroad of present research efforts in quantum spin liquids, chiral phases, emergent skyrmion excitations and anomalous Hall effects to name but a few. In light of this diversity, our goal in this paper is…

Strongly Correlated Electrons · Physics 2016-02-17 K. Essafi , Owen Benton , Ludovic D. C. Jaubert

Neutron spectroscopy and diffuse neutron scattering on herbertsmithite [ZnCu3 (OH)6Cl2], a near-ideal realisation of the s = 1/2 kagome antiferromagnet, reveal the hallmark property of a quantum spin liquid; instantaneous short-ranged…

Strongly Correlated Electrons · Physics 2009-12-21 M. A. de Vries , J. R. Stewart , P. P. Deen , J. O. Piatek , G. J. Nilsen , H. M. Ronnow , A. Harrison

Quantum spin liquids form a novel class of matter where, despite the existence of strong exchange interactions, spins do not order down to the lowest measured temperature. Typically, these occur in lattices that act to frustrate the…

Strongly Correlated Electrons · Physics 2016-12-05 M. R. Norman

The topological quantum spin liquids (SL) and the nature of quantum phase transitions between them have attracted intensive attentions for the past twenty years. The extended kagome spin-1/2 antiferromagnet emerges as the primary candidate…

Strongly Correlated Electrons · Physics 2015-08-05 W. Zhu , S. S. Gong , D. N. Sheng

We investigate the microscopic properties of the kagome compound Cs$_2$Cu$_3$SnF$_{12}$ using $^{63,65}$Cu nuclear quadrupolar resonance (NQR). Analysis of the local hyperfine fields below the N\'eel temperature $T_N = 20$ K indicates a…

Strongly Correlated Electrons · Physics 2026-03-25 M. S. Grbić , I. Jakovac , I. Kupčić , H. Tanaka , M. Horvatić

Quantum spin liquids are highly entangled magnetic states with exotic properties. The $S = 1/2$ square-lattice Heisenberg model is one of the foundational models in frustrated magnetism with a predicted, but never observed, quantum spin…

Quantum spin liquids~(QSLs) represent a unique quantum disordered state of matter that hosts long-range quantum entanglement and fractional excitations. However, structural disorder resulting from site mixing between different types of ions…

Quantum spin liquid (QSL) with spinon Fermi surface is an exotic insulator that hosts neutral Fermi surfaces inside the gap. In an external magnetic field, it has been pointed out that the neutral Fermi surfaces are Landau quantized to form…

Strongly Correlated Electrons · Physics 2023-06-05 Wen-Yu He , Patrick. A. Lee

Y-kapellasite (Y$_3$Cu$_9$(OH)$_{19}$Cl$_8$), which hosts an original anisotropic kagome sublattice, is a promising candidate for studying elusive and complex correlated physics. It exhibits a theoretically predicted in-plane $(1/3, 1/3)$…

The two-dimensional (2D) spin-1/2 kagome Heisenberg antiferromagnet is believed to host quantum spin liquid (QSL) states with no magnetic order, but its ground state remains largely elusive. An important outstanding question concerns the…

Strongly Correlated Electrons · Physics 2024-05-30 S. Suetsugu , T. Asaba , Y. Kasahara , Y. Kohsaka , K. Totsuka , B. Li , Y. Zhao , Y. Li , M. Tokunaga , Y. Matsuda

Quantum spin liquids attract great interest due to their exceptional magnetic properties characterized by the absence of long-range order down to low temperatures despite the strong magnetic interaction. Commonly, these compounds are…

Strongly Correlated Electrons · Physics 2018-05-01 Martin Dressel , Andrej Pustogow

Exotic quantum spin liquid (QSL) is formed with such hypothetic particles as fermionic spinons carrying spin 1/2 and no charge. Here we calculate its thermodynamic and relaxation properties. Our calculations unveil the fundamental…

Strongly Correlated Electrons · Physics 2012-03-02 V. R. Shaginyan , A. Z. Msezane , K. G. Popov , G. S. Japaridze , V. A. Stephanovich