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Related papers: The Breakdown of Mott Physics at VO$_2$ Surfaces

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We use apertureless scattering near-field optical microscopy (SNOM) to investigate the nanoscale optical response of vanadium dioxide (VO2) thin films through a temperature-induced insulator-to-metal transition (IMT). We compare images of…

Mesoscale and Nanoscale Physics · Physics 2018-10-24 H. T. Stinson , A. Sternbach , O. Najera , R. Jing , A. S. Mcleod , T. V. Slusar , A. Mueller , L. Anderegg , H. T. Kim , M. Rozenberg , D. N. Basov

The metal-insulator transition (MIT) in vanadium dioxide (VO2) has the potential to lead to a number of disruptive technologies, including ultra-fast data storage, optical switches, and transistors which move beyond the limitations of…

Strongly Correlated Electrons · Physics 2018-02-28 T. J. Huffman , D. J. Lahneman , S. L. Wang , T. Slusar , Bong-Jun Kim , Hyun-Tak Kim , M. M. Qazilbash

We investigated the magnetic and electric properties of nanometer-sized vanadium dioxide (VO$_2$) particles. VO$_2$ nanoparticles were formed by milling VO$_2$ powder. We measured the magnetic field dependence of the magnetization of the…

Materials Science · Physics 2024-04-05 Tsuyoshi Hatano , Akihiro Fukawa , Hiroki Yamamoto , Keiichirou Akiba , Kouichi Takase

Vanadium dioxide is a correlated electron system that features a metal-insulator phase transition (MIT) above room temperature and is of interest in high speed switching devices. Here, we integrate VO2 into two-terminal coplanar waveguides…

Materials Science · Physics 2013-06-04 Sieu D. Ha , You Zhou , Christopher J. Fisher , Shriram Ramanathan , Jacob P. Treadway

We present results from an experimental study of the equilibrium and non-equilibrium transport properties of vanadium oxide nanobeams near the metal-insulator transition (MIT). Application of a large electric field in the insulating phase…

Strongly Correlated Electrons · Physics 2015-10-28 Adam A. Stabile , Sujay K. Singh , Tai-lung Wu , Luisa Whittaker , Sarbajit Banerjee , G. Sambandamurthy

Surface termination is known to play an important role in determining the physical properties of materials. It is crucial to know how surface termination affects the metal-insulator transition (MIT) of V$_2$O$_3$ films for both fundamental…

Strongly Correlated Electrons · Physics 2021-06-17 Asish K. Kundu , Sukanta Barman , Krishnakumar S. R. Menon

Vanadium dioxide with metal-to-insulator transition (MIT) that is triggered by heat, current or light is a promising material for modern active THz/mid-IR metasurfaces and all-optical big data processing systems. Multilayer VO2-based active…

The temperature dependence of the local structure of V_2O_3 in the vicinity of the metal to insulator transition (MIT) has been investigated using hard X-ray absorption spectroscopy. It is shown that the vanadium pair distance along the…

Strongly Correlated Electrons · Physics 2009-11-11 P. Pfalzer , G. Obermeier , M. Klemm , S. Horn , M. L. denBoer

We present a combined density-functional theory and dynamical mean-field theory (DFT+DMFT) study of the full structural phase space of rutile-based vanadium dioxide (VO$_2$), including also the less studied M2 and T phases, using an…

Strongly Correlated Electrons · Physics 2026-03-30 Peter Mlkvik , Nicola A. Spaldin , Claude Ederer

Nine of the known vanadium oxides, VO$_{2-1/n}$ (n - a positive or negative integer) with n=2 - 6, 8, 9, $\infty$ and -6, undergo metal-insulator transitions accompanied by structural transitions, at various temperatures T$_{MIT}$…

Strongly Correlated Electrons · Physics 2015-12-09 B. Fisher , J. Genossar , G. M. Reisner

New calculations for vanadium dioxide, one of the most controversely discussed materials for decades, reveal that band theory as based on density functional theory is well capable of correctly describing the electronic and magnetic…

Strongly Correlated Electrons · Physics 2011-07-07 V. Eyert

The single crystal VO2, exihibiting a first-order metal-insulator transition (MIT) at 67.2 degrees C and an insulator-insulator transition (IIT) at ~49.7 degrees C, is grown. From synchrotron-based x-ray microdiffraction analysis, the IIT…

Vanadium dioxide (VO2) has drawn significant attention for its near room temperature insulator to metal transition and associated structural phase transition. The underlying Physics behind the temperature induced insulator to metal and…

Materials Science · Physics 2023-04-19 S. R. Sahu , S. S. Majid , A. Ahad , A. Tripathy , K. Dey , S. Pal , B. K. De , Wen-Pin Hsieh , R. Rawat , V. G. Sathe , D. K. Shukla

The last few decades has seen the rapid growth of interest in the bulk perovskite-type transition metal oxides SrVO$_3$ and SrTiO$_3$. The electronic configuration of these perovskites differs by one electron associated to the transition…

Strongly Correlated Electrons · Physics 2023-09-04 A. D. N. James , M. Aichhorn , J. Laverock

Many strongly correlated transition metal oxides exhibit a metal-insulator transition (MIT), the manipulation of which is essential for their application as active device elements. However, such manipulation is hindered by lack of…

Strongly Correlated Electrons · Physics 2015-10-20 Tony Yamin , Yakov M. Strelniker , Amos Sharoni

We report a detail theoretical study of the electronic structure and phase stability of transition metal oxides MnO, FeO, CoO, and NiO in their paramagnetic cubic B1 structure by employing dynamical mean-field theory of correlated electrons…

Strongly Correlated Electrons · Physics 2016-10-26 I. Leonov , L. Pourovskii , A. Georges , I. A. Abrikosov

The metal-insulator transition (MIT) in vanadium dioxide VO$_2$ due to V-V dimerization has been extensively discussed for decades. While it is widely acknowledged that electron correlations, Peierls instabilities, and molecular orbital…

Strongly Correlated Electrons · Physics 2024-03-12 Shunsuke Kitou , Akitoshi Nakano , Masato Imaizumi , Yuiga Nakamura , Ichiro Terasaki , Taka-hisa Arima

We report the first application of critical cluster techniques to the Mott metal-insulator transition in vanadium dioxide. We show that the geometric properties of the metallic and insulating puddles observed by scanning near-field infrared…

Strongly Correlated Electrons · Physics 2016-01-27 Shuo Liu , B. Phillabaum , E. W. Carlson , K. A. Dahmen , N. S. Vidhyadhiraja , M. M. Qazilbash , D. N. Basov

The metal-insulator transition (MIT) in paramagnetic VO2 is studied within LDA+DMFT(IPT), which merges the local density approximation (LDA) with dynamical mean field theory (DMFT). With a fixed value of the Coulomb U=5.0eV, we show how the…

Strongly Correlated Electrons · Physics 2007-05-23 M. S. Laad , L. Craco , E. Müller-Hartmann

The temperature ($T$) dependent metal-insulator transition (MIT) in VO$_2$ is investigated using bulk sensitive hard x-ray ($\sim$ 8 keV) valence band, core level, and V 2$p-3d$ resonant photoemission spectroscopy (PES). The valence band…