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We study nonlinear response of a dimer composed of two identical Mie-resonant dielectric nanoparticles illuminated normally by a circularly polarized light. We develop a general theory describing hybridization of multipolar modes of the…

Topological invariants are crucial quantities for classifying materials with topological phases. Hence, their connections with experimentally measurable quantities are extremely important. In this context, circular dichroism (CD) provides a…

Mesoscale and Nanoscale Physics · Physics 2024-05-27 Ipsita Mandal

Molecular chirality detection and enantiomer discrimination are very important issues for many areas of science and technology, prompting intensive investigations via optical methods. However, these methods are hindered by the intrinsically…

Photoelectron circular dichroism (PECD) is a method where randomly oriented chiral molecules are photoionized due to irradiation by circularly-polarized lasers, yielding large chiral signals in the photoelectron momentum distribution.…

Optics · Physics 2025-12-16 Gal Bouskila , Avner Fleischer , Ofer Neufeld

Molecular chirality plays an important role in chemistry and biology, allows control of biological interactions, affects drugs efficacy and safety, and promotes synthesis of new materials. In general, chirality manifests itself in optical…

Optics · Physics 2026-04-10 Yuanyang Xie , Alexey V. Krasavin , Anatoly V. Zayats

We analyze circular dichroism (CD) in resonant inelastic x-ray scattering (RIXS) in magnetic materials. We define RIXS-CD as the difference between scattering amplitudes for the right- and left-circularly polarized incoming photons and…

Materials Science · Physics 2025-08-07 M. Furo , A. Hariki , J. Kuneš

Chirality is a fundamental asymmetry phenomenon, with chiral optical elements exhibiting asymmetric response in reflection or absorption of circularly polarized light. Recent realizations of such elements include nanoplasmonic systems with…

Molecular chirality, a form of stereochemistry most often describing relative spatial arrangements of bonded neighbors around tetrahedral carbon centers, influences the set of 3D conformers accessible to the molecule without changing its 2D…

Machine Learning · Computer Science 2021-10-12 Keir Adams , Lagnajit Pattanaik , Connor W. Coley

The orbital angular momentum (OAM) of electron states is an essential ingredient for topological and quantum geometric quantities in solids. For example, Dirac surface states with helical spin- and orbital-angular momenta are a hallmark of…

We propose a Babinet-invertible chiral metasurface for achieving dynamically reversible and strong circular dichroism (CD). The proposed metasurface is composed of VO$_2$-metal hybrid structure, and when VO$_2$ transits between the…

Optics · Physics 2021-04-07 Xiaoqing Luo , Fangrong Hu , Guangyuan Li

An efficient first principles approach to calculate X-ray magnetic circular dichroism (XMCD) and X-ray natural circular dichroism (XNCD) is developed and applied in the near edge region at the K-and L1-edges in solids. Computation of…

Metasurfaces, the two-dimensional analogues of metamaterials, are ideal platforms for sensing molecular chirality at the nanoscale, e.g. of inclusions of natural optically active molecules, as they offer large accessible areas (they are…

Applied Physics · Physics 2020-08-19 Sotiris Droulias

We calculate the circular dichroism (CD) for absorption of the twisted photons, or optical vortices, by atoms, caused by atomic excitation into discrete energy levels. The effects of photon spin on the rates and cross sections of atomic…

Quantum Physics · Physics 2017-10-02 Andrei Afanasev , Carl E. Carlson , Maria Solyanik

We develop photoelectron interferometry based on laser-assisted extreme ultraviolet ionization for flexible and robust control of photoelectron circular dichroism in randomly oriented chiral molecules. A comb of XUV photons ionizes a sample…

Circular dichroism (CD) spectroscopy is a useful technique for characterizing chiral molecules. It is more sensitive than total absorption to molecule conformation, and it is routinely used to identify enantiomers. We present here…

Chemical Physics · Physics 2023-11-21 Elena Molteni , Giuseppe Mattioli , Davide Sangalli

Chirality is a structural property of molecules lacking mirror symmetry that has strong implications in diverse fields, ranging from life to materials sciences. Established spectroscopic methods that are sensitive to chirality, such as…

Chiral lattice modes are hybrid states arising from chiral plasmonic particles assembled in ordered arrays with opportune periodicity. These resonances exhibit dependence on excitation handedness, and their observation in plasmonic lattices…

Photoelectron circular dichroism (PECD) is a fascinating phenomenon both from a fundamental science aspect but also due to its emerging role as a highly sensitive analytic tool for chiral recognition in the gas phase. PECD has been studied…

Chemical Physics · Physics 2021-05-21 Alexander Kastner , Tom Ring , Hendrike Braun , Arne Senftleben , Thomas Baumert

Chiral optical terahertz (THz) devices have significant technological implications for telecommunications, spectroscopy, and sensing. Engineering tunable, broadband, and cost-effective THz chiral materials has long been recognized as a…

Selective sensing of chiral molecules is a key aspect in fields spanning biology, chemistry, and pharmacology. However, conventional optical methods, such as circular dichroism (CD), encounter limitations owing to weak chiral light-matter…

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