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An all-optical method of ultrafast spin rotation is put forward to precisely manipulate the polarization of relativistic charged particle beams of leptons or ions. In particular, laser-driven dense ultrashort beams are manipulated via…

The inverse Faraday effect induced in magnetic films by ultrashort laser pulses allows excitation and control of spins at GHz and sub-THz frequencies. Frequency of the excited magnetization precession is easily tunable by the external…

Light-induced rotation of absorbing microscopic particles by transfer of angular momentum from light to the material raises the possibility of optically driven micromachines. The phenomenon has been observed using elliptically polarized…

We report entanglement of a single atom's hyperfine spin state with its motional state in a timescale of less than 3 ns. We engineer a short train of intense laser pulses to impart a spin-dependent momentum transfer of +/- 2 hbar k. Using…

Quantum Physics · Physics 2013-07-04 J. Mizrahi , C. Senko , B. Neyenhuis , K. G. Johnson , W. C. Campbell , C. W. S. Conover , C. Monroe

Dynamical properties of the square-lattice Heisenberg antiferromagnet in applied magnetic field are studied for arbitrary value S of the spin. Above the threshold field for two-particle decays, the standard spin-wave theory yields singular…

Strongly Correlated Electrons · Physics 2010-10-04 M. Mourigal , M. E. Zhitomirsky , A. L. Chernyshev

X-ray magnetic circular dichroism spectroscopy using an X-ray free electron laser is demonstrated with spectra over the Fe L$_{3,2}$-edges. This new ultrafast time-resolved capability is then applied to a fluence-dependent study of…

Strong magnetic field pulses associated with a relativistic electron bunch can imprint switching patterns in magnetic thin films that have uniaxial in-plane anisotropy. In experiments with Fe and FeCo alloy films the pattern shape reveals…

Mesoscale and Nanoscale Physics · Physics 2017-02-24 Ioan Tudosa

Understanding the coherent interplay of light with the magnetization in metals has been a long-standing problem in ultrafast magnetism. While it is known that when laser light acts on a metal it can induce magnetization via the process…

Mesoscale and Nanoscale Physics · Physics 2025-07-08 Theodoros Adamantopoulos , Dongwook Go , Peter M. Oppeneer , Yuriy Mokrousov

We present a theory for the coherent magnetization dynamics induced by a focused ultrafast laser beam in magnetic films, taking into account nonthermal (inverse Faraday effect) and thermal (heating) actuation. The dynamic conversion between…

Mesoscale and Nanoscale Physics · Physics 2015-11-06 Ka Shen , Gerrit E. W. Bauer

Starting from the continuity equation for the magnetization in time-dependent spin-density functional theory, we derive an expression for the effective time-dependent magnetic fields driving the out-of-equilibrium spin dynamics in magnetic…

Mesoscale and Nanoscale Physics · Physics 2017-01-18 Jacopo Simoni , Maria Stamenova , Stefano Sanvito

The demagnetizing factor N is of both conceptual interest and practical importance. Considering localized magnetic moments on a lattice, we show that for non-ellipsoidal samples, N depends on the spin dimensionality (Ising, XY, or…

We use transient absorption spectroscopy with circularly polarized x-rays to detect laser-excited hole states below the Fermi level and compare their dynamics with that of unoccupied states above the Fermi level in ferromagnetic [Co/Pd]…

In this letter, we provide a microscopic model for the ultrafast remagnetization of atomic moments already quenched above Stoner-Curie temperature by a strong laser fluence. Combining first principles density functional theory, atomistic…

Materials Science · Physics 2015-06-11 Raghuveer Chimata , Anders Bergman , Lars Bergqvist , Biplab Sanyal , Olle Eriksson

Laser-induced terahertz spin transport (TST) and ultrafast demagnetization (UDM) are central but so far disconnected phenomena in femtomagnetism and terahertz spintronics. Here, we use broadband terahertz emission spectroscopy to reliably…

Mesoscale and Nanoscale Physics · Physics 2021-05-27 R. Rouzegar , L. Brandt , L. Nadvornik , D. A. Reiss , A. L. Chekhov , O. Gueckstock , C. In , M. Wolf , T. S. Seifert , P. W. Brouwer , G. Woltersdorf , T. Kampfrath

It is now well established that a laser pulse can demagnetize a ferromagnet. However, for a long time, it has not had an analytic theory because it falls into neither nonlinear optics (NLO) nor magnetism. Here we attempt to fill this gap by…

Materials Science · Physics 2025-10-30 G. P. Zhang , Y. H. Bai , Thomas F. George

Here we carry out a first-principles time-dependent calculation to investigate how fast electrons actually move under laser excitation and how large the electron transport affects demagnetization on the shortest time scale. To take into…

Materials Science · Physics 2018-11-14 G. P. Zhang , Y. H. Bai , T. Jenkins , T. F. George

Converting angular momentum between different degrees of freedom within a magnetic material results from a dynamic interplay between electrons, magnons and phonons. This interplay is pivotal to implementing spintronic device concepts that…

Ultrafast magnetization dynamics induced by femtosecond laser pulses have been measured in ferrimagnetic Co0.8Gd0.2, Co.74Tb.26 and Co.86Tb.14 alloys. Using element sensitivity of X-ray magnetic circular dichroism at the Co L3, Tb M5 and Gd…

Materials Science · Physics 2015-06-12 V. Lopez-Flores , N. Bergeard , V. Halte , C Stamm , N. Pontius , M. Hehn , E. Otero , E. Beaurepaire , C. Boeglin

Laser-controlled entanglement between atomic qubits (`spins') and collective motion in trapped ion Coulomb crystals requires conditional momentum transfer from the laser. Since the spin-dependent force is derived from a spatial gradient in…

Atomic Physics · Physics 2021-12-06 Adam D West , Randall Putnam , Wesley C Campbell , Paul Hamilton

In spin-based electronics, information is encoded by the spin state of electron bunches. Processing this information requires the controlled transport of spin angular momentum through a solid, preferably at frequencies reaching the so far…

Mesoscale and Nanoscale Physics · Physics 2013-09-03 T. Kampfrath , M. Battiato , P. Maldonado , G. Eilers , J. Nötzold , I. Radu , F. Freimuth , Y. Mokrousov , S. Blügel , M. Wolf , P. M. Oppeneer , M. Münzenberg