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Exciting a ferromagnetic sample with an ultrashort laser pulse leads to a quenching of the magne- tization on a subpicosecond timescale. On the basis of the equilibration of intensive thermodynamic variables we establish a powerful model to…

Materials Science · Physics 2014-10-22 B. Y. Mueller , B. Rethfeld

The direct manipulation of spins via light may provide a path toward ultrafast energy-efficient devices. However, distinguishing the microscopic processes that can occur during ultrafast laser excitation in magnetic alloys is challenging.…

Ultrafast non-thermal manipulation of magnetization by light relies on either indirect coupling of the electric field component of the light with spins via spin-orbit interaction or direct coupling between the magnetic field component and…

Domain wall motion driven by ultra-short laser pulses is a prerequisite for envisaged low-power spintronics combining storage of information in magneto electronic devices with high speed and long distance transmission of information encoded…

Mesoscale and Nanoscale Physics · Physics 2017-06-28 T. Janda , P. E. Roy , R. M. Otxoa , Z. Soban , A. Ramsay , A. C. Irvine , F. Trojanek , R. P. Campion , B. L. Gallagher , P. Nemec , T. Jungwirth , J. Wunderlich

The control of antiferromagnetic order can pave the way to large storage capacity as well as fast manipulation of stored data. Here achieving a steady-state of sublattice magnetization after switching is crucial to prevent loss of stored…

Materials Science · Physics 2025-10-30 Asliddin Khudoyberdiev , Götz S. Uhrig

Strong laser-induced magnetization of oxygen gas at room temperature and atmospheric pressure is achieved experimentally on the sub-nanosecond time scale. The method is based on controlling the electronic spin of paramagnetic molecules by…

Quantum Physics · Physics 2017-06-21 A. A. Milner , A. Korobenko , V. Milner

Inspired by a recent pressure experiment in fcc Ni, we propose a simple method to use pressure to investigate the laser-induced femtosecond magnetism. Since the pressure effect on the electronic and magnetic properties can be well…

Materials Science · Physics 2015-12-15 M. S. Si , J. Y. Li , D. S. Xue , G. P. Zhang

In quasi-fission, it is unclear what the interaction between the relative orbital angular momentum and the spin of the fragments is from a microscopic perspective. In macroscopic approaches, it is expected that the large value of the…

Nuclear Theory · Physics 2024-11-19 Guillaume Scamps

The spin dynamics in Ni is studied by an exact diagonalization method on the ultrafast time scale. It is shown that the femtosecond relaxation of the magneto-optical response results from exchange interaction and spin-orbit coupling. Each…

Materials Science · Physics 2009-10-30 W. Hubner , G. P. Zhang

We develop a theory of the magnetization dynamics triggered by ultrafast optical excitation of ferromagnetic semiconductors. We describe the effects of the strong carrier spin relaxation on the nonlinear optical response by using the…

Strongly Correlated Electrons · Physics 2008-08-04 J. Chovan , E. G. Kavousanaki , I. E. Perakis

Ultrashort optical pulses are a cornerstone for manipulating electronic and magnetic states in materials on a femtosecond timescale. Conventional models assume that optical excitation primarily modifies the occupation of the electron energy…

Materials Science · Physics 2025-05-12 Sergii Parchenko , Peter M. Oppeneer , Andreas Scherz

In this work, we present evidence for the existence of a magnonic current on the sub-picosecond time-scale in a ferrimagnetic bilayer and its effect on ultrafast spin dynamics. The ferrimagnet, GdFeCo, is a material known to undergo…

Materials Science · Physics 2020-06-16 Sergiu Ruta , Zuwei Fu , Thomas Ostler , Alexey Kimel , Roy Chantrell

Manipulating spin in antiferromagnetic (AFM) materials has great potential in AFM opto-spintronics. Laser pulses can induce a transient ferromagnetic (FM) state in AFM metallic systems, but have never been proven in two-dimensional (2D) AFM…

Materials Science · Physics 2022-03-11 Shuo Li , Junjie He , Thomas Frauenheim

Spintronics had a widespread impact over the past decades due to transferring information by spin rather than electric currents. Its further development requires miniaturization and reduction of characteristic timescales of spin dynamics…

We investigate the ultrafast magnetization dynamics of an interlayer-exchange-coupled Co/Mn/Co trilayer system after excitation with an ultrafast optical pump. We probe element- and time-resolved ferromagnetic order by X-ray magnetic…

We investigate the ultrafast magnetization dynamics of semiconducting antiferromagnetic CrSBr using real-time time-dependent density functional theory. In zero magnetic field, laser excitation modifies only the magnetization along the easy…

Materials Science · Physics 2026-03-16 Ali Kefayati , Yafei Ren

Ultrafast laser excitation of ferromagnetic metals gives rise to correlated, highly non-equilibrium dynamics of electrons, spins and lattice, which are, however, poorly described by the widely-used three-temperature model (3TM). Here, we…

Materials Science · Physics 2024-01-17 Markus Weißenhofer , Peter M. Oppeneer

The absorption of traveling photons resonant with electric dipole transitions of an atomic gas naturally leads to electric dipole spin wave excitations. For a number of applications, it would be highly desirable to shape and coherently…

Atomic Physics · Physics 2021-01-04 Yizun He , Lingjing Ji , Yuzhuo Wang , Liyang Qiu , Jian Zhao , Yudi Ma , Xing Huang , Saijun Wu , Darrick E. Chang

We study the ultrafast demagnetization dynamics of LnRh$_2$Si$_2$ (Ln $=$ Pr, Nd, Sm, Gd, Tb, Dy, Ho) antiferromagnets (AFM) after excitation by a laser pulse, using a combination of density functional theory and atomistic spin and…

The understanding of how spins move at pico- and femtosecond time scales is the goal of much of modern research in condensed matter physics, with implications for ultrafast and more energy-efficient data storage. However, the limited…