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The electronic structure of the ferromagnetic superconductor URhGe in the paramagnetic phase has been studied by angle-resolved photoelectron spectroscopy using soft x rays (hn=595-700 eV). Dispersive bands with large contributions from U…

Plutonium (Pu), in which the 5$f$ valence electrons always wander the boundary between localized and itinerant states, exhibits quite complex crystal structures and unprecedentedly anomalous properties with respect to temperature and…

Strongly Correlated Electrons · Physics 2020-03-26 Li Huang , Haiyan Lu

Hard x-ray photoemission and optical spectroscopies have been performed on YbS and Yb metal to determine the precise $f$-electron occupation. A comparison of the photoemission spectra with the energy loss functions in bulk and surface,…

UTe$_2$ is a recently discovered unconventional superconductor that has attracted much interest due to its many intriguing properties - a large residual density-of-states in the superconducting state, re-entrant superconductivity in high…

Ir-based materials have drawn much attention due to the observation of insulating phase believed to be driven by spin-orbit coupling while Ir 5$d$ states are expected to be weakly correlated due to their large orbital extensions. IrO$_2$, a…

The electronic structure of ThRu2Si2 was studied by angle-resolved photoelectron spectroscopy (ARPES) with incident photon energies of hn=655-745 eV. Detailed band structure and the three-dimensional shapes of Fermi surfaces were derived…

A dramatic temperature dependent enhancement of U 5f spectral weight at $E_F$ is observed in angle-resolved photoemission measurements of $URu_2Si_2$ at the center of an X-point hole-pocket. Comparison of this temperature dependent behavior…

Strongly Correlated Electrons · Physics 2009-11-07 J. D. Denlinger , G. -H. Gweon , J. W. Allen , J. L. Sarrao

To unravel the interplay between the strong electronic correlation and itinerant-localized dual nature in atypical f electron systems, we employed the density functional theory in combination with the single-site dynamical mean-field theory…

Strongly Correlated Electrons · Physics 2021-02-08 Haiyan Lu , Qin Liu

We have performed angle-resolved photoemission spectroscopy (ARPES) experiments on paramagnetic UFeGa5 using soft X-ray synchrotron radiation (hn=500eV) and derived the bulk- and U 5f-sensitive electronic structure of UFeGa5. Although the…

In mixed-valence or heavy-fermion systems, the hybridization between local $f$ orbitals and conduction band states can cause the suppression of long-range magnetic order, which competes with strong spin fluctuations. Ce- and Yb-based…

Combining old and new de Haas-van Alphen (dHvA) and magnetoresistance data, we arrive at a detailed picture of the Fermi surface of the heavy fermion superconductor UPt3. Our work was partially motivated by a new proposal that two 5f…

The microscopic nature of the hidden order state in URu2Si2 is dependent on the low-energy configurations of the uranium ions, and there is currently no consensus on whether it is predominantly 5f^2 or 5f^3. Here we show that measurement of…

Strongly Correlated Electrons · Physics 2013-05-30 Rebecca Flint , Premala Chandra , Piers Coleman

The recently discovered heavy-fermion superconductor, UTe2, is an excellent candidate for spin-triplet superconductors where electrons form spin-triplet Cooper pairs with spin S = 1 and odd parity. Unconventional superconductivity often…

Single crystals of the unconventional superconductor UTe$_2$ have been grown in various conditions which result in different superconducting transition temperature as well as normal state properties. Stoichiometry of the samples has been…

Superconductivity · Physics 2022-03-11 Y. Haga , P. Opletal , Y. Tokiwa , E. Yamamoto , Y. Tokunaga , S. Kambe , H. Sakai

Band structure calculations have been used to identify the different bands contributing to the polarisation-dependent photoemission spectra of the undoped model cuprate Sr$_2$CuO$_2$Cl$_2$ at the high-symmetry points of the CuO$_2$ plane…

The electronic structure and chemical bonding of Beta-Ta synthesized as a thin 001-oriented film (space group P421m) is investigated by 4f core level and valence band X-ray photoelectron spectroscopy and compared to alfa-Ta bulk. For the…

Materials Science · Physics 2018-11-27 Martin Magnuson , Grzegorz Greczynski , Fredrik Eriksson , Lars Hultman , Hans Högberg

The electronic and magnetic structures of A2CrN3 (A = Ce, U) ternary compounds calculated based on band magnetism within DFT exhibit different behaviors of the nf elements (n = 4, 5 resp.). Charge analysis allows to formally express the two…

Materials Science · Physics 2018-08-30 Samir F. Matar , Charbel N. Kfoury

The low temperature hidden order state of URu$_2$Si$_2$ has long been a subject of intense speculation, and is thought to represent an as yet undetermined many-body quantum state not realized by other known materials. Here, X-ray absorption…

Based on a localized crystal electric field model for the U^{4+} in the (5f)^2-configuration, we analyze the resonant x-ray scattering spectra around U M_{IV} and M_{V} edges in URu_{2}Si_{2}, taking full Coulomb and spin-orbit interactions…

Strongly Correlated Electrons · Physics 2009-11-10 Tatsuya Nagao , Jun-ichi Igarashi

The newly discovered UTe2 superconductor is regarded as a heavy fermion mixed-valence system with very peculiar properties within the normal and superconducting states. It shows no signs of magnetic order but strong anisotropy of a magnetic…

Superconductivity · Physics 2023-06-21 S. Khmelevskyi , L. V. Pourovskii , E. A. Tereshina-Chitrova