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Quantum spin liquid (QSL) is a novel state of matter which refuses the conventional spin freezing even at 0 K. Experimentally searching for the structurally perfect candidates is a big challenge in condensed matter physics. Here we report…

The metal-organic-framework (MOF) compound Cu$_3$(HOTP)$_2$, a.k.a. Cu$_3$(HHTP)$_2$, is a small-gap semiconductor containing a kagome lattice of antiferromagnetically coupled $S$=1/2 Cu$^\mathrm{II}$ spins with intra-layer nearest-neighbor…

Strongly Correlated Electrons · Physics 2024-11-28 F. L. Pratt , D. Lopez-Alcala , V. Garcia-Lopez , M. Clemente-Leon , J. J. Baldovi , E. Coronado

Ba3IrTi2O9 crystallizes in a hexagonal structure consisting of a layered triangular arrangement of Ir4+ (Jeff=1/2). Magnetic susceptibility and heat capacity data show no magnetic ordering down to 0.35K inspite of a strong magnetic coupling…

Strongly Correlated Electrons · Physics 2012-10-29 Tusharkanti Dey , A. V. Mahajan , P. Khuntia , M. Baenitz , B. Koteswararao , F. C. Chou

Quantum fluctuations originating phase competition or geometrical frustration of spins lead to novel states such as a quantum critical point and a quantum spin liquid where the strong quantum fluctuations suppress any ordered states even at…

Strongly Correlated Electrons · Physics 2019-11-28 Y. Saito , H. Nakamura , M. Sawada , T. Yamazaki , S. Fukuoka , N. Matsunaga , K. Nomura , M. Dressel , A. Kawamoto

We report results of magnetic susceptibility, specific heat, and muon spin relaxation ($\mu$SR) measurements on the polycrystalline Ba$_6$Nd$_2$Ti$_4$O$_{17}$, a disorder-free triangular-lattice antiferromagnet. The absence of long-range…

Strongly Correlated Electrons · Physics 2024-11-21 C. Y. Jiang , B. L. Chen , K. W. Chen , J. C. Jiao , Y. Wang , Q. Wu , N. Y. Zhang , M. Y. Zou , P. -C. Ho , O. O. Bernal , L. Shu

We introduce the rare-earth delafossite compound TlYbSe$_2$ -- extending the search for quantum spin liquids in frustrated triangular lattice magnets. While the DC magnetisation suggests magnetic exchange interactions in the order of…

Strongly Correlated Electrons · Physics 2025-09-16 Bishnu P. Belbase , Arjun Unnikrishnan , Shi Feng , Eun Sang Choi , Johannes Knolle , Arnab Banerjee

Quantum spin liquids (QSLs) are an exotic state of matter that is subject to extensive research. However, the relationship between the ubiquitous disorder and the QSL behaviors is still unclear. Here, by performing comparative experimental…

The three-dimensional frustrated spin lattice in MgCrGaO4, where Cr3+ ions occupy a pyrochlore-like network, exemplifies a quantum magnet with competing interactions, macroscopic degeneracy, and exotic low-energy excitations. Using…

Strongly Correlated Electrons · Physics 2026-03-17 U. Jena , S. Kundu , Suheon Lee , Q. Faure , F. Damay , S. Rols , Adam Berlie , S. Petit , Kwang-Yong Choi , P. Khuntia

Pursuing fractionalized particles that do not bear properties of conventional measurable objects, exemplified by bare particles in the vacuum such as electrons and elementary excitations such as magnons, is a challenge in physics. Here we…

Strongly Correlated Electrons · Physics 2021-08-17 Yusuke Nomura , Masatoshi Imada

The nature of the magnetic ground state of highly frustrated systems remained puzzling to this day. Here, we have performed multifrequency electron spin resonance (ESR) measurements on a putative quantum spin liquid compound…

Quantum spin liquids are highly entangled ground states of quantum systems with emergent gauge structure, fractionalized spinon excitations, and other unusual properties. While these features clearly distinguish quantum spin liquids from…

Strongly Correlated Electrons · Physics 2013-06-18 Lucile Savary , Leon Balents

We report measurements of the specific heat of the quantum spin liquid system SrCu2(BO3)2 in continuous magnetic fields H of up to 33 T. The specific heat vs temperature at zero field shows an anomaly at 8 K, marking the opening of a gap in…

Strongly Correlated Electrons · Physics 2009-11-10 G. A. Jorge , R. Stern , M. Jaime , N. Harrison , J. Bonca , S. El Shawish , C. D. Batista , H. A. Dabkowska , B. D. Gaulin

A quantum magnet, LiCuSbO4, with chains of edge-sharing S = 1/2 CuO6 octahedra is reported. While the Curie-Weiss constant is ferromagnetic, \theta = 30 K, no phase transition or spin freezing occurs down to 100 mK. Specific heat indicates…

Strongly Correlated Electrons · Physics 2012-05-04 S. E. Dutton , M. Kumar , M. Mourigal , Z. G. Soos , J. -J. Wen , C. L. Broholm , N. H. Andersen , Q. Huang , M. Zbiri , R. Toft-Petersen , R. J. Cava

Scaling behavior in magnetization has been reported in a wide range of quantum spin liquid (QSL) candidates and is often interpreted as evidence for scale-free spin liquid physics. Here we present a comprehensive scaling analysis of…

Strongly Correlated Electrons · Physics 2026-04-16 Shannon Gould , John Singleton , Rabindranath Bag , Sara Haravifard , Sheng Ran

Quantum spin liquid (QSL) represents a new class of condensed matter states characterized by the long-range many-body entanglement of topological orders. The most prominent feature of the elusive QSL state is the existence of fractionalized…

We present the results of muon-spin relaxation measurements on the triangular lattice Heisenberg antiferromagnet $\alpha$-KCrO$_{2}$. We observe sharp changes in behaviour at an ordering temperature of $T_{\mathrm{c}}=23$ K, with an…

Strongly Correlated Electrons · Physics 2014-06-12 F. Xiao , T. Lancaster , P. J. Baker , F. L. Pratt , S. J. Blundell , J. S. Möller , N. Z. Ali , M. Jansen

Quantum spin liquid (QSL) is an exotic quantum phase of matter whose ground state is quantum-mechanically entangled without any magnetic ordering. A central issue concerns emergent excitations that characterize QSLs, which are…

Strongly Correlated Electrons · Physics 2018-05-08 Y. Tokiwa , T. Yamashita , D. Terazawa , K. Kimura , Y. Kasahara , T. Onishi , Y. Kato , M. Halim , P. Gegenwart , T. Shibauchi , S. Nakatsuji , E. -G. Moon , Y. Matsuda

The spin-1/2 Heisenberg antiferromagnetic chain is ideal for realizing one of the simplest gapless quantum spin-liquids (QSLs), supporting a many-body ground state whose elementary excitations are fractional fermionic excitations called…

Strongly Correlated Electrons · Physics 2020-07-01 Thao T. Tran , Chris A. Pocs , Yubo Zhang , Michal J. Winiarski , Jianwei Sun , Minhyea Lee , Tyrel M. McQueen

We analyze measurements of $C_{\rm mag}/T$, specific heat $C_{\rm mag}$ divided by temperature $T$, of the recently observed ultra spin liquid. The measurements are carried out in magnetic fields on the triangular lattice compound $\rm…

Strongly Correlated Electrons · Physics 2021-09-21 V. R. Shaginyan , A. Z. Msezane , S. A. Artamonov , G. S. Japaridze , Y. S. Leevik

We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…

Strongly Correlated Electrons · Physics 2007-05-23 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Yoshida , Y. Takano , A. Suslov , Y. Qiu , J. -H. Chung , D. G. Nocera , Y. S. Lee