Related papers: Observation and laser spectroscopy of ytterbium mo…
In chemistry, biology and materials science, the ability to access interatomic interactions and their dynamical evolution has become possible with the advent of femtosecond lasers. In particular, the observation of vibrational wave packets…
We have investigated the electronic, vibrational, optical, thermal and piezoelectric properties of LiNbO$_3$, LiTaO$_3$ and Li$_2$NbTaO$_6$ using the first-principles calculation based on the density functional theory. It also shows…
We present the first experimental demonstration of radiation pressure force deflection and direct laser cooling for barium monohydride (BaH) molecules resulting from multiple photon scattering. Despite a small recoil velocity (2.7 mm/s) and…
The Stark shift of the ytterbium optical clock transition due to room temperature blackbody radiation is dominated by a static Stark effect, which was recently measured to high accuracy [J. A. Sherman et al., Phys. Rev. Lett. 108, 153002…
Single crystals of the methylammonium (MA) lead halides MAPbI3, MAPbBr3, and MAPbCl3 have been investigated using infrared spectroscopy with the aim of analyzing structural and dynamical aspects of processes that enable the ordering of the…
An inner-shell orbital clock transition $^1S_0 \leftrightarrow 4f^{13}5d6s^2 \: (J=2)$ in neutral ytterbium atoms has attracted much attention as a new optical frequency standard as well as a highly sensitive probe for several new physics…
We calculate the shift, due to interatomic interactions, of an optical transition in an atomic Fermi gas trapped in an optical lattice, as in recent experiments of Campbell {\it et al.}, Science {\bf 324}, 360 (2009). Using a pseudospin…
We report a high-resolution microscope system for imaging ultracold ytterbium atoms trapped in a two-dimensional optical lattice. By using the ultraviolet strong transition combined with a solid immersion lens and high-resolution optics,…
The level structure of negative-ions near the electron detachment limit dictates the low-energy scattering of an electron with the parent neutral atom. We demonstrate that a single ultracold atom bound inside a Rydberg orbit forming an…
Precision searches for time-reversal symmetry violating interactions in polar molecules are extremely sensitive probes of high energy physics beyond the Standard Model. To extend the reach of these probes into the PeV regime, long coherence…
We excite YbF molecules to low-lying vibrational levels of the $A^2\Pi_{1/2}$ state, and of the nearby perturber state sometimes called [18.6]0.5. By dispersing the fluorescence, we measure branching ratios for the radiative decay to…
We investigate cooperative phenomena and superradiance for vibrational transitions in polar molecule spectroscopy when a high optical-depth (OD) sample is studied. Such cooperativity comes from the build-up of inter-particle coherence…
Due to the necessity of making a series of random adjustments after mode-locking in most experiments for preparing soliton molecules, the repeatability of the preparations remains a challenge. Here, we introduce a novel…
We study optical cycling in the polar free radical calcium monohydroxide (CaOH) and establish an experimental path towards scattering $\sim$$10^4$ photons. We report rovibronic branching ratio measurements with precision at the…
We show that optical spectroscopy of Rydberg states can provide accurate {\em in situ} thermometry at room-temperature. Transitions from a metastable state to Rydberg states with principal quantum numbers of 25 to 30 have 200 times larger…
Large amounts of hyperpolarized 3He gas with high nuclear polarization rates are required for use in neutron spin filters or nuclear magnetic resonance imaging of human lung. Very high efficiency can be obtained by metastability exchange…
We demonstrate a technique for frequency measurements of UV transitions with sub-MHz precision. The frequency is measured using a ring-cavity resonator whose length is calibrated against a reference laser locked to the $D_2$ line of…
We report radiation pressure slowing of YbF molecules to low velocity. In YbF, laser slowing is hindered by leaks out of the optical cycle attributed to low-lying metastable electronic states arising from inner-shell excitation. We bring…
The lifetimes of the lower-lying vibrational states of ultralong-range strontium Rydberg molecules comprising one ground-state 5s2 1S0 atom and one Rydberg atom in the 5s38s 3S1 state are reported. The molecules are created in an ultracold…
We generate 555.8nm light with sub-MHz linewidth through the use of laser injection-locking of a semiconductor diode at 1111.6nm, followed by frequency doubling in a resonant cavity. The integrity of the injection lock is investigated by…