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As a candidate Kitaev material, Na$_2$Co$_2$TeO$_6$ exhibits intriguing magnetism on a honeycomb lattice that is believed to be $C_3$-symmetric. Here we report a neutron diffraction study of high quality single crystals under $a$-axis…

Strongly Correlated Electrons · Physics 2023-06-06 Weiliang Yao , Yang Zhao , Yiming Qiu , Christian Balz , J. Ross Stewart , Jeffrey W. Lynn , Yuan Li

BaCo$_2$(AsO$_4$)$_2$ (BCAO), a honeycomb cobaltate, is considered a promising candidate for materials displaying the Kitaev quantum spin liquid state. This assumption is based on the distinctive characteristics of Co$^{2+}$ ions (3$d^7$)…

Strongly Correlated Electrons · Physics 2024-08-02 Sangyun Lee , Shengzhi Zhang , S. M. Thomas , L. Pressley , C. A. Bridges , Eun Sang Choi , Vivien S. Zapf , Stephen M. Winter , Minseong Lee

Candidate materials for Kitaev spin liquid phase have been intensively studied recently because of their potential applications in fault-tolerant quantum computing. Although most of the studies on Kitaev spin liquid have been done in 4$d$…

Strongly Correlated Electrons · Physics 2022-12-02 Subhasis Samanta , Panyalak Detrattanawichai , Sutassana Na-Phattalung , Heung-Sik Kim

Strong spin-orbital-coupling magnetic systems with the honeycomb structure can provide bond-directional interactions which may result in Kitaev quantum spin liquids and exotic anyonic excitations. However, one of the key ingredients in real…

In the quest to find quantum spin liquids, layered cobalt oxides Na2Co2TeO6 and Na3Co2SbO6 have been proposed as promising candidates for approximating the Kitaev honeycomb model. Yet, their suitability has been thrown into question due to…

Strongly Correlated Electrons · Physics 2024-04-25 Ping Miao , Xianghong Jin , Weiliang Yao , Yue Chen , Akihiro Koda , Zhenhong Tan , Wu Xie , Wenhai Ji , Takashi Kamiyama , Yuan Li

We report on magnetization $M(H)$, dc/ac magnetic susceptibility $\chi(T)$, specific heat $C_{\mathrm{m}}(T)$ and muon spin relaxation ($\mu$SR) measurements of the Kitaev honeycomb iridate Cu$_2$IrO$_2$ with quenched disorder. In spite of…

In the quest for materials hosting Kitaev spin liquids, much of the efforts have been focused on the fourth- and fifth-row transition metal compounds, which are spin-orbit coupling assisted Mott insulators. Here, we study the structural and…

Strongly Correlated Electrons · Physics 2022-12-20 Shishir Kumar Pandey , Ji Feng

Very recently, a 3$d$ based honeycomb cobaltate Na$_2$Co$_2$TeO$_6$ has garnered tremendous attention due to the proposed proximity to the Kitaev spin-liquid state as its 4$d$/5$d$ counterparts. Here, we use Zn to substitute Co in a broad…

The Kitaev model, characterized by bond-dependent Ising spin interactions among spin-orbit entangled dipole moments in Mott insulators, offered a new approach to quantum spin liquids. Motivated by another type of bond-dependent interaction…

Strongly Correlated Electrons · Physics 2023-03-08 Ahmed Rayyan , Derek Churchill , Hae-Young Kee

Recently, honeycomb cobaltates with 3$d^7$ were proposed to display Kitaev physics despite weak spin-orbit coupling. However, other theoretical and experimental works found leading XXZ Heisenberg and negligible Kitaev interactions in…

Strongly Correlated Electrons · Physics 2023-03-01 Xiaoyu Liu , Hae-Young Kee

The detection of considerable spin frustration in honeycomb cobalt oxide compounds indicates the presence of sizable Kitaev interactions in these systems, enlarging the pool of Kitaev spin liquid candidates. Several key questions remain to…

Strongly Correlated Electrons · Physics 2026-04-07 Pritam Bhattacharyya , Abdul Basit , Thorben Petersen , Stephan Rachel , Satoshi Nishimoto , Liviu Hozoi

We report inelastic neutron scattering measurements on Na2IrO3, a candidate for the Kitaev spin model on the honeycomb lattice. We observe spin-wave excitations below 5 meV with a dispersion that can be accounted for by including…

The magnetic structures and spin dynamics of Na$_{2}$Co$_{2}$TeO$_{6}$ and Na$_{2}$Ni$_{2}$TeO$_{6}$ are investigated by means of elastic and inelastic neutron scattering measurements and the results are discussed in the context of a…

Strongly Correlated Electrons · Physics 2021-11-24 Anjana M. Samarakoon , Qiang Chen , Haidong Zhou , V. Ovidiu Garlea

Kitaev exchange, a new paradigm in quantum magnetism research, occurs for 90$^{\circ}$ metal-ligand-metal links, $t_{2g}^5$ transition ions, and sizable spin-orbit coupling. It is being studied in honeycomb compounds but also on triangular…

Strongly Correlated Electrons · Physics 2023-10-11 Pritam Bhattacharyya , Nikolay A. Bogdanov , Satoshi Nishimoto , Stephen D. Wilson , Liviu Hozoi

We delineate quantum magnetism in the strongly spin-orbit coupled, distorted honeycomb-lattice antiferromagnet BiYbGeO$_{5}$. Our magnetization and heat capacity measurements reveal that its low-temperature behavior is well described by an…

Despite exhibiting magnetic long-range order below $T_\mathrm{N} = 26.7\,\mathrm{K}$, the honeycomb cobaltate Na$_2$Co$_2$TeO$_6$ is predicted to enter a Kitaev spin liquid state when subjected to small external perturbations. While most of…

Strongly Correlated Electrons · Physics 2026-03-04 J. Arneth , R. Kalaivanan , R. Sankar , K. -Y. Choi , R. Klingeler

The Kitaev candidate material Na$_2$Co$_2$TeO$_6$ is proposed to be proximate to a quantum spin liquid state but a suitable spin model and the nature of its ground states are still under debate. Our high-frequency/high-field electron spin…

Strongly Correlated Electrons · Physics 2025-09-08 Luca Bischof , Jan Arneth , Raju Kalaivanan , Raman Sankar , Kwang-Yong Choi , Rüdiger Klingeler

Topological spin liquids in two spatial dimensions are stable phases in the presence of a small magnetic field, but may give way to field-induced phenomena at intermediate field strengths. Sandwiched between the low-field spin liquid…

Strongly Correlated Electrons · Physics 2021-02-17 Ciarán Hickey , Matthias Gohlke , Christoph Berke , Simon Trebst

The magnetic field response of the Mott-insulating honeycomb iridate Na$_{2}$IrO$_{3}$ is investigated using torque magnetometry measurements in magnetic fields up to 60 tesla. A peak-dip structure is observed in the torque response at…

We report a combined $^{115}$In NQR, $^{51}$V NMR and $\mu$SR spectroscopic study of the low-temperature magnetic properties of InCu$_{2/3}$V$_{1/3}$O$_3$, a quasi-two dimensional (2D) compound comprising in the spin sector a honeycomb…