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Hybrid quantum dot (QD) / transition metal dichalcogenide (TMD) heterostructures are attractive components of next generation optoelectronic devices, which take advantage of the spectral tunability of QDs and the charge and exciton…

Materials Science · Physics 2018-07-18 Aaron J. Goodman , Nabeel S. Dahod , William A. Tisdale

Ta$_{3}$N$_{5}$ is among the most intensively studied photoanode materials for solar-driven water oxidation, yet its performance often remains limited by short carrier lifetimes and defect mediated recombination. Although transient…

We investigate near-field energy transfer between chemically synthesized quantum dots (QDs) and two-dimensional semiconductors. We fabricate devices in which electrostatically gated semiconducting monolayer molybdenum disulfide (MoS2) is…

Hybrid systems, which take advantage of low material dimensionality, have great potential for designing nanoscale devices. Quantum dots (QDs) -- a 0D nanostructure -- can be combined with 2D monolayers to achieve success in photovoltaics…

Computational Physics · Physics 2022-11-23 Matthew Ciesler , Han Wang , Shengbai Zhang , Damien West

Charge transfer between photoexcited quantum dots and molecular acceptors is one of the key limiting processes in most applications of colloidal nanostructures, most prominently in photovoltaics. An atomistic detailed description of this…

Building up a solid-state material from quantum dots (QD), which are often referred to as artificial atoms, offers the potential to create new materials with unprecedented macroscopic properties. The investigation of the electronic…

Mesoscale and Nanoscale Physics · Physics 2024-12-13 Morteza Shokrani , Dorothea Scheunemann , Clemens Göhler , Martijn Kemerink

The studies of the nonlinear optical (NLO) properties of the transition metal dichalcogenides (TMDs) coupled with photoactive particles, plasmonic nanocavities, waveguides, and metamaterials remain in their infancy. This study investigates…

The coupling of light to electrical charge carriers in semiconductors is the foundation of many technological applications. Attosecond transient absorption spectroscopy measures simultaneously how excited electrons and the vacancies they…

Materials Science · Physics 2023-05-03 Z. Schumacher , S. A. Sato , S. Neb , A. Niedermayr , L. Gallmann , A. Rubio , U. Keller

In this study, we investigate the electronic structure, charge transport dynamics, and optical properties of a quantum dot light-emitting diode (QD-LED) featuring a double nanorod (NR) emission layer composed of CdSe-ZnS core-shell…

Mesoscale and Nanoscale Physics · Physics 2026-03-25 A. G. Melkonyan , G. A. Mantashian , D. B. Hayrapetyan

The attachment of semiconducting nanoparticles to carbon nanotubes is one of the most challenging subjects in nanotechnology. Successful high coverage attachment and control over the charge transfer mechanism and photo-current generation…

Materials Science · Physics 2015-07-20 Alina Chanaewa , Beatriz H. Juarez , Horst Weller , Christian Klinke

Recently, transition metal dichalcogenides (TMDCs) semiconductors have been utilized for investigating quantum phenomena because of their unique band structures and novel electronic properties. In a quantum dot (QD), electrons are confined…

Mesoscale and Nanoscale Physics · Physics 2020-03-04 Gang Luo , Zhuo-Zhi Zhang , Hai-Ou Li , Xiang-Xiang Song , Guang-Wei Deng , Gang Cao , Ming Xiao , Guo-Ping Guo

Understanding charge transport in semiconductor quantum dot (QD) assemblies is important for developing the next generation of solar cells and light-harvesting devices based on QD technology. One of the key factors that governs the…

Chemical Physics · Physics 2025-01-22 Bokang Hou , Matthew Coley-O'Rourke , Uri Banin , Michael Thoss , Eran Rabani

Understanding electron transfer in organic molecules is of great interest in quantum materials for light harvesting, energy conversion, and integration of molecules into solar cells. This, however, poses the challenge of designing specific…

Chemical Physics · Physics 2019-07-24 Duvalier Madrid-Úsuga , Cristian E. Susa , John H. Reina

We report an improved photosensitivity in few-layer tin disulfide (SnS2) field-effect transistors (FETs) following doping with CdSe/ZnS core/shell quantum dots (QDs). The hybrid QD-SnS2 FET devices achieve more than 500 percent increase in…

Mesoscale and Nanoscale Physics · Physics 2016-04-20 Yuan Huang , Huidong Zang , Jia-Shiang Chen , Eli A. Sutter , Peter W. Sutter , Chang-Yong Nam , Mircea Cotlet

We investigate equilibrium and non-equilibrium charge-transfer processes by performing high-resolution transport spectroscopy. Using electrostatically defined quantum dots for energy-selective emission and detection, we achieved…

We study the charge transfer dynamics between a silicon quantum dot and an individual phosphorous donor using the conduction through the quantum dot as a probe for the donor ionization state. We use a silicon n-MOSFET (metal oxide field…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 G. Mazzeo , E. Prati , M. Belli , G. Leti , S. Cocco , M. Fanciulli , F. Guagliardo , G. Ferrari

Many linked processes occur concurrently in strongly excited semiconductors, such as interband and intraband absorption, scattering of electrons and holes by the heated lattice, Pauli blocking, bandgap renormalization and the formation of…

Graphene quantum dots (GQD) are interesting materials due to the confined sizes which allow to exploit their optoelectronic properties, especially when they interface with organic molecules through physisorption. In particular, when…

Materials Science · Physics 2019-10-23 Silvio Osella , Stefan Knippenberg

Quantum energy teleportation (QET) is a proposed protocol related to the quantum vacuum. The edge channels in a quantum Hall system is well suited for the experimental verification of QET. For this purpose, we examine a charge density wave…

Mesoscale and Nanoscale Physics · Physics 2018-03-14 Masahiro Matsuura , Takaaki Mano , Takeshi Noda , Naokazu Shibata , Masahiro Hotta , Go Yusa

Electron transfer (ET) between primary electron donors and acceptors is modeled in the photosystem II reaction center (RC). Our model includes (i) two discrete energy levels associated with donor and acceptor, interacting through a…

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