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Related papers: Quantum confined Rydberg excitons in Cu$_2$O nanop…

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Hosting giant Rydberg excitons with principal quantum numbers up to n = 30, cuprous oxide (Cu2O) provides a rare solid-state setting for exploring Rydberg physics, as exemplified by the blockade effect. Here we access the strongly…

Rydberg excitons in the semiconductor Cu$_2$O have been observed in absorption experiments up to a principal quantum number of n = 28 at millikelvin temperatures [1]. Here, we extend the experimental parameter space by variing both…

Mesoscale and Nanoscale Physics · Physics 2025-11-03 Julian Heckötter , David Janas , Marc Aßmann , Manfred Bayer

Rydberg excitons are, with their ultrastrong mutual interactions, giant optical nonlinearities, and very high sensitivity to external fields, promising for applications in quantum sensing and nonlinear optics at the single-photon level. To…

Rydberg excitons in Cu2O can be an emergent platform for solid-state quantum information processing by utilizing the exaggerated properties of high-lying excited states within the material. To develop practical quantum systems,…

Mesoscale and Nanoscale Physics · Physics 2021-05-19 Dungeon Daniel Kang , Aaron Gross , HeeBong Yang , Yusuke Morita , Kyung Soo Choi , Kosuke Yoshioka , Na Young Kim

Highly excited atoms with an electron moved into a level with large principal quantum number are fascinating hydrogen-like objects. The giant extension of these Rydberg atoms leads to huge interaction effects. Monitoring these interactions…

Mesoscale and Nanoscale Physics · Physics 2014-11-13 Tomasz Kazimierczuk , Dietmar Fröhlich , Stefan Scheel , Heinrich Stolz , Manfred Bayer

Due to quantum confinement, excitons in finite-sized crystals behave rather differently than in bulk materials. We investigate the dependence of energies of Rydberg excitons on the strengths of parabolic as well as rectangular confinement…

Mesoscale and Nanoscale Physics · Physics 2024-06-07 Pavel A. Belov , Florian Morawetz , Sjard Ole Krüger , Niklas Scheuler , Patric Rommel , Jörg Main , Harald Giessen , Stefan Scheel

Rydberg excitons are the solid-state analog of Rydberg atoms and can, e.g., for cuprous oxide, easily reach a large size in the region of $\mu$m for principal quantum numbers up to $n=25$. The fabrication of quantum well-like structures in…

Mesoscale and Nanoscale Physics · Physics 2024-04-29 Niklas Scheuler , Patric Rommel , Jörg Main , Pavel A. Belov

Rydberg states of excitons can reach microns in size and require extremely pure crystals. We introduce an experimental method for the rapid and spatially-resolved characterization of Rydberg excitons in copper oxide (Cu2O) with sub-micron…

Quantum Gases · Physics 2024-02-06 Kerwan Morin , Delphine Lagarde , Angélique Gillet , Xavier Marie , Thomas Boulier

Rydberg excitons (analogues of Rydberg atoms in condensed matter systems) are highly excited bound electron-hole states with large Bohr radii. The interaction between them as well as exciton coupling to light may lead to strong optical…

High-lying Rydberg states of Mott-Wannier excitons are receiving considerable interest due to the possibility of adding long-range interactions to the physics of exciton-polaritons. Here, we study Rydberg excitation in bulk synthetic…

Coherent optical control of individual particles has been demonstrated both for atoms and semiconductor quantum dots. Here we demonstrate the emergence of quantum coherent effects in semiconductor Rydberg excitons in bulk Cu$_2$O. Due to…

Mesoscale and Nanoscale Physics · Physics 2016-09-28 P. Grünwald , M. Aßmann , J. Heckötter , D. Fröhlich , M. Bayer , H. Stolz , S. Scheel

We investigate the nonlinear refraction and the nonlinear Kerr phase shift which are due to Rydberg excitons induced in Cu2O crystal by short-time pulses. We observe the phenomenon of quantum beats, analogous to that observed in exciton…

Mesoscale and Nanoscale Physics · Physics 2025-11-06 Gerard Czajkowski

Cuprous oxide (Cu$_2$O) is a semiconductor with large exciton binding energy and significant technological importance in applications such as photovoltaics and solar water splitting. It is also a superior material system for quantum optics…

Cuprous oxide (Cu${}_2$O) has recently been proposed as a promising solid-state host for excitonic Rydberg states with large principal quantum numbers ($n$), whose exaggerated wavefunction sizes ($\propto n^2)$ facilitate gigantic…

Quantum Physics · Physics 2022-11-01 Jacob DeLange , Kinjol Barua , Val Zwiller , Stephan Steinhauer , Hadiseh Alaeian

We propose a scheme for calculation of optical functions of a semiconductor with Rydberg excitons, for a wide interval of dimensions. We start with 2-dimensional structure, then going to thin films and ending on 3-dimensional bulk crystals.…

Mesoscale and Nanoscale Physics · Physics 2020-05-13 David Ziemkiewicz , Karol Karpiński , Sylwia Zielińska-Raczyńska , Gerard Czajkowski

Rydberg atoms have attracted considerable interest due to their huge interaction among each other and with external fields. They demonstrate characteristic scaling laws in dependence on the principal quantum number $n$ for features such as…

Materials Science · Physics 2017-09-26 J. Heckötter , M. Freitag , D. Fröhlich , M. Aßmann , M. Bayer , M. A. Semina , M. M. Glazov

The enhanced Coulomb interaction in two-dimensional (2D) semiconductors leads to the tightly bound electron-hole pairs known as excitons. The large binding energy of excitons enables the formation of Rydberg excitons with high principal…

Mesoscale and Nanoscale Physics · Physics 2024-02-21 Zhen Lian , Yun-Mei Li , Li Yan , Lei Ma , Dongxue Chen , Takashi Taniguchi , Kenji Watanabe , Chuanwei Zhang , Su-Fei Shi

Solid-state platforms provide exceptional opportunities for advancing on-chip quantum technologies by enhancing interaction strengths through coupling, scalability, and robustness. Cuprous oxide ($\text{Cu}_{2}\text{O}$) has recently…

We investigate the nonlinear refraction induced by Rydberg excitons in $\mathrm{Cu_2O}$. Using a high-precision interferometry imaging technique that spatially resolves the nonlinear phase shift, we observe significant shifts at extremely…

We present a study of even parity Rydberg exciton states in cuprous oxide using time-resolved second harmonic generation (SHG). Excitonic states with principal quantum number n = 5 - 12 were excited by nanosecond pulses around 1143 nm.…

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