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We report the formation of alternating strings and clusters in a binary suspension of repulsive charged colloids with double layers larger than the particle size. Within a binary cell model we include many-body and charge-regulation effects…

Soft Condensed Matter · Physics 2016-08-16 Jeffrey C. Everts , Marjolein N. van der Linden , Alfons van Blaaderen , René van Roij

The behavior of mobile linkers connecting two semi-flexible charged polymers, such as polyvalent counterions connecting DNA or F-actin chains, is studied theoretically. The chain bending rigidity induces an effective repulsion between…

Soft Condensed Matter · Physics 2009-11-07 I. Borukhov , R. F. Bruinsma , W. M. Gelbart , A. J. Liu

At sufficiently low temperatures and high densities, repulsive spherical particles in two-dimensions (2d) form close-packed structures with six-fold symmetry. By contrast, when the interparticle interaction has an attractive anisotropic…

Soft Condensed Matter · Physics 2018-09-13 T. Geigenfeind , C. S. Dias , M. M. Telo da Gama , D. de las Heras , N. A. M. Araújo

The microphase separated morphology of a melt of a specific class of comb-coil diblock copolymers, consisting of an AB comb block and a linear homopolymer A block, is analyzed in the weak segregation limit. On increasing the length of the…

Soft Condensed Matter · Physics 2009-11-07 Rikkert J. Nap , Gerrit ten Brinke

Block copolymer (BCP) melt assembly has been the subject of decades of study, with focus largely on self-organized spatial patterns of periodically-ordered segment density. In this study, we demonstrate that underlying these otherwise…

Soft Condensed Matter · Physics 2017-06-21 Ishan Prasad , Youngmi Seo , Lisa M. Hall , Gregory M. Grason

Using video-microscopy imaging we demonstrate the existence of a short-ranged equilibrium attraction between heavy silica colloids diffusing on soft surfaces of cross-linked polymer gels. The inter-colloid potential can be tuned by changing…

Soft Condensed Matter · Physics 2013-05-29 Lorenzo Di Michele , Taiki Yanagishima , Anthony R. Brewer , Jurij Kotar , Seth Fraden , Erika Eiser

Using molecular dynamics simulation of a standard bead-spring model we investigate the density crossover scaling of strictly two-dimensional self-avoiding polymer chains focusing on properties related to the contact exponent set by the…

Soft Condensed Matter · Physics 2015-06-03 N. Schulmann , H. Meyer , J. P. Wittmer , A. Johner , J. Baschnagel

The mechanism of multivalent counterion-induced bundle formation by filamentous actin (F-actin) is studied using a coarse-grained model and molecular dynamics simulation. Real diameter size, helically ordered charge distribution and twist…

Soft Condensed Matter · Physics 2012-03-01 Sarah Mohammadinejad , Ramin Golestanian , Hossein Fazli

We carry out a computational study on the geometric and electronic properties of multi-layers of silicene in different stacking configurations using a state-of-art abinitio density functional theory based calculations. In this work we…

Materials Science · Physics 2015-02-26 C. Kamal , Aparna Chakrabarti , Arup Banerjee , S. K. Deb

We devise a method for designing materials that will have some desired structural characteristics. We apply it to multiblock copolymers that have two different types of monomers, A and B. We show how to determine what sequence of A's and…

Condensed Matter · Physics 2009-10-28 Tanya Kurosky , J. M. Deutsch

Active matter systems - such as a collection of active colloidal particles - operate far from equilibrium with complex inter-particle interactions that govern their collective dynamics. Predicting the collective dynamics of such systems may…

Soft Condensed Matter · Physics 2024-08-06 Arvin Gopal Subramaniam , Manoj Kumar , Shashi Thutupalli , Rajesh Singh

We demonstrate formation of hierarchical structures in two-dimensional systems with multiple length scales in the inter-particle interaction. These include states such as clusters of clusters, concentric rings, clusters inside a ring, and…

Superconductivity · Physics 2013-09-25 Christopher N. Varney , Karl A. H. Sellin , Qingze Wang , Hans Fangohr , Egor Babaev

At low temperatures, colloidal particles with short-range attractive and long-range repulsive interactions can form various periodic microphases in bulk.In this paper, we investigate the self-assembly behaviour of colloids with competing…

Soft Condensed Matter · Physics 2023-12-12 Ningyi Li , Junhong Li , Lijingting Qing , Shicheng Ma , Yao Li , Baohui Li

Strong, long-range interactions present a unique challenge for the theoretical investigation of quantum many-body lattice models, due to the generation of large numbers of competing states at low energy. Here, we investigate a class of…

We investigate the phenomenon of multilayer formation via layer-by-layer deposition of alternating charge polyelectrolytes. Using mean-field theory, we find that a strong short-range attraction between the two types of polymer chains is…

Soft Condensed Matter · Physics 2012-01-31 Adi Shafir , David Andelman

We explore the effect of an attractive interaction between parallel-aligned polymers, which are perpendicularly grafted on a substrate. Such an attractive interaction could be due to, e.g., reversible cross-links. The competition between…

Soft Condensed Matter · Physics 2013-10-08 Panayotis Benetatos , Eugene M. Terentjev , Annette Zippelius

We construct a one-bead-per-residue coarse-grained dynamical model to describe intrinsically disordered proteins at significantly longer timescales than in the all-atom models. In this model, inter-residue contacts form and disappear during…

Biomolecules · Quantitative Biology 2018-07-23 Łukasz Mioduszewski , Marek Cieplak

Dried droplets of polymer solutions of different molecular weights and concentrations leave various types of 'coffee-ring' patterns. These patterns are consequence of contact line motion. We have observed for very low molecular weight the…

Soft Condensed Matter · Physics 2014-03-20 Nupur Biswas , Alokmay Datta

Molecular dynamics simulations have been employed to study the formation of a physical (thermoreversible) gel by amphiphilic A-B-A triblock copolymers in aqueous solution. In order to mimic the structure of hydrogel-forming polypeptides…

Soft Condensed Matter · Physics 2007-05-23 Lei Guo , Erik Luijten

Using Brownian Dynamics (BD) simulations we investigate the non-equilibrium structure formation of a two-dimensional (2D) binary system of dipolar colloids propelling in opposite directions. Despite of a pronounced tendency for chain…

Soft Condensed Matter · Physics 2015-06-23 Florian Kogler , Sabine H. L. Klapp