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Large scale atomistic simulations with suitable interatomic potentials are widely employed by scientists or engineers of different areas. Quick generation of high-quality interatomic potentials is of urgent need under present circumstances,…

Materials Science · Physics 2016-11-23 Kun Wang , Wenjun Zhu , Shifang Xiao , Jun Chen , Wangyu Hu

This article reviews how nuclear fission is described within nuclear density functional theory. In spontaneous fission, half-lives are the main observables and quantum tunnelling the essential concept, while in induced fission the focus is…

Nuclear Theory · Physics 2018-02-21 N. Schunck , L. M. Robledo

Finite size scaling for the Schr\"{o}dinger equation is a systematic approach to calculate the quantum critical parameters for a given Hamiltonian. This approach has been shown to give very accurate results for critical parameters by using…

Quantum Physics · Physics 2012-03-16 Edwin Antillon , Birgit Wehefritz-Kaufmann , Sabre Kais

Understanding the mechanisms of induced nuclear fission for a broad range of neutron energies could help resolve fundamental science issues, such as the formation of elements in the universe, but could have also a large impact on societal…

Nuclear Theory · Physics 2015-03-26 N. Schunck , D. Duke , H. Carr

Current work discusses methods for estimating the moments of inertia of fission fragments for spontaneous fission of the isotope Cf-252, in particular, two main approaches are mentioned: statistical and microscopic. In addition, the methods…

Nuclear Theory · Physics 2024-08-27 D. E. Lyubashevsky , P. V. Kostryukov , A. A. Pisklyukov , J. D. Shcherbina

In numerous astrophysical scenarios, such as core-collapse supernovae and neutron star mergers, as in well as heavy-ion collision experiments, transitions between thermally populated nuclear excited states have been shown to play an…

Nuclear Theory · Physics 2022-09-22 E. M. Ney , A. Ravlić , J. Engel , N. Paar

We show that the total kinetic energy (TKE) of nuclei after the spontaneous fission of $^{258}$Fm can be well reproduced using simple assumptions on the quantum collective phase-space explored by the nucleus after passing the fission…

Nuclear Theory · Physics 2017-04-19 Yusuke Tanimura , Denis Lacroix , Sakir Ayik

We present a real-space formulation and higher-order finite-difference implementation of periodic Orbital-free Density Functional Theory (OF-DFT). Specifically, utilizing a local reformulation of the electrostatic and kernel terms, we…

Computational Physics · Physics 2015-12-23 Swarnava Ghosh , Phanish Suryanarayana

Spontaneous fission half-lives of actinide and super-heavy nuclei are calculated, using the least-action integral, through the WKB tunneling probability of the barrier that appears in the deformation landscape obtained in the…

Nuclear Theory · Physics 2023-10-18 J. Marin Blanco , A. Dobrowolski , A. Zdeb , J. Bartel

The augmented Lagrangiam method (ALM), widely used in quantum chemistry constrained optimization problems, is applied in the context of the nuclear Density Functional Theory (DFT) in the self-consistent constrained Skyrme…

Nuclear Theory · Physics 2014-11-21 A. Staszczak , M. Stoitsov , A. Baran , W. Nazarewicz

We develop a new framework of the deformed quasiparticle-random-phase approximation (QRPA) where the Skyrme density functional and the density-dependent pairing functional are consistently treated. Numerical applications are carried out for…

Nuclear Theory · Physics 2009-11-23 Kenichi Yoshida , Nguyen Van Giai

Random Phase Approximation (RPA) is the basic method for calculation of excited states of nuclei over the Hartree-Fock ground state, suitable also for energy density functionals (EDF or DFT). We developed a convenient formalism for…

Nuclear Theory · Physics 2025-06-19 Anton Repko , Jan Kvasil , V. O. Nesterenko , P. -G. Reinhard

The response of a nucleus to an electromagnetic probe is a key quantity to simulate photabsorption or photodeexcitation processes. For large calculations at the scale of the entire mass table, this response can be estimated by linear…

Nuclear Theory · Physics 2024-04-05 Tong Li , Nicolas Schunck

Hybrid quantum mechanical-molecular mechanical (QM/MM) simulations are widely used in enzyme simulation. Over ten convergence studies of QM/MM methods have revealed over the past several years that key energetic and structural properties…

Chemical Physics · Physics 2017-01-11 Maria Karelina , Heather J. Kulik

We present a large scale survey of life-times for spontaneous fission in the regime of super-heavy elements (SHE), i.e. nuclei with Z=104-122. This is done on the basis of the Skyrme-Hartree-Fock model. The axially symmetric fission path is…

Nuclear Theory · Physics 2010-02-02 N. Schindzielorz , J. Erler , P. Klüpfel , P. -G. Reinhard , G. Hager

Background: The complete event fission simulation code FREYA is used to study correlations in fission. To make the best possible simulations, FREYA one must find the optimized values of the five physics-based parameters which characterize…

Nuclear Theory · Physics 2019-01-10 Jackson Van Dyke , Lee Bernstein , Ramona Vogt

A microscopic model aimed at the description of charge-exchange nuclear excitations along isotopic chains which include open-shell systems, is developed. It consists of quasiparticle random phase approximation (QRPA) made on top of…

Nuclear Theory · Physics 2009-02-18 S. Fracasso , G. Colo`

Background: Nuclear fission is a complex large-amplitude collective decay mode in heavy nuclei. Microscopic density functional studies of fission have previously concentrated on adiabatic approaches based on constrained static calculations…

Nuclear Theory · Physics 2016-02-03 P. M. Goddard , P. D. Stevenson , A. Rios

An iterative method we previously proposed to compute nuclear strength functions is developed to allow it to accurately calculate properties of individual nuclear states. The approach is based on the quasi-particle-random-phase…

Nuclear Theory · Physics 2015-06-04 B. G. Carlsson , J. Toivanen , A. Pastore

At present there are two vastly different ab initio approaches to the description of the the many-body dynamics: the Density Functional Theory (DFT) and the functional integral (path integral) approaches. On one hand, if implemented…

Nuclear Theory · Physics 2014-11-20 Aurel Bulgac