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Strong magnetic-ferroelectric coupling in hexagonal HoMnO3 has been observed previously at spin reorientation temperature between P6'3cm' and the P6'3cm' magnetic phases. In contrast, YMnO3 has only a single magnetic phase (P6'3cm') and no…

Strongly Correlated Electrons · Physics 2013-03-26 Jagath Gunasekera , Owen P. Vajk , Yuan Wang , Kevin Tarwater , Tom W. Heitmann

From low-temperature Synchrotron X-ray diffraction, a precise thermal characterization of octahedral distortions in single phase Ruddlesden-Popper Ca3Mn2O7 is performed. Highly sensitive close-steps temperature dependences of Mn-O-Mn bond…

Materials Science · Physics 2020-04-24 Pooja Sahlot , A. K. Sinha , A. M. Awasthi

The origin of the low-temperature ferromagnetic instability in YTiO3 driven by the interplay between lattice, orbital, spin, and charge degrees of freedom is on the background of lattice dynamics. We present a comprehensive study of…

Strongly Correlated Electrons · Physics 2022-02-16 N. N. Kovaleva , O. E. Kusmartseva , A. Maljuk

We demonstrate a new approach for directly measuring the ultrafast energy transfer between elec- trons and magnons, enabling us to track spin dynamics in an antiferromagnet (AFM). In multiferroic HoMnO3, optical photoexcitation creates hot…

Strongly Correlated Electrons · Physics 2016-10-05 P. Bowlan , S. A. Trugman , J. Bowlan , J. -X. Zhu , N. J. Hur , A. J. Taylor , D. A. Yarotski , R. P. Prasankumar

The enhancement of spin-phonon coupling in gadolinium filled double walled carbon nanotubes (GdCl3@DWNTs) is demonstrated through temperature dependent magnetrometry and polarized Raman Spectroscopy (PRS). Temperature dependent…

Mesoscale and Nanoscale Physics · Physics 2019-06-05 S. Ncube , R. Erasmus , S. Bhattacharyya

Polarized Raman-scattering spectra of non-superconducting, single-crystalline FeTe are investigated as function of temperature. We have found a relation between the magnitude of ordered magnetic moments and the linewidth of A1g phonons at…

Strongly Correlated Electrons · Physics 2015-05-27 V. Gnezdilov , Yu. Pashkevich , P. Lemmens , A. Gusev , K. Lamonova , I. Vitebskiy , O. Afanasiev , S. Gnatchenko , V. Tsurkan , J. Deisenhofer , A. Loidl

We utilize ultrafast photoexcitation to drive coherent lattice oscillations in the layered ferrimagnetic crystal Mn3Si2Te6, which significantly stiffen below the magnetic ordering temperature. We suggest that this is due to an…

We investigate the experimental signatures of Raman spectroscopy of bi- and tri-magnon excitations in the distorted triangular lattice antiferromagnets alpha-LCr2O4 (L=Sr, Ca). We utilize spin wave theory to analyze the nearly 120 degree…

Strongly Correlated Electrons · Physics 2023-05-23 Junli Li , Shangjian Jin , Trinanjan Datta , Dao-Xin Yao

We report the influence of Ce$^{3+}$ substitution on the magnetic structures and phonon dynamics in SmCrO$_3$ perovskites. Magnetic landscapes are spanned by long-range canted anti-ferromagnetism, AFM with Neel temperatures $\sim$196 K…

Materials Science · Physics 2025-12-30 Shaona Das , Ravi Kiran Dokala , Subhash Thota

We report the results of our investigation of the physical properties of mixed metal oxides RFe0.5Cr0.5O3 (R = Er and Yb). ErFe0.5Cr0.5O3 undergoes an antiferromagnetic ordering around 270 K followed by spin reorientation (SR) transitions…

Strongly Correlated Electrons · Physics 2020-07-15 Kavita Yadav , Gurpreet Kaur , Mohit K. Sharma , K. Mukherjee

We have used polarized Raman scattering to probe lattice vibrations and charge ordering in 12 nm thick, epitaxially strained PrNiO$_3$ films, and in superlattices of PrNiO$_3$ with the band-insulator PrAlO$_3$. A carefully adjusted confocal…

Strongly Correlated Electrons · Physics 2015-06-23 M. Hepting , M. Minola , A. Frano , G. Cristiani , G. Logvenov , E. Schierle , M. Wu , M. Bluschke , E. Weschke , H. U. Habermeier , E. Benckiser , M. Le Tacon , B. Keimer

Thermoelectric phenomena in magnetic materials present tantalizing possibilities for manipulating spin-information using heat in future 'spin caloritronic' devices. Key to unraveling their underlying physics is to understand spin-lattice…

The observation of strongly coupled lattice and spin dynamics in altermagnet CoF$_2$ is reported. On the background of the expected spin-phonon interaction leading to renormalization of all phonons at the Neel temperature an additional…

Materials Science · Physics 2024-05-14 M. A. Prosnikov , M. Bal , R. V. Pisarev , P. C. M. Christianen , A. M. Kalashnikova

The electronic valence state of Mn in Pb(Zr0.2Ti0.8)O3/La0.8Sr0.2MnO3 multiferroic heterostructures is probed by near edge x-ray absorption spectroscopy as a function of the ferroelectric polarization. We observe a temperature independent…

Materials Science · Physics 2010-04-13 C. A. F. Vaz , J. Hoffman , Y. Segal , J. W. Reiner , R. D. Grober , Z. Zhang , C. H. Ahn , F. J. Walker

We investigate spin dynamics in $\alpha$-Fe$_{2}$O$_{3}$/Ni$_{80}$Fe$_{20}$ (Py) heterostructures, uncovering a robust mechanism for in-situ modulation of ferromagnetic resonance (FMR) through precise control of temperature, applied…

Inelastic light scattering spectra of Bi_2Se_3 and Sb_2Te_3 single crystals have been measured over the temperature range from 5 K to 300 K. The temperature dependence of dominant A^{2}_{1g} phonons shows similar behavior in both materials.…

Lattice vibrations are highly sensitive to crystal symmetries and their changes across phase transitions. The latter can modify irreducible (co)representations and corresponding infrared and Raman selection rules of phonons. This concept is…

Micro-Raman spectroscopy has been used to study lattice dynamics associated with the ferroelectric domains of a BiFeO$_3$ single crystal at low temperature. The phonon assignment shows a large frequency splitting between the transverse and…

Strongly Correlated Electrons · Physics 2009-11-13 M. Cazayous , D. Malka , D. Lebeugle , D. Colson

In the quest of understanding significant variations in the physical, chemical and electronic properties of the novel functional materials, low temperature Synchrotron X-ray Diffraction (LT-SXRD) measurements on CTO (a type-II) and CMTO (a…

Materials Science · Physics 2016-08-09 Harishchandra Singh , A. K. Sinha , M. N. Singh , A. Upadhyay , Archna Sagdeo

We report on bifurcations effect mediated by the electron-phonon coupling in a concentrated rare-earth-containing antiferromagnet, observed in the spectra of coupled $4f$-electron-phonon modes under the influence of an external magnetic…