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The pyrochlore iridates R2Ir2O7 have emerged as a unique playground for exploring exotic quantum phenomena arising from the intricate interplay of strong spin-orbit coupling, electron correlations, and geometric frustration. While bulk…

Strongly Correlated Electrons · Physics 2026-05-27 Xiaoran Liu , Michael Terilli , Ana-Marija Nedic , Jiandong Guo , Jak Chakhalian

In this review we provide an introduction to the physics of a series of frustrated quantum rare-earth pyrochlores. We first give a background on the microscopic single- and two-ion physics of these materials, discussing the origins and…

Strongly Correlated Electrons · Physics 2019-03-26 Jeffrey G. Rau , Michel J. P. Gingras

The Tb$_2$Ti$_2$O$_7$ pyrochlore magnetic material is attracting much attention for its {\em spin liquid} state, failing to develop long range order down to 50 mK despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K. In this paper…

Statistical Mechanics · Physics 2007-05-23 Hamid R. Molavian , Michel J. P. Gingras , Benjamin Canals

While pyrochlore iridate thin films are theoretically predicted to possess a variety of emergent topological properties, experimental verification of these predictions can be obstructed by the challenge in thin film growth. Here we report…

AB$_2$O$_4$ normal spinels with a magnetic B site can host a variety of magnetic and orbital frustrations leading to spin-liquid phases and field-induced phase transitions. Here we report the first epitaxial growth of (111)-oriented…

Frustrated magnets can host numerous exotic many-body quantum and topological phenomena. GeNi$_2$O$_4$ is a three dimensional $S=1$ frustrated magnet with an unusual two-stage transition to the two-dimensional antiferromagnetic ground…

Strongly Correlated Electrons · Physics 2021-06-30 Denis M. Vasiukov , Mikhail Kareev , Fangdi Wen , Liang Wu , Padraic Shafer , Elke Arenholz , Xiaoran Liu , Jak Chakhalian

Topological quantum materials that show strongly correlated electrons as well as topological order, for which spin-orbit coupling is a key ingredient, exhibit novel states of matter. One such example is the family of pyrochlore iridates,…

Strongly Correlated Electrons · Physics 2025-01-14 Araceli Gutiérrez-Llorente

Minimizing the energy of a many body system tends to favor order, but classical frustration and quantum fluctuations destabilize that order. The tension between these effects can produce exotic quantum states of matter. Quantum spin liquid…

Strongly Correlated Electrons · Physics 2026-03-17 Sandesh S. Kalantre , Johanna Nordlander , Margaret A. Anderson , Julia A. Mundy , David Goldhaber-Gordon

The pyrochlore iridates have become ideal platforms to unravel fascinating correlated and topolog?ical phenomena that stem from the intricate interplay among strong spin-orbit coupling, electronic correlations, lattice with geometric…

A quantum spin liquid is a novel state of matter characterized by quantum entanglement and the absence of any broken symmetry. In condensed matter, the frustrated rare-earth pyrochlore magnets Ho$_2$Ti$_2$O$_7$ and Dy$_2$Ti$_2$O$_7$,…

Strongly Correlated Electrons · Physics 2017-04-05 E. Kermarrec , J. Gaudet , K. Fritsch , R. Khasanov , Z. Guguchia , C. Ritter , K. A. Ross , H. A. Dabkowska , B. D. Gaulin

We report on the emergent magnetic state of (111)-oriented CoCr2O4 ultrathin films sandwiched by Al2O3 in the quantum confined geometry. At the two-dimensional crossover, polarized neutron reflectometry reveals an anomalous enhancement of…

Strongly Correlated Electrons · Physics 2020-01-08 Xiaoran Liu , B. J. Kirby , Zhicheng Zhong , Yanwei Cao , B. Pal , M. Kareev , S. Middey , J. W. Freeland , P. Shafer , E. Arenholz , J. Chakhalian

The search for quantum spin liquids (QSL) -- topological magnets with fractionalized excitations -- has been a central theme in condensed matter and materials physics. While theories are no longer in short supply, tracking down materials…

Strongly Correlated Electrons · Physics 2022-05-11 Anish Bhardwaj , Shu Zhang , Han Yan , Roderich Moessner , Andriy H. Nevidomskyy , Hitesh J. Changlani

The pyrochlore compounds Ho2Ti2O7 and Dy2Ti2O7 show an exotic form of magnetism called the spin ice state, resulting from the interplay between geometrical frustration and ferromagnetic coupling. A fascinating feature of this state is the…

Materials Science · Physics 2013-09-11 D. P. Leusink , F. Coneri , M. Hoek , S. Turner , H. Idrissi , G. Van Tendeloo , H. Hilgenkamp

Quantum spin liquids (QSLs) are exotic phases of matter exhibiting long-range entanglement and supporting emergent gauge fields. A vigorous search for experimental realizations of these states has identified several materials with…

Strongly Correlated Electrons · Physics 2018-07-24 Owen Benton

While the spin ice state of bulk pyrochlores such as $\rm{Dy_2Ti_2O_7}$ and $\rm{Ho_2Ti_2O_7}$ has been extensively studied in the last several decades due to its unique degenerate ground state and emergent monopole excitation, whether it…

Actively shought since the turn of the century, two-dimensional quantum spin liquids (QSLs) are exotic phases of matter where magnetic moments remain disordered even at extremely low temperatures. Despite ongoing searches, QSLs remain…

Strongly Correlated Electrons · Physics 2015-07-22 Juan Carrasquilla , Zhihao Hao , Roger G. Melko

The existence of rich Fermiology in anomalous metal phase in exotic superconductors has attracted considerable interests, as exemplified in copper, iron-based, and intermetallic frustrated kagome-based compounds. A common feature in these…

Three-dimensionally (3D) frustrated magnets generally exist in the magnetic diamond and pyrochlore lattices, in which quantum fluctuations suppress magnetic orders and generate highly entangled ground states (GS). LiYbSe2 in a previously…

Strongly Correlated Electrons · Physics 2022-06-15 Ranuri S. Dissanayaka Mudiyanselage , Haozhe Wang , Olivia Vilella , Martin Mourigal , Gabriel Kotliar , Weiwei Xie

We highlight recent advances in the theory, materials fabrication, and experimental characterization of strongly correlated and topological states in [111] oriented transition metal oxide thin films and heterostructures, which are…

Strongly Correlated Electrons · Physics 2020-05-19 Jak Chakhalian , Xiaoran Liu , Gregory A. Fiete

Geometrical frustration among interacting spins combined with strong quantum fluctuations destabilize long-range magnetic order in favour of more exotic states such as spin liquids. By following this guiding principle, a number of spin…

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