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We perform a systematic {\it ab initio} study of the electronic structure of Sr(V,Mo,Mn)O$_3$ perovskites, using the parameter-free $GW$+EDMFT method. This approach self-consistently calculates effective interaction parameters, taking into…

Strongly Correlated Electrons · Physics 2020-02-26 Francesco Petocchi , Fredrik Nilsson , Ferdi Aryasetiawan , Philipp Werner

The cubic perovskite SrVO$_3$ is generally considered to be a prototype strongly correlated metal with a characteristic three-peak structure of the $d$-electron spectral function, featuring a renormalized quasiparticle band in between…

Strongly Correlated Electrons · Physics 2016-11-16 Lewin Boehnke , Fredrik Nilsson , Ferdi Aryasetiawan , Philipp Werner

We use angle-resolved photoemission to map the Fermi surface and quasiparticle dispersion of bulk-like thin films of SrMoO$_3$ grown by pulsed laser deposition. The electronic self-energy deduced from our data reveals weak to moderate…

First-principles density functional calculations are performed within the local density approximation to study the electronic properties of SrZrO$_3$, an insulating 4d-perovskite, in its high-temperature cubic phase, above 1400 K, as well…

Strongly Correlated Electrons · Physics 2007-05-23 E. Mete , R. Shaltaf , S. Ellialtioglu

The importance of electronic correlation effects in the layered perovskite Sr$_2$RuO$_4$ is evidenced. To this end we use state-of-the-art LDA+DMFT (Local Density Approximation + Dynamical Mean-Field Theory) in the basis of Wannier…

Strongly Correlated Electrons · Physics 2007-05-23 Z. V. Pchelkina , I. A. Nekrasov , Th. Pruschke , A. Sekiyama , S. Suga , V. I. Anisimov , D. Vollhardt

We investigate the electronic structure of a perovskite-type Pauli paramagnet SrMoO3 (t2g2) thin film using hard x-ray photoemission spectroscopy and compare the results to the realistic calculations that combine the density functional…

We investigate the electronic structure of highly conducting perovskite SrMoO$_{3}$ using valence band photoemission spectroscopy and electronic structure calculations. Large intensity corresponding to coherent feature close to Fermi level…

Strongly Correlated Electrons · Physics 2023-01-24 Asif Ali , B. H. Reddy , Ravi Shankar Singh

In this article, we review recent progress in angle-resolved photoemission (ARPES) studies of the Mott-Hubbard-type correlated electron systems SrVO3. It has the d1 electron configuration and is an ideal model compound to study electron…

Strongly Correlated Electrons · Physics 2016-08-31 T. Yoshida , M. Kobayashi , K. Yoshimatsu , H. Kumigashira , A. Fujimori

We use density functional theory methods to study the electronic structures of a series of $s-p$ cubic perovskites $ABX_{3}$: the experimentally available SrBiO$_{3}$, BaBiO$_{3}$, BaSbO$_3$, CsTlF$_{3}$, and CsTlCl$_{3}$, as well as the…

The multi-tier $GW$+EDMFT scheme is an ab-initio method for calculating the electronic structure of correlated materials. While the approach is free from ad-hoc parameters, it requires a selection of appropriate energy windows for…

Strongly Correlated Electrons · Physics 2024-08-15 Ruslan Mushkaev , Francesco Petocchi , Viktor Christiansson , Philipp Werner

The semi-metallic behavior of the perovskite iridate SrIrO3 shifts the end-member of the strongly spin-orbit (SO) coupled Ruddlesden-Popper series Srn+1IrnO3n+1 away from the Mott insulating regime and the half-filled pseudospin Jeff=1/2…

Strongly Correlated Electrons · Physics 2025-02-06 Dirk Fuchs , Arun Kumar Jaiswal , Fabrice Wilhelm , Di Wang , Andre Rogalev , Matthieu Le Tacon

Cubic perovskite oxides are emerging high-mobility transparent conducting oxides (TCOs), but Ge-based TCOs had not been known until the discovery of metastable cubic SrGeO$_3$. $0.5 \times 0.4 \times 0.2$-mm$^3$ large single crystals of the…

Photoemission spectra of the perovskites Ca$_x$Sr$_{1-x}$VO$_3$, Ca$_x$La$_{1-x}$VO$_3$, and SrRuO$_3$ indicate that Coulomb correlations are more pronounced at the surface than in the bulk. To investigate this effect we use the dynamical…

Strongly Correlated Electrons · Physics 2009-11-10 A. Liebsch

In a model system with three S=1 pseudo-spins situated in an anisotropic mean field we compute the thermodynamic response in a self consistent manner. An adhoc uniform broadening of all energy levels of the (localized) spins due to their…

Strongly Correlated Electrons · Physics 2015-10-19 Bellave Shivaram

The correlated electronic structure of SrVO3 has been investigated by angle-resolved photoemission spectroscopy using in-situ prepared thin films. Pronounced features of band renormalization have been observed: a sharp kink ~60 meV below…

Strongly Correlated Electrons · Physics 2012-12-11 S. Aizaki , T. Yoshida , K. Yoshimatsu , M. Takizawa , M. Minohara , S. Ideta , A. Fujimori , K. Gupta , P. Mahadevan , K. Horiba , H. Kumigashira , M. Oshima

In this study, we report a tetragonal perovskite structure of SrIrO$_3$ (P4/mmm, a = 3.9362(9) \r{A}, c = 7.880(3) \r{A}) synthesized at 6 GPa and 1400 $\deg$C, employing the ambient pressure monoclinic SrIrO$_3$ with distorted 6H structure…

The accurate ab-initio simulation of periodic solids with strong correlations is one of the grand challenges of condensed matter. While mature methods exist for weakly correlated solids, the ab-initio description of strongly correlated…

Strongly Correlated Electrons · Physics 2020-08-12 Sergei Iskakov , Chia-Nan Yeh , Emanuel Gull , Dominika Zgid

In this study, we investigate the structural properties, chemical stability, and electronic, optical, and thermoelectric properties of $\mathrm{Sr_2PrSbO_6}$ using first-principles calculations based on Density Functional Theory (DFT). The…

Materials Science · Physics 2025-10-22 Md. Mohiuddin , Alamgir Kabir

The two-dimensional layered perovskite Sr2IrO4 was proposed to be a spin-orbit Mott insulator, where the effect of Hubbard interaction is amplified on a narrow J_{eff} = 1/2 band due to strong spin-orbit coupling. On the other hand, the…

Strongly Correlated Electrons · Physics 2012-03-08 Jean-Michel Carter , V. Vijay Shankar , M. Ahsan Zeb , Hae-Young Kee

We investigated the electronic properties of epitaxially stabilized perovskite SrIrO3 and demonstrated the effective strain-control on its electronic structure. Comprehensive transport measurements showed that the strong spin-orbit coupling…

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