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We demonstrate via a muon spin rotation experiment that the electronic ground state of the iridium spinel compound, CuIr$_2$S$_4$, is not the presumed spin-singlet state but a novel paramagnetic state, showing a quasistatic spin glass-like…

Strongly Correlated Electrons · Physics 2014-02-27 K. M. Kojima , 2 R. Kadono , M. Miyazaki , M. Hiraishi , I. Yamauchi , A. Koda , Y. Tsuchiya , H. S. Suzuki , H. Kitazawa

Spinel ferrites in general show a rich interplay of structural, electronic, and magnetic properties. Here, we particularly focus on zinc ferrite (ZFO), which has been observed experimentally to crystallise in the cubic $normal$ spinel…

Materials Science · Physics 2018-10-26 Daniel Fritsch

Single-phase Mg-doped ZnFe$_2$O$_4$ nanoparticles with x= 0, 0.3, 0.5, 0.7 have been prepared by the glycol-thermal method without any subsequent calcination. The crystallite size, microstructure and magnetic properties of the prepared…

Materials Science · Physics 2025-08-20 Kemi Y. Adewale , Itegbeyogene P. Ezekiel

The structural, magnetic, and electronic properties of NdFe$_{0.5}$Mn$_{0.5}$O$_3$ have been studied in detail using bulk magnetization, neutron/x-ray diffraction and first principles density functional theory calculations. The material…

Strongly Correlated Electrons · Physics 2017-10-25 Ankita Singh , A. Jain , Avijeet Ray , B. Padmanabhan , S. M. Yusuf , T. Maitra , V. K. Malik

We investigate magnetic properties of the $s$ = 1/2 compound K$_{2}$Cu$_{3}$(MoO$_{4}$)$_{4}$ by combining magnetic susceptibility, magnetization, specific heat, and electron spin resonance (ESR) with density functional calculations. Its…

Complex magneto structural behaviour of rare rich intermetallic Tb$_3$Co is reported in this study. Below the 84K (T$_N$), it undergoes a first order magnetic transition 72K confirmed from specific heat and magnetization measurements.…

Materials Science · Physics 2019-08-23 Srikanta Goswami , P. D. Babu , R. Rawat

LiCu$_3$O$_3$ is a novel 2D S=1/2 antiferromagnet with randomly depleted square lattice. The crystal structure contains two types of square planes with different Cu$^{2+}\rightarrow$ Li$^{+}$ substitution rates (20% and 40%). $^7$Li NMR and…

Strongly Correlated Electrons · Physics 2024-09-09 A. A. Bush , S. K. Gotovko , V. Yu. Ivanov , V. I. Kozlov , E. G. Nikolaev , L. E. Svistov

We have performed Electron Spin Resonance measurements on single crystals of the doped spin-Peierls compounds CuGe$_{1-y}$Si$_y$O$_3$ and Cu$_{1-x}$M$_x$GeO$_3$ with M = Zn, Mg, Ni ($x, y\leq 0.1$). The first part of our experiments was…

Strongly Correlated Electrons · Physics 2009-11-07 B. Grenier , P. Monod , M. Hagiwara , M. Matsuda , K. Katsumata , S. Clément , J. -P. Renard , A. L. Barra , G. Dhalenne , A. Revcolevschi

The experimental studies of the paramagnetic-antiferromagnetic phase transition through M\"{o}ssbauer spectroscopy and measurements of temperature and field dependencies of magnetic susceptibility in the layered Cu$_{0.15}$Fe$_{0.85}$PS$_3$…

Computational Physics · Physics 2023-01-05 V. Pashchenko , O. Bludov , D. Baltrunas , K. Mazeika , S. Motria , K. Glukhov , Yu. Vysochanskii

Recent experiments on Mn doped multiferroic $CoCr_{2}O_{4}$ indicate that a possible distribution of Mn atoms among tetrahedrally and octahedrally coordinated sites in the spinel lattice give rise to different variations in the structural…

Materials Science · Physics 2017-01-04 Debashish Das , Subhradip Ghosh

To study the relationship between the properties of low-dimensional spin systems with weakly coupled Cu-triangles and their crystal structure, single crystals of $Cs_3Cu_3Cl_8OH$ (1) and the new $Cs_3Cu_3Cl_{7.6}Br_{0.4}OH$ (2) were grown.…

Muon spin relaxation measurements are reported on samples of dimethylammonium metal formates containing magnetic divalent nickel, cobalt, manganese, and copper ions. These hybrid organic-inorganic perovskites exhibit weak ferromagnetism and…

Strongly Correlated Electrons · Physics 2015-05-19 P. J. Baker , T. Lancaster , I. Franke , W. Hayes , S. J. Blundell , F. L. Pratt , P. Jain , Z. -M. Wang , M. Kurmoo

The crystal and magnetic structures of stoichiometric ZnCr2Se4 have been investigated using synchrotron X-ray and neutron powder diffraction, muon spin relaxation (muSR) and inelastic neutron scattering. Synchrotron X-ray diffraction shows…

Strongly Correlated Electrons · Physics 2017-04-12 P. Zajdel , W-Y. Li , W. Van Beek , A. Lappas , A. Ziolkowska , S. Jaskiewicz , C. Stock , M. A. Green

We report magnetization, nuclear magnetic resonance (NMR), nuclear quadrupole resonance (NQR), and transmission electron microscopy (TEM) studies on the quasi-two-dimensional spin-gap system (CuCl)LaNb2O7, a possible candidate for the J1-J2…

Strongly Correlated Electrons · Physics 2017-12-01 M. Yoshida , N. Ogata , M. Takigawa , J. Yamaura , M. Ichihara , T. Kitano , H. Kageyama , Y. Ajiro , K. Yoshimura

In frustrated spinel antiferromagnets, dilution with non-magnetic ions can be a powerful strategy for probing unconventional spin states or uncovering interesting phenomena. Here, we present X-ray, neutron scattering and thermodynamic…

Strongly Correlated Electrons · Physics 2018-06-20 A. V. Zakrzewski , S. Gangopadhyay , A. A. Aczel , S. Calder , T. J. Williams , G. J. MacDougall

The A-site spinel material, CoAl2O4, is a physical realization of the frustrated diamond-lattice antiferromagnet, a model in which is predicted to contain unique incommensurate or `spin-spiral liquid' ground states. Our previous…

We investigated the crystal and magnetic structures of the spin-1/2 frustrated antiferromagnet Cu3Mo2O9 in which the spin system consists of antiferromagnetic chains and dimers. The space group at room temperature has been reported to be…

LiV$_2$O$_4$ spinel is known to exhibit heavy fermion-like behavior below a characteristic temperature $T_K\simeq 20$ K, while it preserves a paramagnetic state down to $T\sim10^{-2}$ K due to geometrical frustration. Here, it is shown that…

Strongly Correlated Electrons · Physics 2019-01-23 H. Okabe , M. Hiraishi , A. Koda , K. M. Kojima , S. Takeshita , I. Yamauchi , Y. Matsushita , Y. Kuramoto , R. Kadono

We report the results of magnetic susceptibility $\chi$ and $^1$H nuclear magnetic resonance (NMR) measurements on a three-dimensional hyper-honeycomb lattice compound [(C$_2$H$_5$)$_3$NH]$_2$Cu$_2$(C$_2$O$_4$)$_3$ (CCCO). The average value…

Strongly Correlated Electrons · Physics 2022-03-29 Q. -P. Ding , C. Dissanayake , Santanu Pakhira , W. J. Newsome , F. Uribe-Romo , D. C. Johnston , Y. Nakajima , Y. Furukawa

We report our nuclear magnetic resonance (NMR) study on the structurally spin chain compound Ni$_2$NbBO$_6$ with complex magnetic coupling. The antiferromagnetic transition is monitored by the line splitting resulting from the staggered…

Strongly Correlated Electrons · Physics 2021-07-16 K. Y. Zeng , Long Ma , L. M. Xu , Z. M. Tian , L. S. Ling , Li Pi