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Monolayer transition metal dichalcogenides host a variety of optically excited quasiparticles species that stem from two-dimensional confinement combined with relatively large carrier effective masses and reduced dielectric screening. The…

Boron nitride single layer belongs to the family of 2D materials whose optical properties are currently receiving considerable attention. Strong excitonic effects have already been observed in the bulk and still stronger effects are…

Electron irradiation-induced damage is often the limiting factor in imaging materials prone to ionization or electronic excitations due to inelastic electron scattering. Quantifying the related processes at the atomic scale has only become…

Heterostructures made from 2D transition-metal dichalcogenides are known as ideal platforms to explore excitonic phenomena ranging from correlated moir\'e excitons to degenerate interlayer exciton ensembles. So far, it is assumed that the…

Recent experiments have realized exciton condensation in bilayer materials such as graphene double layers and the van der Waals heterostructure MoSe$_2$-WSe$_2$ with the potential for nearly frictionless energy transport. Here we…

Mesoscale and Nanoscale Physics · Physics 2024-11-06 Lillian I. Payne Torres , Anna O. Schouten , David A. Mazziotti

The strong Coulomb forces in monolayer transition metal dichalcogenides ensure that optical excitation of band electrons gives rise to Wannier-Mott excitonic states, each of which can be conceptualized as a composite of a Gaussian…

Mesoscale and Nanoscale Physics · Physics 2019-10-16 Eric Chatterjee , Daniel B. S. Soh , Christopher Rogers , Dodd J. Gray , Hideo Mabuchi

Long-lived interlayer excitons with distinct spin-valley physics in van der Waals heterostructures based on transition metal dichalcogenides make them promising for information processing in next-generation devices. While the emission…

Mesoscale and Nanoscale Physics · Physics 2021-10-18 Alberto Ciarrocchi , Dmitrii Unuchek , Ahmet Avsar , Kenji Watanabe , Takashi Taniguchi , Andras Kis

Defects in conventional semiconductors substantially lower the photoluminescence (PL) quantum yield (QY), a key metric of optoelectronic performance that directly dictates the maximum device efficiency. Two-dimensional (2D) transition metal…

The predicted formation of moire superlattices leading to confined excitonic states in heterostructures formed by stacking two lattice mismatched transition metal dichalcogenide (TMD) monolayers was recently experimentally confirmed. Such…

Single quantum emitters (SQEs) are at the heart of quantum optics and photonic quantum information technologies. To date, all demonstrated solid-state single-photon sources are confined in three-dimensional materials. Here, we report a new…

Mesoscale and Nanoscale Physics · Physics 2014-11-11 Yu-Ming He , G. Clark , J. R. Schaibley , Yu He , M. -C. Chen , Y. -J. Wei , X. Ding , Qiang Zhang , Wang Yao , Xiaodong Xu , Chao-Yang Lu , Jian-Wei Pan

We examine a mechanism by which excitons undergo ultrafast relaxation in common monolayer transition metal dichalcogenides. It is shown that at densities $\approx$ 1$\times$ 10$^{11}$ cm$^{-2}$ and temperatures $ \le 60$ K, excitons in well…

Mesoscale and Nanoscale Physics · Physics 2016-06-29 A. Thilagam

The layer dependent structural, electronic and vibrational properties of SnS2 and SnSe2 are investigated using first-principles density functional theory (DFT). The in-plane lattice constants, interlayer distances and binding energies are…

Materials Science · Physics 2016-10-05 Joseph M. Gonzalez , Ivan I. Oleynik

Atomically flat semiconducting materials such as monolayer WSe$_2$ hold great promise for novel optoelectronic devices. Recently, quantum light emission has been observed from bound excitons in exfoliated WSe$_2$. As part of developing…

Mesoscale and Nanoscale Physics · Physics 2018-07-10 L. C. Flatten , L. Weng , A. Branny , S. Johnson , P. R. Dolan , A. A. P. Trichet , B. D. Gerardot , J. M. Smith

The exciton dynamics in monolayer black phosphorus is investigated over a very wide range of photoexcited exciton densities using time resolved photoluminescence. At low excitation densities, the exciton dynamics is successfully described…

Mesoscale and Nanoscale Physics · Physics 2016-08-30 A. Surrente , A. A. Mitioglu , K. Galkowski , L. Klopotowski , W. Tabis , B. Vignolle , D. K. Maude , P. Plochocka

The Landau quantization space is based on the respective motion of the electron and hole in a magnetic field and can provide a new route to understand the bound exciton behaviors observed in the experiments. In this paper, we study the…

Mesoscale and Nanoscale Physics · Physics 2026-03-26 Kunxiang Li , Yi-Xiang Wang

It has recently been shown that quantum-confined states can appear in epitaxially grown van der Waals material heterobilayers without a rotational misalignment ($\theta=0^\circ$), associated with flat bands in the Brillouin zone of the…

We perform coherent nonlinear spectroscopy of excitons in single-layers of MoSe$_2$ and WSe$_2$ encapsulated between thin films of hexagonal boron nitride. Employing four-wave mixing microscopy we identify virtually disorder free areas,…

A very long lifetime emission with non-single exponential decay characteristic has been reported for single InAs/GaAs quantum dot (QD) samples, in which there exists a long-lived metastable state in the wetting layer (WL) [ACS Photonics…

We have experimentally determined the energies of the ground and first four excited excitonic states of the fundamental optical transition in monolayer WS2, a model system for the growing class of atomically thin two-dimensional…

Large-area and high-quality single-layer transition metal dichalcogenides can be synthesized by epitaxial growth on single-crystal substrates. An important advantage of this approach is that the interaction between the single-layer and the…