Related papers: Characterizing multielectron dynamics during recol…
We numerically investigate attosecond streaking time delays in the photoemission of valence and 2p core electrons of aluminum surface. We find that electron emission from the core level band is delayed by $\Delta \tau =100$ attoseconds…
Intense light with frequencies above typical atomic or molecular ionization potentials as provided by free-electron lasers couples many photons into extended targets such as clusters and biomolecules. This implies, in contrast to…
Laser pulses with stable electric field waveforms establish the opportunity to achieve coherent control on attosecond timescales. We present experimental and theoretical results on the steering of electronic motion in a multi-electron…
Electrons in atoms and molecules can not react immediately to the action of intense laser field. A time lag (about 100 attoseconds) between instants of the field maximum and the ionization-rate maximum emerges. This lag characterizes the…
A great deal of theoretical and experimental efforts have been devoted in the last decades to the study of long-wavelength photodetection mechanisms in field-effect transistors hosting two-dimensional (2D) electron systems. A particularly…
Strong-field physics is currently experiencing a shift towards the use of mid-IR driving wavelengths. This is because they permit conducting experiments unambiguously in the quasi-static regime and enable exploiting the effects related to…
A novel technique to sensitively and selectively isolate multiple-quantum coherences in a femtosecond pump-probe setup is presented. Detecting incoherent observables and imparting lock-in amplification, even weak signals of highly dilute…
We investigate the rates for multielectron recombination within a dense plasma environment in local thermodynamic equilibrium (LTE). We find that these multielectron recombination rates can be high within dense plasmas, and they should be…
We study laser-assisted photodetachment time delays by attosecond pulse trains from the closed-shell negative ions F- and Cl-. We investigate the separability of the delay into two contributions: (i) the Wigner-like delay associated with…
Dissipation of electromagnetic energy through absorption is a fundamental process that underpins phenomena ranging from photovoltaics to photography, analytical spectroscopy, photosynthesis, and human vision. Absorption is also a dynamic…
This tutorial presents an introduction to the interaction of light and matter on the attosecond timescale. Our aim is to detail the theoretical description of ultra-short time-delays, and to relate these to the phase of extreme ultraviolet…
Time-resolved photoemission experiments can reveal fascinating quantum dynamics of correlated electrons. However, the thermalization of the electronic system is typically so fast that very short probe pulses are necessary to resolve the…
The use of ultrafast pump-probe conductivity (PPC) for studies of photoelectron dynamics in nonpolar molecular liquids has been based upon the perturbation of geminate recombination dynamics of trapped electrons by their laser…
Two oppositely charged particles created within a microscopic space-time region can be separated, accelerated over a much larger distance, and brought to a recollision by a laser field. Consequently, new reactions become feasible, where the…
We theoretically propose a multidimensional high-harmonic echo spectroscopy technique which utilizes strong optical fields to resolve coherent electron dynamics spanning an energy range of multiple electron Volts. Using our recently…
Photoelectron spectroscopy earlier probed oscillations in C60 valence emissions, producing series of minima whose energy separation depends on the molecular cavity. We show here that the quantum phase at these cavity minima exhibits…
Radiative double electron capture (RDEC), the one-step process occurring in ion-atom collisions, has been investigated for bare fluorine ions colliding with carbon. RDEC is completed when two target electrons are captured to a bound state…
Current advances in ultrafast electron microscopy make it possible to combine optical pumping of a nanostructure and electron beam probing with sub{\aa}ngstrom and femtosecond spatiotemporal resolution. We present a theory predicting that…
We investigate theoretically the relative time delay of photoelectrons originating from different atomic subshells of noble gases. This quantity was measured via attosecond streaking and studied theoretically by Schultze et al. [Science…
We present calculations for attosecond atomic delays in photoionization of noble gas atoms based on full two-color two-photon Random-Phase Approximation with Exchange in both length and velocity gauge. Gauge invariant atomic delays are…